Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study
By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Liu, Xiaohan [verfasserIn] Song, Meng [verfasserIn] Wang, Hongzhen [verfasserIn] Chen, Shihao [verfasserIn] Zheng, Wei [verfasserIn] Wang, Xiujuan [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023 |
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| Schlagwörter: |
Polymer-matrix composites (PMCs) |
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| Übergeordnetes Werk: |
Enthalten in: Composites science and technology - Amsterdam [u.a.] : Elsevier, 1985, 240 |
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| Übergeordnetes Werk: |
volume:240 |
| DOI / URN: |
10.1016/j.compscitech.2023.110083 |
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| Katalog-ID: |
ELV010334858 |
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| 520 | |a By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. | ||
| 650 | 4 | |a Polymer-matrix composites (PMCs) | |
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| 700 | 1 | |a Zheng, Wei |e verfasserin |4 aut | |
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10.1016/j.compscitech.2023.110083 doi (DE-627)ELV010334858 (ELSEVIER)S0266-3538(23)00176-8 DE-627 ger DE-627 rda eng 660 670 VZ 51.75 bkl Liu, Xiaohan verfasserin aut Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. Polymer-matrix composites (PMCs) Graphene and other 2D-materials Molecular dynamics Damping response Song, Meng verfasserin aut Wang, Hongzhen verfasserin aut Chen, Shihao verfasserin aut Zheng, Wei verfasserin aut Wang, Xiujuan verfasserin (orcid)0000-0003-4007-797X aut Enthalten in Composites science and technology Amsterdam [u.a.] : Elsevier, 1985 240 Online-Ressource (DE-627)320509095 (DE-600)2013182-3 (DE-576)098330314 1879-1050 nnns volume:240 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.75 Verbundwerkstoffe Schichtstoffe VZ AR 240 |
| spelling |
10.1016/j.compscitech.2023.110083 doi (DE-627)ELV010334858 (ELSEVIER)S0266-3538(23)00176-8 DE-627 ger DE-627 rda eng 660 670 VZ 51.75 bkl Liu, Xiaohan verfasserin aut Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. Polymer-matrix composites (PMCs) Graphene and other 2D-materials Molecular dynamics Damping response Song, Meng verfasserin aut Wang, Hongzhen verfasserin aut Chen, Shihao verfasserin aut Zheng, Wei verfasserin aut Wang, Xiujuan verfasserin (orcid)0000-0003-4007-797X aut Enthalten in Composites science and technology Amsterdam [u.a.] : Elsevier, 1985 240 Online-Ressource (DE-627)320509095 (DE-600)2013182-3 (DE-576)098330314 1879-1050 nnns volume:240 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.75 Verbundwerkstoffe Schichtstoffe VZ AR 240 |
| allfields_unstemmed |
10.1016/j.compscitech.2023.110083 doi (DE-627)ELV010334858 (ELSEVIER)S0266-3538(23)00176-8 DE-627 ger DE-627 rda eng 660 670 VZ 51.75 bkl Liu, Xiaohan verfasserin aut Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. Polymer-matrix composites (PMCs) Graphene and other 2D-materials Molecular dynamics Damping response Song, Meng verfasserin aut Wang, Hongzhen verfasserin aut Chen, Shihao verfasserin aut Zheng, Wei verfasserin aut Wang, Xiujuan verfasserin (orcid)0000-0003-4007-797X aut Enthalten in Composites science and technology Amsterdam [u.a.] : Elsevier, 1985 240 Online-Ressource (DE-627)320509095 (DE-600)2013182-3 (DE-576)098330314 1879-1050 nnns volume:240 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.75 Verbundwerkstoffe Schichtstoffe VZ AR 240 |
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10.1016/j.compscitech.2023.110083 doi (DE-627)ELV010334858 (ELSEVIER)S0266-3538(23)00176-8 DE-627 ger DE-627 rda eng 660 670 VZ 51.75 bkl Liu, Xiaohan verfasserin aut Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. Polymer-matrix composites (PMCs) Graphene and other 2D-materials Molecular dynamics Damping response Song, Meng verfasserin aut Wang, Hongzhen verfasserin aut Chen, Shihao verfasserin aut Zheng, Wei verfasserin aut Wang, Xiujuan verfasserin (orcid)0000-0003-4007-797X aut Enthalten in Composites science and technology Amsterdam [u.a.] : Elsevier, 1985 240 Online-Ressource (DE-627)320509095 (DE-600)2013182-3 (DE-576)098330314 1879-1050 nnns volume:240 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.75 Verbundwerkstoffe Schichtstoffe VZ AR 240 |
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10.1016/j.compscitech.2023.110083 doi (DE-627)ELV010334858 (ELSEVIER)S0266-3538(23)00176-8 DE-627 ger DE-627 rda eng 660 670 VZ 51.75 bkl Liu, Xiaohan verfasserin aut Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. Polymer-matrix composites (PMCs) Graphene and other 2D-materials Molecular dynamics Damping response Song, Meng verfasserin aut Wang, Hongzhen verfasserin aut Chen, Shihao verfasserin aut Zheng, Wei verfasserin aut Wang, Xiujuan verfasserin (orcid)0000-0003-4007-797X aut Enthalten in Composites science and technology Amsterdam [u.a.] : Elsevier, 1985 240 Online-Ressource (DE-627)320509095 (DE-600)2013182-3 (DE-576)098330314 1879-1050 nnns volume:240 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.75 Verbundwerkstoffe Schichtstoffe VZ AR 240 |
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Liu, Xiaohan @@aut@@ Song, Meng @@aut@@ Wang, Hongzhen @@aut@@ Chen, Shihao @@aut@@ Zheng, Wei @@aut@@ Wang, Xiujuan @@aut@@ |
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Liu, Xiaohan |
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Liu, Xiaohan ddc 660 bkl 51.75 misc Polymer-matrix composites (PMCs) misc Graphene and other 2D-materials misc Molecular dynamics misc Damping response Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study |
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660 670 VZ 51.75 bkl Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study Polymer-matrix composites (PMCs) Graphene and other 2D-materials Molecular dynamics Damping response |
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hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: molecular simulation and experimental study |
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Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study |
| abstract |
By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. |
| abstractGer |
By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. |
| abstract_unstemmed |
By combining molecular dynamics (MD) simulation and experiments, this work describes a systematic, quantitative study on the nanoscale damping of nitrile butadiene rubber (NBR) by adding graphene oxide (GO) with different oxidation degrees. Using MD simulation, the proposed two-component solubility parameters predict that GO2 (O wt %, 17.05%) and NBR have excellent thermodynamic compatibility. GO2/NBR system shows the largest molar concentration of intermolecular hydrogen bonds and the lowest free volume fraction and mean square displacement. GO2 presents a strong adsorption effect on NBR polymer chains. Meanwhile, the green preparation method of reduced graphene oxide has been developed for improving damping properties of reduced graphene oxide/nitrile butadiene rubber (RGO/NBR) composites. The prepared RGO/NBR composites with tailor-made oxidation degrees are adopted to validate the theoretical prediction by MD simulation. Fourier transform infrared spectroscopy verifies that hydrogen bond networks exist between GO and NBR polymer chains. Two main factors, the number of intermolecular hydrogen bonds and the degree of wrinkles of GO sheets dominate the damping performance of the composites. The results indicate that when the GO oxidation degree is about 17.05%, the damping capability of GO/NBR composites is maximum improved. These results pave the way for the environmentally modifying interface to design high performance GO/rubber composites. |
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Hydrogen bond networks and wrinkles in graphene oxide/nitrile butadiene rubber composites for enhancement of damping capability: Molecular simulation and experimental study |
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|
| score |
7.4000015 |