Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity

Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles w...
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Gespeichert in:

Autor*in:	Li, Yan [verfasserIn] Chen, Guangyu [verfasserIn] Wu, Hualong [verfasserIn] Ding, Helei [verfasserIn] zhang, Chentong [verfasserIn] Huang, Liuqing [verfasserIn] Luo, Xuetao [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Volatile silicon waste Anode ALD ZnO Carbon coating Lithium-ion battery

Übergeordnetes Werk:	Enthalten in: Applied surface science - Amsterdam : Elsevier, 1985, 634
Übergeordnetes Werk:	volume:634

DOI / URN:	10.1016/j.apsusc.2023.157651

Katalog-ID:	ELV010336192

Internformat


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245	1	0	\|a Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity
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520			\|a Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste.
650		4	\|a Volatile silicon waste
650		4	\|a Anode
650		4	\|a ALD ZnO
650		4	\|a Carbon coating
650		4	\|a Lithium-ion battery
700	1		\|a Chen, Guangyu \|e verfasserin \|4 aut
700	1		\|a Wu, Hualong \|e verfasserin \|4 aut
700	1		\|a Ding, Helei \|e verfasserin \|4 aut
700	1		\|a zhang, Chentong \|e verfasserin \|4 aut
700	1		\|a Huang, Liuqing \|e verfasserin \|4 aut
700	1		\|a Luo, Xuetao \|e verfasserin \|0 (orcid)0000-0002-7608-2386 \|4 aut
773	0	8	\|i Enthalten in \|t Applied surface science \|d Amsterdam : Elsevier, 1985 \|g 634 \|h Online-Ressource \|w (DE-627)312151128 \|w (DE-600)2002520-8 \|w (DE-576)094476985 \|7 nnns
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912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
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912			\|a GBV_ILN_4323
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936	b	k	\|a 52.78 \|j Oberflächentechnik \|j Wärmebehandlung \|q VZ
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Indexfelder

author_variant	y l yl g c gc h w hw h d hd c z cz l h lh x l xl
matchkey_str	liyanchenguangyuwuhualongdingheleizhangc:2023----:osrcigrpertcessozoaoeeiefovltlslcnatfrn
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publishDate	2023
allfields	10.1016/j.apsusc.2023.157651 doi (DE-627)ELV010336192 (ELSEVIER)S0169-4332(23)01330-2 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Li, Yan verfasserin aut Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste. Volatile silicon waste Anode ALD ZnO Carbon coating Lithium-ion battery Chen, Guangyu verfasserin aut Wu, Hualong verfasserin aut Ding, Helei verfasserin aut zhang, Chentong verfasserin aut Huang, Liuqing verfasserin aut Luo, Xuetao verfasserin (orcid)0000-0002-7608-2386 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 634 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:634 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 634
spelling	10.1016/j.apsusc.2023.157651 doi (DE-627)ELV010336192 (ELSEVIER)S0169-4332(23)01330-2 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Li, Yan verfasserin aut Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste. Volatile silicon waste Anode ALD ZnO Carbon coating Lithium-ion battery Chen, Guangyu verfasserin aut Wu, Hualong verfasserin aut Ding, Helei verfasserin aut zhang, Chentong verfasserin aut Huang, Liuqing verfasserin aut Luo, Xuetao verfasserin (orcid)0000-0002-7608-2386 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 634 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:634 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 634
allfields_unstemmed	10.1016/j.apsusc.2023.157651 doi (DE-627)ELV010336192 (ELSEVIER)S0169-4332(23)01330-2 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Li, Yan verfasserin aut Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste. Volatile silicon waste Anode ALD ZnO Carbon coating Lithium-ion battery Chen, Guangyu verfasserin aut Wu, Hualong verfasserin aut Ding, Helei verfasserin aut zhang, Chentong verfasserin aut Huang, Liuqing verfasserin aut Luo, Xuetao verfasserin (orcid)0000-0002-7608-2386 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 634 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:634 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 634
allfieldsGer	10.1016/j.apsusc.2023.157651 doi (DE-627)ELV010336192 (ELSEVIER)S0169-4332(23)01330-2 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Li, Yan verfasserin aut Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste. Volatile silicon waste Anode ALD ZnO Carbon coating Lithium-ion battery Chen, Guangyu verfasserin aut Wu, Hualong verfasserin aut Ding, Helei verfasserin aut zhang, Chentong verfasserin aut Huang, Liuqing verfasserin aut Luo, Xuetao verfasserin (orcid)0000-0002-7608-2386 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 634 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:634 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 634
allfieldsSound	10.1016/j.apsusc.2023.157651 doi (DE-627)ELV010336192 (ELSEVIER)S0169-4332(23)01330-2 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Li, Yan verfasserin aut Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste. Volatile silicon waste Anode ALD ZnO Carbon coating Lithium-ion battery Chen, Guangyu verfasserin aut Wu, Hualong verfasserin aut Ding, Helei verfasserin aut zhang, Chentong verfasserin aut Huang, Liuqing verfasserin aut Luo, Xuetao verfasserin (orcid)0000-0002-7608-2386 aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 634 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:634 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 634
language	English
source	Enthalten in Applied surface science 634 volume:634
sourceStr	Enthalten in Applied surface science 634 volume:634
format_phy_str_mv	Article
bklname	Oberflächen Dünne Schichten Grenzflächen Kolloidchemie Grenzflächenchemie Oberflächentechnik Wärmebehandlung
institution	findex.gbv.de
topic_facet	Volatile silicon waste Anode ALD ZnO Carbon coating Lithium-ion battery
dewey-raw	670
isfreeaccess_bool	false
container_title	Applied surface science
authorswithroles_txt_mv	Li, Yan @@aut@@ Chen, Guangyu @@aut@@ Wu, Hualong @@aut@@ Ding, Helei @@aut@@ zhang, Chentong @@aut@@ Huang, Liuqing @@aut@@ Luo, Xuetao @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	312151128
dewey-sort	3670
id	ELV010336192
language_de	englisch
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author	Li, Yan
spellingShingle	Li, Yan ddc 670 bkl 33.68 bkl 35.18 bkl 52.78 misc Volatile silicon waste misc Anode misc ALD ZnO misc Carbon coating misc Lithium-ion battery Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity
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topic_title	670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity Volatile silicon waste Anode ALD ZnO Carbon coating Lithium-ion battery
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title	Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity
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title_full	Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity
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title_sort	constructing triple-protected si/sioxzno@c anode derived from volatile silicon waste for enhanced lithium storage capacity
title_auth	Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity
abstract	Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste.
abstractGer	Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste.
abstract_unstemmed	Silicon anode is deemed to be one of the most promising anode materials and has attracted wide attention from all walks of life. However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. This work not only opens a novel and economic strategy for the manufacture of high-performance silicon-based anode but also furnishes an original approach for recycling and resource utilization of silicon waste.
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title_short	Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity
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However, its commercial application is severely limited owing to the high cost, serious volume expansion, and poor electrical conductivity. Herein, Si/SiOx nanoparticles were successfully prepared by sand milling the low-cost volatile deposited silicon waste from electron beam refining polycrystalline silicon. Furthermore, the atomic layer deposited (ALD) zine oxide on Si/SiOx nanoparticles enhances the integrity of the electrode structure and provides a steady solid electrolyte layer (SEI). The outer layer is wrapped by a uniform carbon shell to restrict the volume expansion and boost the conductivity of the electrode during lithiation/delithiation. Impressively, lithium-ion batteries (LIBs) employing the Si/SiOxZnO@C anodes display excellent rate performance (up to 844.48 mAh g−1 at 2 A g−1) and cycle stability (912.7 mAh g−1 at 1A g−1 over 50 cycles). Moreover, the Si/SiOx@ZnO@C electrode exhibits high initial coulombic efficiency (76.8 %) and the reversible specific capacity maintains at 846 mAh g−1 over 200 cycles with a current density at 0.5 A g−1. The improvement is ascribed to the synergistic effect of triple-protected layer that effectively enhances the stability of SEI and the conductivity of the electrode. 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Constructing triple-protected Si/SiOxZnO@C anode derived from volatile silicon waste for enhanced lithium storage capacity

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