Comparative study of the catalytic

The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could p...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Gao, Xiong [verfasserIn] Zhou, Zhen [verfasserIn] Wang, Jiawei [verfasserIn] Tian, Hong [verfasserIn] Qing, Mengxia [verfasserIn] Jiang, Liyang [verfasserIn] Cheng, Yi [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Polypropylene Catalytic co-pyrolysis Hydrocarbons Synergistic effects

Übergeordnetes Werk:	Enthalten in: Fuel processing technology - New York, NY [u.a.] : Science Direct, 1977, 241
Übergeordnetes Werk:	volume:241

DOI / URN:	10.1016/j.fuproc.2022.107520

Katalog-ID:	ELV01058692X

Internformat


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520			\|a The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%).
650		4	\|a Polypropylene
650		4	\|a Catalytic co-pyrolysis
650		4	\|a Hydrocarbons
650		4	\|a Synergistic effects
700	1		\|a Zhou, Zhen \|e verfasserin \|4 aut
700	1		\|a Wang, Jiawei \|e verfasserin \|4 aut
700	1		\|a Tian, Hong \|e verfasserin \|4 aut
700	1		\|a Qing, Mengxia \|e verfasserin \|4 aut
700	1		\|a Jiang, Liyang \|e verfasserin \|4 aut
700	1		\|a Cheng, Yi \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t Fuel processing technology \|d New York, NY [u.a.] : Science Direct, 1977 \|g 241 \|h Online-Ressource \|w (DE-627)300898681 \|w (DE-600)1483666-X \|w (DE-576)09618860X \|7 nnns
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912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2065
912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2088
912			\|a GBV_ILN_2106
912			\|a GBV_ILN_2110
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912			\|a GBV_ILN_2152
912			\|a GBV_ILN_2153
912			\|a GBV_ILN_2190
912			\|a GBV_ILN_2232
912			\|a GBV_ILN_2336
912			\|a GBV_ILN_2470
912			\|a GBV_ILN_2507
912			\|a GBV_ILN_2522
912			\|a GBV_ILN_4035
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912			\|a GBV_ILN_4126
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912			\|a GBV_ILN_4251
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912			\|a GBV_ILN_4307
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912			\|a GBV_ILN_4325
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publishDate	2022
allfields	10.1016/j.fuproc.2022.107520 doi (DE-627)ELV01058692X (ELSEVIER)S0378-3820(22)00360-5 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Gao, Xiong verfasserin aut Comparative study of the catalytic 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%). Polypropylene Catalytic co-pyrolysis Hydrocarbons Synergistic effects Zhou, Zhen verfasserin aut Wang, Jiawei verfasserin aut Tian, Hong verfasserin aut Qing, Mengxia verfasserin aut Jiang, Liyang verfasserin aut Cheng, Yi verfasserin aut Enthalten in Fuel processing technology New York, NY [u.a.] : Science Direct, 1977 241 Online-Ressource (DE-627)300898681 (DE-600)1483666-X (DE-576)09618860X nnns volume:241 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 241
spelling	10.1016/j.fuproc.2022.107520 doi (DE-627)ELV01058692X (ELSEVIER)S0378-3820(22)00360-5 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Gao, Xiong verfasserin aut Comparative study of the catalytic 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%). Polypropylene Catalytic co-pyrolysis Hydrocarbons Synergistic effects Zhou, Zhen verfasserin aut Wang, Jiawei verfasserin aut Tian, Hong verfasserin aut Qing, Mengxia verfasserin aut Jiang, Liyang verfasserin aut Cheng, Yi verfasserin aut Enthalten in Fuel processing technology New York, NY [u.a.] : Science Direct, 1977 241 Online-Ressource (DE-627)300898681 (DE-600)1483666-X (DE-576)09618860X nnns volume:241 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 241
allfields_unstemmed	10.1016/j.fuproc.2022.107520 doi (DE-627)ELV01058692X (ELSEVIER)S0378-3820(22)00360-5 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Gao, Xiong verfasserin aut Comparative study of the catalytic 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%). Polypropylene Catalytic co-pyrolysis Hydrocarbons Synergistic effects Zhou, Zhen verfasserin aut Wang, Jiawei verfasserin aut Tian, Hong verfasserin aut Qing, Mengxia verfasserin aut Jiang, Liyang verfasserin aut Cheng, Yi verfasserin aut Enthalten in Fuel processing technology New York, NY [u.a.] : Science Direct, 1977 241 Online-Ressource (DE-627)300898681 (DE-600)1483666-X (DE-576)09618860X nnns volume:241 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 241
allfieldsGer	10.1016/j.fuproc.2022.107520 doi (DE-627)ELV01058692X (ELSEVIER)S0378-3820(22)00360-5 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Gao, Xiong verfasserin aut Comparative study of the catalytic 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%). Polypropylene Catalytic co-pyrolysis Hydrocarbons Synergistic effects Zhou, Zhen verfasserin aut Wang, Jiawei verfasserin aut Tian, Hong verfasserin aut Qing, Mengxia verfasserin aut Jiang, Liyang verfasserin aut Cheng, Yi verfasserin aut Enthalten in Fuel processing technology New York, NY [u.a.] : Science Direct, 1977 241 Online-Ressource (DE-627)300898681 (DE-600)1483666-X (DE-576)09618860X nnns volume:241 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 241
allfieldsSound	10.1016/j.fuproc.2022.107520 doi (DE-627)ELV01058692X (ELSEVIER)S0378-3820(22)00360-5 DE-627 ger DE-627 rda eng 660 VZ 58.21 bkl Gao, Xiong verfasserin aut Comparative study of the catalytic 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%). Polypropylene Catalytic co-pyrolysis Hydrocarbons Synergistic effects Zhou, Zhen verfasserin aut Wang, Jiawei verfasserin aut Tian, Hong verfasserin aut Qing, Mengxia verfasserin aut Jiang, Liyang verfasserin aut Cheng, Yi verfasserin aut Enthalten in Fuel processing technology New York, NY [u.a.] : Science Direct, 1977 241 Online-Ressource (DE-627)300898681 (DE-600)1483666-X (DE-576)09618860X nnns volume:241 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.21 Brennstoffe Kraftstoffe Explosivstoffe VZ AR 241
language	English
source	Enthalten in Fuel processing technology 241 volume:241
sourceStr	Enthalten in Fuel processing technology 241 volume:241
format_phy_str_mv	Article
bklname	Brennstoffe Kraftstoffe Explosivstoffe
institution	findex.gbv.de
topic_facet	Polypropylene Catalytic co-pyrolysis Hydrocarbons Synergistic effects
dewey-raw	660
isfreeaccess_bool	false
container_title	Fuel processing technology
authorswithroles_txt_mv	Gao, Xiong @@aut@@ Zhou, Zhen @@aut@@ Wang, Jiawei @@aut@@ Tian, Hong @@aut@@ Qing, Mengxia @@aut@@ Jiang, Liyang @@aut@@ Cheng, Yi @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	300898681
dewey-sort	3660
id	ELV01058692X
language_de	englisch
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author	Gao, Xiong
spellingShingle	Gao, Xiong ddc 660 bkl 58.21 misc Polypropylene misc Catalytic co-pyrolysis misc Hydrocarbons misc Synergistic effects Comparative study of the catalytic
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topic_title	660 VZ 58.21 bkl Comparative study of the catalytic Polypropylene Catalytic co-pyrolysis Hydrocarbons Synergistic effects
topic	ddc 660 bkl 58.21 misc Polypropylene misc Catalytic co-pyrolysis misc Hydrocarbons misc Synergistic effects
topic_unstemmed	ddc 660 bkl 58.21 misc Polypropylene misc Catalytic co-pyrolysis misc Hydrocarbons misc Synergistic effects
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title	Comparative study of the catalytic
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title_full	Comparative study of the catalytic
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title_sort	comparative study of the catalytic
title_auth	Comparative study of the catalytic
abstract	The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%).
abstractGer	The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%).
abstract_unstemmed	The co-pyrolysis of microalgae with plastic for valuable chemical production is promising to address the inferiority of microalgae conversion while solving waste plastic problems. A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. ZSM-5 was selective for aromatic hydrocarbons conversion (from 12.23% to 14.56%), while CaO was more inclined to aliphatic hydrocarbons formation (from 70.67% to 80.95%).
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title_short	Comparative study of the catalytic
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author2	Zhou, Zhen Wang, Jiawei Tian, Hong Qing, Mengxia Jiang, Liyang Cheng, Yi
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up_date	2024-07-06T18:31:01.120Z
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A deep understanding of the synergistic effects of different catalysts on the co-pyrolysis and reaction pathways could promote process intensification through interpreting the kinetics and product characterizations. The thermogravimetric analyzer (TGA), diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS), and thermal cracking-gas chromatography/mass spectrometer (py-GC/MS) facilitated the understanding of the process. The weight-loss rates of the catalytic co-pyrolysis showed a pattern of non-catalytic < CaO < ZSM-5. The experimental and theoretical values of the co-pyrolysis activation energy were 114.99 kJ/mol and 194.80 kJ/mol, respectively. ZSM-5 reduced the co-pyrolysis activation energy, while CaO had the opposite effects. Both CaO and ZSM-5 reduced the compositions of the oxygen- and nitrogen-containing groups in the pyrolysis product, but CaO preferred oxygen removal, and ZSM-5 favored the nitrogen removal. 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Comparative study of the catalytic

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