Pt/3D-graphene/FTO electrodes: Electrochemical preparation and their enhanced electrocatalytic activity
We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Yang, Shaolin [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2014transfer abstract |
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| Schlagwörter: |
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| Umfang: |
9 |
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| Übergeordnetes Werk: |
Enthalten in: External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs - Dedhia, Kavita ELSEVIER, 2018, official journal of the International Association for Hydrogen Energy, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:39 ; year:2014 ; number:27 ; day:12 ; month:09 ; pages:15063-15071 ; extent:9 |
| Links: |
|---|
| DOI / URN: |
10.1016/j.ijhydene.2014.07.036 |
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| 520 | |a We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. | ||
| 520 | |a We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. | ||
| 650 | 7 | |a Electrocatalysis |2 Elsevier | |
| 650 | 7 | |a Platinum |2 Elsevier | |
| 650 | 7 | |a Methanol oxidation |2 Elsevier | |
| 650 | 7 | |a Electrodeposition |2 Elsevier | |
| 650 | 7 | |a 3D graphene |2 Elsevier | |
| 650 | 7 | |a Fuel cell |2 Elsevier | |
| 700 | 1 | |a Huang, Yongwei |4 oth | |
| 700 | 1 | |a Zhu, Wei |4 oth | |
| 700 | 1 | |a Deng, Bingchen |4 oth | |
| 700 | 1 | |a Wang, Hong |4 oth | |
| 700 | 1 | |a Zhang, Zihan |4 oth | |
| 700 | 1 | |a Bao, Pengfei |4 oth | |
| 700 | 1 | |a Wang, Guanzhong |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Dedhia, Kavita ELSEVIER |t External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs |d 2018 |d official journal of the International Association for Hydrogen Energy |g New York, NY [u.a.] |w (DE-627)ELV000127019 |
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10.1016/j.ijhydene.2014.07.036 doi GBVA2014011000026.pica (DE-627)ELV012326186 (ELSEVIER)S0360-3199(14)01993-4 DE-627 ger DE-627 rakwb eng 660 620 660 DE-600 620 DE-600 610 VZ 44.94 bkl Yang, Shaolin verfasserin aut Pt/3D-graphene/FTO electrodes: Electrochemical preparation and their enhanced electrocatalytic activity 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. Electrocatalysis Elsevier Platinum Elsevier Methanol oxidation Elsevier Electrodeposition Elsevier 3D graphene Elsevier Fuel cell Elsevier Huang, Yongwei oth Zhu, Wei oth Deng, Bingchen oth Wang, Hong oth Zhang, Zihan oth Bao, Pengfei oth Wang, Guanzhong oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:39 year:2014 number:27 day:12 month:09 pages:15063-15071 extent:9 https://doi.org/10.1016/j.ijhydene.2014.07.036 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 39 2014 27 12 0912 15063-15071 9 045F 660 |
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10.1016/j.ijhydene.2014.07.036 doi GBVA2014011000026.pica (DE-627)ELV012326186 (ELSEVIER)S0360-3199(14)01993-4 DE-627 ger DE-627 rakwb eng 660 620 660 DE-600 620 DE-600 610 VZ 44.94 bkl Yang, Shaolin verfasserin aut Pt/3D-graphene/FTO electrodes: Electrochemical preparation and their enhanced electrocatalytic activity 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. Electrocatalysis Elsevier Platinum Elsevier Methanol oxidation Elsevier Electrodeposition Elsevier 3D graphene Elsevier Fuel cell Elsevier Huang, Yongwei oth Zhu, Wei oth Deng, Bingchen oth Wang, Hong oth Zhang, Zihan oth Bao, Pengfei oth Wang, Guanzhong oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:39 year:2014 number:27 day:12 month:09 pages:15063-15071 extent:9 https://doi.org/10.1016/j.ijhydene.2014.07.036 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 39 2014 27 12 0912 15063-15071 9 045F 660 |
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10.1016/j.ijhydene.2014.07.036 doi GBVA2014011000026.pica (DE-627)ELV012326186 (ELSEVIER)S0360-3199(14)01993-4 DE-627 ger DE-627 rakwb eng 660 620 660 DE-600 620 DE-600 610 VZ 44.94 bkl Yang, Shaolin verfasserin aut Pt/3D-graphene/FTO electrodes: Electrochemical preparation and their enhanced electrocatalytic activity 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. Electrocatalysis Elsevier Platinum Elsevier Methanol oxidation Elsevier Electrodeposition Elsevier 3D graphene Elsevier Fuel cell Elsevier Huang, Yongwei oth Zhu, Wei oth Deng, Bingchen oth Wang, Hong oth Zhang, Zihan oth Bao, Pengfei oth Wang, Guanzhong oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:39 year:2014 number:27 day:12 month:09 pages:15063-15071 extent:9 https://doi.org/10.1016/j.ijhydene.2014.07.036 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 39 2014 27 12 0912 15063-15071 9 045F 660 |
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10.1016/j.ijhydene.2014.07.036 doi GBVA2014011000026.pica (DE-627)ELV012326186 (ELSEVIER)S0360-3199(14)01993-4 DE-627 ger DE-627 rakwb eng 660 620 660 DE-600 620 DE-600 610 VZ 44.94 bkl Yang, Shaolin verfasserin aut Pt/3D-graphene/FTO electrodes: Electrochemical preparation and their enhanced electrocatalytic activity 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. Electrocatalysis Elsevier Platinum Elsevier Methanol oxidation Elsevier Electrodeposition Elsevier 3D graphene Elsevier Fuel cell Elsevier Huang, Yongwei oth Zhu, Wei oth Deng, Bingchen oth Wang, Hong oth Zhang, Zihan oth Bao, Pengfei oth Wang, Guanzhong oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:39 year:2014 number:27 day:12 month:09 pages:15063-15071 extent:9 https://doi.org/10.1016/j.ijhydene.2014.07.036 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 39 2014 27 12 0912 15063-15071 9 045F 660 |
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10.1016/j.ijhydene.2014.07.036 doi GBVA2014011000026.pica (DE-627)ELV012326186 (ELSEVIER)S0360-3199(14)01993-4 DE-627 ger DE-627 rakwb eng 660 620 660 DE-600 620 DE-600 610 VZ 44.94 bkl Yang, Shaolin verfasserin aut Pt/3D-graphene/FTO electrodes: Electrochemical preparation and their enhanced electrocatalytic activity 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. Electrocatalysis Elsevier Platinum Elsevier Methanol oxidation Elsevier Electrodeposition Elsevier 3D graphene Elsevier Fuel cell Elsevier Huang, Yongwei oth Zhu, Wei oth Deng, Bingchen oth Wang, Hong oth Zhang, Zihan oth Bao, Pengfei oth Wang, Guanzhong oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:39 year:2014 number:27 day:12 month:09 pages:15063-15071 extent:9 https://doi.org/10.1016/j.ijhydene.2014.07.036 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 39 2014 27 12 0912 15063-15071 9 045F 660 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:39 year:2014 number:27 day:12 month:09 pages:15063-15071 extent:9 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:39 year:2014 number:27 day:12 month:09 pages:15063-15071 extent:9 |
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External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs |
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Yang, Shaolin @@aut@@ Huang, Yongwei @@oth@@ Zhu, Wei @@oth@@ Deng, Bingchen @@oth@@ Wang, Hong @@oth@@ Zhang, Zihan @@oth@@ Bao, Pengfei @@oth@@ Wang, Guanzhong @@oth@@ |
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Pt/3D-graphene/FTO electrodes: Electrochemical preparation and their enhanced electrocatalytic activity |
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We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. |
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We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. |
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We report a facile, low-cost and green route to fabricate platinum nanoparticle (Pt NP) decorated three-dimensional (3D) graphene assembled on fluorine-doped tin oxide (FTO) electrodes (Pt/3D-G/FTO) with enhanced electrocatalytic activity. The fabrication process was accomplished by preparation of 3D graphene (3D-G/FTO) electrodes through electrochemical reduction of a graphene oxide suspension followed by electrodeposition of Pt NPs onto them. The Pt/3D-G/FTO electrode exhibits much higher catalytic activity and better stability for methanol oxidation compared with the electrodes prepared by electrodeposition of Pt NPs onto two-dimensional graphene sheets substrate (Pt/G/FTO) or bare FTO (Pt/FTO) under the same condition. These enhancements can be attributed to the high surface area, large void volume and high electrical conductivity as well as smaller size of Pt NPs in the hollows of the 3D architecture and a large amount of ridges on it. |
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