Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying
Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to expl...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Marr, M. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2014transfer abstract |
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| Schlagwörter: |
Yttria-stabilized zirconia (YSZ) |
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| Umfang: |
8 |
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| Übergeordnetes Werk: |
Enthalten in: Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method - Xiao, Hong ELSEVIER, 2013, the international journal on the science and technology of electrochemical energy systems, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:245 ; year:2014 ; day:1 ; month:01 ; pages:398-405 ; extent:8 |
| Links: |
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| DOI / URN: |
10.1016/j.jpowsour.2013.06.092 |
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ELV01235094X |
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| 245 | 1 | 0 | |a Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying |
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| 520 | |a Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. | ||
| 520 | |a Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. | ||
| 650 | 7 | |a Suspension plasma spray (SPS) |2 Elsevier | |
| 650 | 7 | |a Electrolyte |2 Elsevier | |
| 650 | 7 | |a Yttria-stabilized zirconia (YSZ) |2 Elsevier | |
| 650 | 7 | |a Solution precursor plasma spray (SPPS) |2 Elsevier | |
| 650 | 7 | |a Solid oxide fuel cell (SOFC) |2 Elsevier | |
| 700 | 1 | |a Kuhn, J. |4 oth | |
| 700 | 1 | |a Metcalfe, C. |4 oth | |
| 700 | 1 | |a Harris, J. |4 oth | |
| 700 | 1 | |a Kesler, O. |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Xiao, Hong ELSEVIER |t Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |d 2013 |d the international journal on the science and technology of electrochemical energy systems |g New York, NY [u.a.] |w (DE-627)ELV00098745X |
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10.1016/j.jpowsour.2013.06.092 doi GBVA2014012000006.pica (DE-627)ELV01235094X (ELSEVIER)S0378-7753(13)01099-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Marr, M. verfasserin aut Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying 2014transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Suspension plasma spray (SPS) Elsevier Electrolyte Elsevier Yttria-stabilized zirconia (YSZ) Elsevier Solution precursor plasma spray (SPPS) Elsevier Solid oxide fuel cell (SOFC) Elsevier Kuhn, J. oth Metcalfe, C. oth Harris, J. oth Kesler, O. oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:245 year:2014 day:1 month:01 pages:398-405 extent:8 https://doi.org/10.1016/j.jpowsour.2013.06.092 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 245 2014 1 0101 398-405 8 045F 620 |
| spelling |
10.1016/j.jpowsour.2013.06.092 doi GBVA2014012000006.pica (DE-627)ELV01235094X (ELSEVIER)S0378-7753(13)01099-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Marr, M. verfasserin aut Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying 2014transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Suspension plasma spray (SPS) Elsevier Electrolyte Elsevier Yttria-stabilized zirconia (YSZ) Elsevier Solution precursor plasma spray (SPPS) Elsevier Solid oxide fuel cell (SOFC) Elsevier Kuhn, J. oth Metcalfe, C. oth Harris, J. oth Kesler, O. oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:245 year:2014 day:1 month:01 pages:398-405 extent:8 https://doi.org/10.1016/j.jpowsour.2013.06.092 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 245 2014 1 0101 398-405 8 045F 620 |
| allfields_unstemmed |
10.1016/j.jpowsour.2013.06.092 doi GBVA2014012000006.pica (DE-627)ELV01235094X (ELSEVIER)S0378-7753(13)01099-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Marr, M. verfasserin aut Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying 2014transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Suspension plasma spray (SPS) Elsevier Electrolyte Elsevier Yttria-stabilized zirconia (YSZ) Elsevier Solution precursor plasma spray (SPPS) Elsevier Solid oxide fuel cell (SOFC) Elsevier Kuhn, J. oth Metcalfe, C. oth Harris, J. oth Kesler, O. oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:245 year:2014 day:1 month:01 pages:398-405 extent:8 https://doi.org/10.1016/j.jpowsour.2013.06.092 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 245 2014 1 0101 398-405 8 045F 620 |
| allfieldsGer |
10.1016/j.jpowsour.2013.06.092 doi GBVA2014012000006.pica (DE-627)ELV01235094X (ELSEVIER)S0378-7753(13)01099-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Marr, M. verfasserin aut Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying 2014transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Suspension plasma spray (SPS) Elsevier Electrolyte Elsevier Yttria-stabilized zirconia (YSZ) Elsevier Solution precursor plasma spray (SPPS) Elsevier Solid oxide fuel cell (SOFC) Elsevier Kuhn, J. oth Metcalfe, C. oth Harris, J. oth Kesler, O. oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:245 year:2014 day:1 month:01 pages:398-405 extent:8 https://doi.org/10.1016/j.jpowsour.2013.06.092 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 245 2014 1 0101 398-405 8 045F 620 |
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10.1016/j.jpowsour.2013.06.092 doi GBVA2014012000006.pica (DE-627)ELV01235094X (ELSEVIER)S0378-7753(13)01099-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Marr, M. verfasserin aut Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying 2014transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. Suspension plasma spray (SPS) Elsevier Electrolyte Elsevier Yttria-stabilized zirconia (YSZ) Elsevier Solution precursor plasma spray (SPPS) Elsevier Solid oxide fuel cell (SOFC) Elsevier Kuhn, J. oth Metcalfe, C. oth Harris, J. oth Kesler, O. oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:245 year:2014 day:1 month:01 pages:398-405 extent:8 https://doi.org/10.1016/j.jpowsour.2013.06.092 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 245 2014 1 0101 398-405 8 045F 620 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:245 year:2014 day:1 month:01 pages:398-405 extent:8 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:245 year:2014 day:1 month:01 pages:398-405 extent:8 |
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Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |
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The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. 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Marr, M. ddc 620 ddc 690 bkl 50.92 Elsevier Suspension plasma spray (SPS) Elsevier Electrolyte Elsevier Yttria-stabilized zirconia (YSZ) Elsevier Solution precursor plasma spray (SPPS) Elsevier Solid oxide fuel cell (SOFC) Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying |
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ddc 620 ddc 690 bkl 50.92 Elsevier Suspension plasma spray (SPS) Elsevier Electrolyte Elsevier Yttria-stabilized zirconia (YSZ) Elsevier Solution precursor plasma spray (SPPS) Elsevier Solid oxide fuel cell (SOFC) |
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ddc 620 ddc 690 bkl 50.92 Elsevier Suspension plasma spray (SPS) Elsevier Electrolyte Elsevier Yttria-stabilized zirconia (YSZ) Elsevier Solution precursor plasma spray (SPPS) Elsevier Solid oxide fuel cell (SOFC) |
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Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |
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Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |
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electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying |
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Electrochemical performance of solid oxide fuel cells having electrolytes made by suspension and solution precursor plasma spraying |
| abstract |
Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. |
| abstractGer |
Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. |
| abstract_unstemmed |
Yttria-stabilized zirconia (YSZ) electrolytes were deposited by suspension plasma spraying (SPS) and solution precursor plasma spraying (SPPS). The electrolytes were evaluated for permeability, microstructure, and electrochemical performance. With SPS, three different suspensions were tested to explore the influence of powder size distribution and liquid properties. Electrolytes made from suspensions of a powder with d 50 = 2.6 μm were more gas-tight than those made from suspensions of a powder with d 50 = 0.6 μm. A peak open circuit voltage of 1.00 V was measured at 750 °C with a cell with an electrolyte made from a suspension of d 50 = 2.6 μm powder. The use of a flammable suspension liquid was beneficial for improving electrolyte conductivity when using lower energy plasmas, but the choice of liquid was less important when using higher energy plasmas. With SPPS, peak electrolyte conductivities were comparable to the peak conductivities of the SPS electrolytes. However, leak rates through the SPPS electrolytes were higher than those through the electrolytes made from suspensions of d 50 = 2.6 μm powder. The electrochemical test data on SPPS electrolytes are the first reported in the literature. |
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