Optical properties of Fe-doped BaTiO3 films deposited on quartz substrates by sol-gel method
Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion e...
Ausführliche Beschreibung
Autor*in: |
Tian, Jianjun [verfasserIn] |
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Englisch |
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2016transfer abstract |
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Enthalten in: Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners - Jacobs, Jacquelyn A. ELSEVIER, 2017, JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics, Lausanne |
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volume:687 ; year:2016 ; day:5 ; month:12 ; pages:529-533 ; extent:5 |
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DOI / URN: |
10.1016/j.jallcom.2016.06.154 |
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520 | |a Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. | ||
520 | |a Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. | ||
650 | 7 | |a Sol-gel |2 Elsevier | |
650 | 7 | |a Doping |2 Elsevier | |
650 | 7 | |a Optical property |2 Elsevier | |
650 | 7 | |a BaTiO3 |2 Elsevier | |
650 | 7 | |a Thin film |2 Elsevier | |
700 | 1 | |a Gao, Huiping |4 oth | |
700 | 1 | |a Deng, Weibing |4 oth | |
700 | 1 | |a Zheng, Haiwu |4 oth | |
700 | 1 | |a Tan, Furui |4 oth | |
700 | 1 | |a Zhang, Weifeng |4 oth | |
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10.1016/j.jallcom.2016.06.154 doi GBV00000000000226A.pica (DE-627)ELV014291827 (ELSEVIER)S0925-8388(16)31877-1 DE-627 ger DE-627 rakwb eng 670 540 670 DE-600 540 DE-600 630 VZ Tian, Jianjun verfasserin aut Optical properties of Fe-doped BaTiO3 films deposited on quartz substrates by sol-gel method 2016transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Sol-gel Elsevier Doping Elsevier Optical property Elsevier BaTiO3 Elsevier Thin film Elsevier Gao, Huiping oth Deng, Weibing oth Zheng, Haiwu oth Tan, Furui oth Zhang, Weifeng oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:687 year:2016 day:5 month:12 pages:529-533 extent:5 https://doi.org/10.1016/j.jallcom.2016.06.154 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 687 2016 5 1205 529-533 5 045F 670 |
spelling |
10.1016/j.jallcom.2016.06.154 doi GBV00000000000226A.pica (DE-627)ELV014291827 (ELSEVIER)S0925-8388(16)31877-1 DE-627 ger DE-627 rakwb eng 670 540 670 DE-600 540 DE-600 630 VZ Tian, Jianjun verfasserin aut Optical properties of Fe-doped BaTiO3 films deposited on quartz substrates by sol-gel method 2016transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Sol-gel Elsevier Doping Elsevier Optical property Elsevier BaTiO3 Elsevier Thin film Elsevier Gao, Huiping oth Deng, Weibing oth Zheng, Haiwu oth Tan, Furui oth Zhang, Weifeng oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:687 year:2016 day:5 month:12 pages:529-533 extent:5 https://doi.org/10.1016/j.jallcom.2016.06.154 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 687 2016 5 1205 529-533 5 045F 670 |
allfields_unstemmed |
10.1016/j.jallcom.2016.06.154 doi GBV00000000000226A.pica (DE-627)ELV014291827 (ELSEVIER)S0925-8388(16)31877-1 DE-627 ger DE-627 rakwb eng 670 540 670 DE-600 540 DE-600 630 VZ Tian, Jianjun verfasserin aut Optical properties of Fe-doped BaTiO3 films deposited on quartz substrates by sol-gel method 2016transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Sol-gel Elsevier Doping Elsevier Optical property Elsevier BaTiO3 Elsevier Thin film Elsevier Gao, Huiping oth Deng, Weibing oth Zheng, Haiwu oth Tan, Furui oth Zhang, Weifeng oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:687 year:2016 day:5 month:12 pages:529-533 extent:5 https://doi.org/10.1016/j.jallcom.2016.06.154 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 687 2016 5 1205 529-533 5 045F 670 |
allfieldsGer |
10.1016/j.jallcom.2016.06.154 doi GBV00000000000226A.pica (DE-627)ELV014291827 (ELSEVIER)S0925-8388(16)31877-1 DE-627 ger DE-627 rakwb eng 670 540 670 DE-600 540 DE-600 630 VZ Tian, Jianjun verfasserin aut Optical properties of Fe-doped BaTiO3 films deposited on quartz substrates by sol-gel method 2016transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Sol-gel Elsevier Doping Elsevier Optical property Elsevier BaTiO3 Elsevier Thin film Elsevier Gao, Huiping oth Deng, Weibing oth Zheng, Haiwu oth Tan, Furui oth Zhang, Weifeng oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:687 year:2016 day:5 month:12 pages:529-533 extent:5 https://doi.org/10.1016/j.jallcom.2016.06.154 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 687 2016 5 1205 529-533 5 045F 670 |
allfieldsSound |
10.1016/j.jallcom.2016.06.154 doi GBV00000000000226A.pica (DE-627)ELV014291827 (ELSEVIER)S0925-8388(16)31877-1 DE-627 ger DE-627 rakwb eng 670 540 670 DE-600 540 DE-600 630 VZ Tian, Jianjun verfasserin aut Optical properties of Fe-doped BaTiO3 films deposited on quartz substrates by sol-gel method 2016transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. Sol-gel Elsevier Doping Elsevier Optical property Elsevier BaTiO3 Elsevier Thin film Elsevier Gao, Huiping oth Deng, Weibing oth Zheng, Haiwu oth Tan, Furui oth Zhang, Weifeng oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:687 year:2016 day:5 month:12 pages:529-533 extent:5 https://doi.org/10.1016/j.jallcom.2016.06.154 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 687 2016 5 1205 529-533 5 045F 670 |
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Enthalten in Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners Lausanne volume:687 year:2016 day:5 month:12 pages:529-533 extent:5 |
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optical properties of fe-doped batio3 films deposited on quartz substrates by sol-gel method |
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Optical properties of Fe-doped BaTiO3 films deposited on quartz substrates by sol-gel method |
abstract |
Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. |
abstractGer |
Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. |
abstract_unstemmed |
Fe-doped BaTiO3 films were prepared on quartz substrates by sol-gel route. Linearly optical constants of the films were obtained by fitting transmittance spectra with Adachi’s model. With increasing Fe composition, refractive index n at 532 nm increases, single oscillator energy E c and dispersion energy E d increase, but optical band gap E g decreases from 3.78 to 3.63 eV. In addition, nonlinear optical properties of the Fe-doped BaTiO3 films were analyzed by Z-scan method. Nonlinear optical responses of the BaTiO3 films were enhanced by Fe doping. For BaTi0.96Fe0.04O3 film, the third-order nonlinear refractive index coefficient γ, the nonlinear refractive index coefficient n 2 , the nonlinear absorption coefficient β and the third-order nonlinear susceptibility χ(3) are 1.98 × 10−13 m2/W, 1.03 × 10−6 esu, 1.33 × 10−7 m/W, 2.38 × 10−7 esu respectively. The nonlinearity is predominated by the nonlinear refractive behavior. These results suggest that Fe doping may tune the linear and nonlinear optical properties of BaTiO3 films, which indicates that Fe-doped BaTiO3 films are promising materials for applications in optical devices. |
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Optical properties of Fe-doped BaTiO3 films deposited on quartz substrates by sol-gel method |
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