Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment
Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness...
Ausführliche Beschreibung
Autor*in: |
Endo, Satoshi [verfasserIn] |
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Englisch |
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2017transfer abstract |
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8 |
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Übergeordnetes Werk: |
Enthalten in: MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata - Shterenlikht, Anton ELSEVIER, 2019, chemistry, biology and toxicology as related to environmental problems, Amsterdam [u.a.] |
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Übergeordnetes Werk: |
volume:184 ; year:2017 ; pages:358-365 ; extent:8 |
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DOI / URN: |
10.1016/j.chemosphere.2017.06.005 |
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ELV01475584X |
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520 | |a Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. | ||
520 | |a Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. | ||
650 | 7 | |a Sorption kinetics |2 Elsevier | |
650 | 7 | |a Passive sampling |2 Elsevier | |
650 | 7 | |a Sediment porewater |2 Elsevier | |
650 | 7 | |a Freely dissolved concentration |2 Elsevier | |
650 | 7 | |a Equilibrium partitioning |2 Elsevier | |
700 | 1 | |a Yabuki, Yoshinori |4 oth | |
700 | 1 | |a Tanaka, Shuhei |4 oth | |
773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a Shterenlikht, Anton ELSEVIER |t MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata |d 2019 |d chemistry, biology and toxicology as related to environmental problems |g Amsterdam [u.a.] |w (DE-627)ELV002112701 |
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10.1016/j.chemosphere.2017.06.005 doi GBV00000000000254A.pica (DE-627)ELV01475584X (ELSEVIER)S0045-6535(17)30907-4 DE-627 ger DE-627 rakwb eng 333.7 333.7 DE-600 004 620 VZ 54.25 bkl Endo, Satoshi verfasserin aut Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Sorption kinetics Elsevier Passive sampling Elsevier Sediment porewater Elsevier Freely dissolved concentration Elsevier Equilibrium partitioning Elsevier Yabuki, Yoshinori oth Tanaka, Shuhei oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:184 year:2017 pages:358-365 extent:8 https://doi.org/10.1016/j.chemosphere.2017.06.005 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 184 2017 358-365 8 045F 333.7 |
spelling |
10.1016/j.chemosphere.2017.06.005 doi GBV00000000000254A.pica (DE-627)ELV01475584X (ELSEVIER)S0045-6535(17)30907-4 DE-627 ger DE-627 rakwb eng 333.7 333.7 DE-600 004 620 VZ 54.25 bkl Endo, Satoshi verfasserin aut Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Sorption kinetics Elsevier Passive sampling Elsevier Sediment porewater Elsevier Freely dissolved concentration Elsevier Equilibrium partitioning Elsevier Yabuki, Yoshinori oth Tanaka, Shuhei oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:184 year:2017 pages:358-365 extent:8 https://doi.org/10.1016/j.chemosphere.2017.06.005 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 184 2017 358-365 8 045F 333.7 |
allfields_unstemmed |
10.1016/j.chemosphere.2017.06.005 doi GBV00000000000254A.pica (DE-627)ELV01475584X (ELSEVIER)S0045-6535(17)30907-4 DE-627 ger DE-627 rakwb eng 333.7 333.7 DE-600 004 620 VZ 54.25 bkl Endo, Satoshi verfasserin aut Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Sorption kinetics Elsevier Passive sampling Elsevier Sediment porewater Elsevier Freely dissolved concentration Elsevier Equilibrium partitioning Elsevier Yabuki, Yoshinori oth Tanaka, Shuhei oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:184 year:2017 pages:358-365 extent:8 https://doi.org/10.1016/j.chemosphere.2017.06.005 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 184 2017 358-365 8 045F 333.7 |
allfieldsGer |
10.1016/j.chemosphere.2017.06.005 doi GBV00000000000254A.pica (DE-627)ELV01475584X (ELSEVIER)S0045-6535(17)30907-4 DE-627 ger DE-627 rakwb eng 333.7 333.7 DE-600 004 620 VZ 54.25 bkl Endo, Satoshi verfasserin aut Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Sorption kinetics Elsevier Passive sampling Elsevier Sediment porewater Elsevier Freely dissolved concentration Elsevier Equilibrium partitioning Elsevier Yabuki, Yoshinori oth Tanaka, Shuhei oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:184 year:2017 pages:358-365 extent:8 https://doi.org/10.1016/j.chemosphere.2017.06.005 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 184 2017 358-365 8 045F 333.7 |
allfieldsSound |
10.1016/j.chemosphere.2017.06.005 doi GBV00000000000254A.pica (DE-627)ELV01475584X (ELSEVIER)S0045-6535(17)30907-4 DE-627 ger DE-627 rakwb eng 333.7 333.7 DE-600 004 620 VZ 54.25 bkl Endo, Satoshi verfasserin aut Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. Sorption kinetics Elsevier Passive sampling Elsevier Sediment porewater Elsevier Freely dissolved concentration Elsevier Equilibrium partitioning Elsevier Yabuki, Yoshinori oth Tanaka, Shuhei oth Enthalten in Elsevier Science Shterenlikht, Anton ELSEVIER MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata 2019 chemistry, biology and toxicology as related to environmental problems Amsterdam [u.a.] (DE-627)ELV002112701 volume:184 year:2017 pages:358-365 extent:8 https://doi.org/10.1016/j.chemosphere.2017.06.005 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.25 Parallele Datenverarbeitung VZ AR 184 2017 358-365 8 045F 333.7 |
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Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment |
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Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment |
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MPI vs Fortran coarrays beyond 100k cores: 3D cellular automata |
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comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: mutual validation and possible correction by polymer-polymer partition experiment |
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Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment |
abstract |
Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. |
abstractGer |
Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. |
abstract_unstemmed |
Two sediment passive samplers, polyethylene (PE) and polyoxymethylene (POM), were compared and mutually validated for measuring freely dissolved concentrations (C free) of polychlorinated biphenyls (PCBs) in sediment porewater. PE and POM strips in commonly used dimensions (30 and 76 μm in thickness, respectively) were exposed to sediment slurries for 28 d. The C free values calculated using literature polymer-water partition coefficients were consistently higher for PE than for POM by a factor of 2 on average. Time series experiments over 96 d show that 28 d are sufficient for attaining partition equilibrium of PCBs for PE, whereas even 96 d may not be enough for POM. To gain additional insight, POM and PE strips were co-exposed to bovine serum albumin suspension spiked with PCBs. The POM/PE concentration ratios increased over 56 d, and the ratios at 28 d were in agreement with the POM-to-PE ratios of PCB concentrations from the 28-d sediment slurry experiments. This agreement suggests that the use of apparent POM-water partition coefficients (i.e., non-equilibrium concentration ratios) suitable for a 28-d exposure to sediment slurries may correct the non-attainment of equilibrium and could provide more accurate C free values. |
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Comparing polyethylene and polyoxymethylene passive samplers for measuring sediment porewater concentrations of polychlorinated biphenyls: Mutual validation and possible correction by polymer-polymer partition experiment |
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