Nafion/graphene oxide composite membranes for low humidifying polymer electrolyte membrane fuel cell
Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increa...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Lee, D.C. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2014transfer abstract |
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| Schlagwörter: |
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| Umfang: |
9 |
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| Übergeordnetes Werk: |
Enthalten in: Steering charge kinetics in W - Yue, Xin-Zheng ELSEVIER, 2019, the official journal of the North American Membrane Society, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:452 ; year:2014 ; day:15 ; month:02 ; pages:20-28 ; extent:9 |
| Links: |
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| DOI / URN: |
10.1016/j.memsci.2013.10.018 |
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ELV017537452 |
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| 245 | 1 | 0 | |a Nafion/graphene oxide composite membranes for low humidifying polymer electrolyte membrane fuel cell |
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| 520 | |a Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. | ||
| 520 | |a Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. | ||
| 650 | 7 | |a OCV |2 Elsevier | |
| 650 | 7 | |a Proton conductivity |2 Elsevier | |
| 650 | 7 | |a Water uptake |2 Elsevier | |
| 650 | 7 | |a Graphene oxide |2 Elsevier | |
| 650 | 7 | |a Cell performance |2 Elsevier | |
| 700 | 1 | |a Yang, H.N. |4 oth | |
| 700 | 1 | |a Park, S.H. |4 oth | |
| 700 | 1 | |a Kim, W.J. |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Yue, Xin-Zheng ELSEVIER |t Steering charge kinetics in W |d 2019 |d the official journal of the North American Membrane Society |g New York, NY [u.a.] |w (DE-627)ELV002478420 |
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10.1016/j.memsci.2013.10.018 doi GBVA2014012000015.pica (DE-627)ELV017537452 (ELSEVIER)S0376-7388(13)00819-3 DE-627 ger DE-627 rakwb eng 570 570 DE-600 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Lee, D.C. verfasserin aut Nafion/graphene oxide composite membranes for low humidifying polymer electrolyte membrane fuel cell 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. OCV Elsevier Proton conductivity Elsevier Water uptake Elsevier Graphene oxide Elsevier Cell performance Elsevier Yang, H.N. oth Park, S.H. oth Kim, W.J. oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:452 year:2014 day:15 month:02 pages:20-28 extent:9 https://doi.org/10.1016/j.memsci.2013.10.018 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 452 2014 15 0215 20-28 9 045F 570 |
| spelling |
10.1016/j.memsci.2013.10.018 doi GBVA2014012000015.pica (DE-627)ELV017537452 (ELSEVIER)S0376-7388(13)00819-3 DE-627 ger DE-627 rakwb eng 570 570 DE-600 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Lee, D.C. verfasserin aut Nafion/graphene oxide composite membranes for low humidifying polymer electrolyte membrane fuel cell 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. OCV Elsevier Proton conductivity Elsevier Water uptake Elsevier Graphene oxide Elsevier Cell performance Elsevier Yang, H.N. oth Park, S.H. oth Kim, W.J. oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:452 year:2014 day:15 month:02 pages:20-28 extent:9 https://doi.org/10.1016/j.memsci.2013.10.018 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 452 2014 15 0215 20-28 9 045F 570 |
| allfields_unstemmed |
10.1016/j.memsci.2013.10.018 doi GBVA2014012000015.pica (DE-627)ELV017537452 (ELSEVIER)S0376-7388(13)00819-3 DE-627 ger DE-627 rakwb eng 570 570 DE-600 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Lee, D.C. verfasserin aut Nafion/graphene oxide composite membranes for low humidifying polymer electrolyte membrane fuel cell 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. OCV Elsevier Proton conductivity Elsevier Water uptake Elsevier Graphene oxide Elsevier Cell performance Elsevier Yang, H.N. oth Park, S.H. oth Kim, W.J. oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:452 year:2014 day:15 month:02 pages:20-28 extent:9 https://doi.org/10.1016/j.memsci.2013.10.018 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 452 2014 15 0215 20-28 9 045F 570 |
| allfieldsGer |
10.1016/j.memsci.2013.10.018 doi GBVA2014012000015.pica (DE-627)ELV017537452 (ELSEVIER)S0376-7388(13)00819-3 DE-627 ger DE-627 rakwb eng 570 570 DE-600 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Lee, D.C. verfasserin aut Nafion/graphene oxide composite membranes for low humidifying polymer electrolyte membrane fuel cell 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. OCV Elsevier Proton conductivity Elsevier Water uptake Elsevier Graphene oxide Elsevier Cell performance Elsevier Yang, H.N. oth Park, S.H. oth Kim, W.J. oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:452 year:2014 day:15 month:02 pages:20-28 extent:9 https://doi.org/10.1016/j.memsci.2013.10.018 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 452 2014 15 0215 20-28 9 045F 570 |
| allfieldsSound |
10.1016/j.memsci.2013.10.018 doi GBVA2014012000015.pica (DE-627)ELV017537452 (ELSEVIER)S0376-7388(13)00819-3 DE-627 ger DE-627 rakwb eng 570 570 DE-600 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Lee, D.C. verfasserin aut Nafion/graphene oxide composite membranes for low humidifying polymer electrolyte membrane fuel cell 2014transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. OCV Elsevier Proton conductivity Elsevier Water uptake Elsevier Graphene oxide Elsevier Cell performance Elsevier Yang, H.N. oth Park, S.H. oth Kim, W.J. oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:452 year:2014 day:15 month:02 pages:20-28 extent:9 https://doi.org/10.1016/j.memsci.2013.10.018 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 452 2014 15 0215 20-28 9 045F 570 |
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Nafion/graphene oxide composite membranes for low humidifying polymer electrolyte membrane fuel cell |
| abstract |
Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. |
| abstractGer |
Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. |
| abstract_unstemmed |
Graphene oxide was prepared from graphite using Hummer's method. Pt nanoparticles with 1.8nm in average size are successfully obtained via in-situ Pt nanoparticles deposition onto graphene oxide (GO) using a microwave method, finally resulting in Pt-graphene (Pt-G). Water uptake of GO is increased with GO content in a Nafion/GO composite membrane due to the hydrophilic GO while that of Nafion/Pt-G composite membrane is much lower than that of Nafion/GO composite membrane. The MEAs fabricated with the Nafion/GO composite membrane show significant enhancement in cell performance: that is, 0.802A, 1.27A, 0.827A at 0.6V under 100% relative humidity (RH) for 0.5wt%, 3.0wt% and 4.5wt% of GO content in the composite membrane, respectively, compared to 0.435A for casting Nafion membrane. The Nafion/Pt-G composite membrane, however, does not show sufficient enhancement under various RHs. It is attributed to poor water retention ability of hydrophobic graphene and electron loss due to the formation of electrical network by too much Pt within the membrane. Constant open circuit voltage (OCV) down to low RH indicates that GO and graphene could be prospective as filler in low humidifying polymer electrolyte fuel cell. |
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