Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons
Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal po...
Ausführliche Beschreibung
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| Autor*in: |
Sánchez-Sánchez, Angela [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2014transfer abstract |
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| Umfang: |
11 |
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| Übergeordnetes Werk: |
Enthalten in: Dynamic patterns of open review process - Zhao, Zhi-Dan ELSEVIER, 2021, an international journal sponsored by the American Carbon Society, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:70 ; year:2014 ; pages:119-129 ; extent:11 |
| Links: |
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| DOI / URN: |
10.1016/j.carbon.2013.12.080 |
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ELV017964342 |
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| 245 | 1 | 0 | |a Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons |
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| 520 | |a Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. | ||
| 520 | |a Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. | ||
| 700 | 1 | |a Suárez-García, Fabián |4 oth | |
| 700 | 1 | |a Martínez-Alonso, Amelia |4 oth | |
| 700 | 1 | |a Tascón, Juan M.D. |4 oth | |
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10.1016/j.carbon.2013.12.080 doi GBVA2014020000004.pica (DE-627)ELV017964342 (ELSEVIER)S0008-6223(13)01235-9 DE-627 ger DE-627 rakwb eng 540 540 DE-600 500 VZ 33.25 bkl 31.00 bkl Sánchez-Sánchez, Angela verfasserin aut Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons 2014transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Suárez-García, Fabián oth Martínez-Alonso, Amelia oth Tascón, Juan M.D. oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:70 year:2014 pages:119-129 extent:11 https://doi.org/10.1016/j.carbon.2013.12.080 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 70 2014 119-129 11 045F 540 |
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10.1016/j.carbon.2013.12.080 doi GBVA2014020000004.pica (DE-627)ELV017964342 (ELSEVIER)S0008-6223(13)01235-9 DE-627 ger DE-627 rakwb eng 540 540 DE-600 500 VZ 33.25 bkl 31.00 bkl Sánchez-Sánchez, Angela verfasserin aut Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons 2014transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Suárez-García, Fabián oth Martínez-Alonso, Amelia oth Tascón, Juan M.D. oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:70 year:2014 pages:119-129 extent:11 https://doi.org/10.1016/j.carbon.2013.12.080 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 70 2014 119-129 11 045F 540 |
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10.1016/j.carbon.2013.12.080 doi GBVA2014020000004.pica (DE-627)ELV017964342 (ELSEVIER)S0008-6223(13)01235-9 DE-627 ger DE-627 rakwb eng 540 540 DE-600 500 VZ 33.25 bkl 31.00 bkl Sánchez-Sánchez, Angela verfasserin aut Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons 2014transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Suárez-García, Fabián oth Martínez-Alonso, Amelia oth Tascón, Juan M.D. oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:70 year:2014 pages:119-129 extent:11 https://doi.org/10.1016/j.carbon.2013.12.080 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 70 2014 119-129 11 045F 540 |
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10.1016/j.carbon.2013.12.080 doi GBVA2014020000004.pica (DE-627)ELV017964342 (ELSEVIER)S0008-6223(13)01235-9 DE-627 ger DE-627 rakwb eng 540 540 DE-600 500 VZ 33.25 bkl 31.00 bkl Sánchez-Sánchez, Angela verfasserin aut Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons 2014transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Suárez-García, Fabián oth Martínez-Alonso, Amelia oth Tascón, Juan M.D. oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:70 year:2014 pages:119-129 extent:11 https://doi.org/10.1016/j.carbon.2013.12.080 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 70 2014 119-129 11 045F 540 |
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10.1016/j.carbon.2013.12.080 doi GBVA2014020000004.pica (DE-627)ELV017964342 (ELSEVIER)S0008-6223(13)01235-9 DE-627 ger DE-627 rakwb eng 540 540 DE-600 500 VZ 33.25 bkl 31.00 bkl Sánchez-Sánchez, Angela verfasserin aut Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons 2014transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. Suárez-García, Fabián oth Martínez-Alonso, Amelia oth Tascón, Juan M.D. oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:70 year:2014 pages:119-129 extent:11 https://doi.org/10.1016/j.carbon.2013.12.080 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 70 2014 119-129 11 045F 540 |
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aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons |
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Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons |
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Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. |
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Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. |
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Polyamides are used for the first time as precursors in the synthesis of nitrogen- and oxygen-doped ordered mesoporous carbons (OMCs) by applying two synthetic methods, named here as: (i) organic phase synthesis (infiltration in situ by Yamazaki reaction-based method) and (ii) solid-state thermal polymerization (liquid infiltration and thermal polymerization of the monomer into the porosity of the template). In both cases, 3-aminobenzoic acid (MABA) and SBA-15 mesoporous silica are used as precursor and template, respectively, and the infiltration takes place in one single step. In the first method, the infiltration process is accomplished in situ through Yamazaki reaction of the MABA; in the second one, the MABA monomer is introduced into the channels of the silica template by incipient wetness dissolved in a common and low polluting organic solvent. After carbonization at 900°C and removal of the template, OMCs with very narrow pore size distributions and nitrogen and oxygen contents as large as ∼6 and 6.4–11.5wt.%, respectively, are obtained. This work opens a new way to prepare advanced carbon materials, due to the wide variety of polyamides that can be synthesized by applying the two proposed methods to a large number of both aliphatic and aromatic precursors. |
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Aromatic polyamides as new precursors of nitrogen and oxygen-doped ordered mesoporous carbons |
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