Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry
Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed...
Ausführliche Beschreibung
Autor*in: |
Steven, Jared T. [verfasserIn] Golovko, Vladimir B. [verfasserIn] Johannessen, Bernt [verfasserIn] Marshall, Aaron T. [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2015 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Electrochimica acta - New York, NY [u.a.] : Elsevier, 1959, 187, Seite 593-604 |
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Übergeordnetes Werk: |
volume:187 ; pages:593-604 |
DOI / URN: |
10.1016/j.electacta.2015.11.096 |
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ELV019793375 |
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520 | |a Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. | ||
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10.1016/j.electacta.2015.11.096 doi (DE-627)ELV019793375 (ELSEVIER)S0013-4686(15)30869-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Steven, Jared T. verfasserin aut Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry 2015 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. Gold nanoparticles electrocatalysis electrochemical stability Golovko, Vladimir B. verfasserin aut Johannessen, Bernt verfasserin aut Marshall, Aaron T. verfasserin (orcid)0000-0002-3530-7251 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 187, Seite 593-604 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:187 pages:593-604 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2098 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines VZ AR 187 593-604 |
spelling |
10.1016/j.electacta.2015.11.096 doi (DE-627)ELV019793375 (ELSEVIER)S0013-4686(15)30869-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Steven, Jared T. verfasserin aut Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry 2015 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. Gold nanoparticles electrocatalysis electrochemical stability Golovko, Vladimir B. verfasserin aut Johannessen, Bernt verfasserin aut Marshall, Aaron T. verfasserin (orcid)0000-0002-3530-7251 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 187, Seite 593-604 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:187 pages:593-604 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2098 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines VZ AR 187 593-604 |
allfields_unstemmed |
10.1016/j.electacta.2015.11.096 doi (DE-627)ELV019793375 (ELSEVIER)S0013-4686(15)30869-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Steven, Jared T. verfasserin aut Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry 2015 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. Gold nanoparticles electrocatalysis electrochemical stability Golovko, Vladimir B. verfasserin aut Johannessen, Bernt verfasserin aut Marshall, Aaron T. verfasserin (orcid)0000-0002-3530-7251 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 187, Seite 593-604 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:187 pages:593-604 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2098 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines VZ AR 187 593-604 |
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10.1016/j.electacta.2015.11.096 doi (DE-627)ELV019793375 (ELSEVIER)S0013-4686(15)30869-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Steven, Jared T. verfasserin aut Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry 2015 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. Gold nanoparticles electrocatalysis electrochemical stability Golovko, Vladimir B. verfasserin aut Johannessen, Bernt verfasserin aut Marshall, Aaron T. verfasserin (orcid)0000-0002-3530-7251 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 187, Seite 593-604 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:187 pages:593-604 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2098 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines VZ AR 187 593-604 |
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10.1016/j.electacta.2015.11.096 doi (DE-627)ELV019793375 (ELSEVIER)S0013-4686(15)30869-0 DE-627 ger DE-627 rda eng 540 VZ 35.00 bkl Steven, Jared T. verfasserin aut Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry 2015 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. Gold nanoparticles electrocatalysis electrochemical stability Golovko, Vladimir B. verfasserin aut Johannessen, Bernt verfasserin aut Marshall, Aaron T. verfasserin (orcid)0000-0002-3530-7251 aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 187, Seite 593-604 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:187 pages:593-604 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2070 GBV_ILN_2086 GBV_ILN_2098 GBV_ILN_2106 GBV_ILN_2108 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2116 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines VZ AR 187 593-604 |
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Steven, Jared T. ddc 540 bkl 35.00 misc Gold nanoparticles misc electrocatalysis misc electrochemical stability Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry |
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540 VZ 35.00 bkl Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry Gold nanoparticles electrocatalysis electrochemical stability |
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Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry |
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Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry |
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electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry |
title_auth |
Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry |
abstract |
Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. |
abstractGer |
Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. |
abstract_unstemmed |
Cyclic voltammetry has been used to assess the electrochemical stability of gold nanoparticle-based electrocatalysts with differing initial particle size distributions in sulphuric acid electrolyte. The electrochemically active surface area (EASA), based on the gold oxide reduction charge, revealed that the electrocatalyst containing gold nanoparticles with an initial number-weighted average diameter of 4.5nm was stable over 100 voltammetry cycles. Conversely, the electrocatalysts based on 3.1nm and 2.9nm gold nanoparticles showed a continuous decrease in the EASA in line with TEM and EXAFS data which confirmed growth of the gold particles during cycling. Importantly, we find no evidence to suggest that the nature of the stabilising ligand used during the gold nanoparticle synthesis, has any effect of the electrochemical stability of gold nanoparticles. When the anodic limit of the cyclic voltammograms was limited to below the gold oxide formation potential, the nanoparticles were stable, confirming that the loss in EASA is primarily related to the dissolution and growth of gold nanoparticles associated with the Au-AuOx redox process. Interestingly, an electrocatalyst initially containing 0.8nm diameter gold nanoclusters had a surprisingly low EASA (these clusters appear not to exhibit normal Au-AuOx redox behaviour typical for the larger gold nanoparticles), but still showed significant particle growth during the cycling as confirmed by TEM and XPS analysis. |
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Electrochemical stability of carbon-supported gold nanoparticles in acidic electrolyte during cyclic voltammetry |
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score |
7.398386 |