Development and performance of anode material based on A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ perovskites for solid oxide fuel cells
Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Feng, Jie [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2016transfer abstract |
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| Umfang: |
8 |
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| Übergeordnetes Werk: |
Enthalten in: Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch - Zhang, Lei ELSEVIER, 2018, the journal of the International Society of Electrochemistry (ISE), New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:215 ; year:2016 ; day:10 ; month:10 ; pages:592-599 ; extent:8 |
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| DOI / URN: |
10.1016/j.electacta.2016.08.088 |
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ELV019799284 |
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| 245 | 1 | 0 | |a Development and performance of anode material based on A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ perovskites for solid oxide fuel cells |
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| 520 | |a Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. | ||
| 520 | |a Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. | ||
| 650 | 7 | |a A-site deficiency |2 Elsevier | |
| 650 | 7 | |a Perovskite |2 Elsevier | |
| 650 | 7 | |a Solid oxide fuel cells |2 Elsevier | |
| 650 | 7 | |a Anode |2 Elsevier | |
| 700 | 1 | |a Qiao, Jinshuo |4 oth | |
| 700 | 1 | |a Wang, Wenyi |4 oth | |
| 700 | 1 | |a Wang, Zhenhua |4 oth | |
| 700 | 1 | |a Sun, Wang |4 oth | |
| 700 | 1 | |a Sun, Kening |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Zhang, Lei ELSEVIER |t Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch |d 2018 |d the journal of the International Society of Electrochemistry (ISE) |g New York, NY [u.a.] |w (DE-627)ELV001212419 |
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10.1016/j.electacta.2016.08.088 doi GBVA2016021000010.pica (DE-627)ELV019799284 (ELSEVIER)S0013-4686(16)31812-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.00 bkl Feng, Jie verfasserin aut Development and performance of anode material based on A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ perovskites for solid oxide fuel cells 2016transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. A-site deficiency Elsevier Perovskite Elsevier Solid oxide fuel cells Elsevier Anode Elsevier Qiao, Jinshuo oth Wang, Wenyi oth Wang, Zhenhua oth Sun, Wang oth Sun, Kening oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:215 year:2016 day:10 month:10 pages:592-599 extent:8 https://doi.org/10.1016/j.electacta.2016.08.088 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 215 2016 10 1010 592-599 8 045F 540 |
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10.1016/j.electacta.2016.08.088 doi GBVA2016021000010.pica (DE-627)ELV019799284 (ELSEVIER)S0013-4686(16)31812-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.00 bkl Feng, Jie verfasserin aut Development and performance of anode material based on A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ perovskites for solid oxide fuel cells 2016transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. A-site deficiency Elsevier Perovskite Elsevier Solid oxide fuel cells Elsevier Anode Elsevier Qiao, Jinshuo oth Wang, Wenyi oth Wang, Zhenhua oth Sun, Wang oth Sun, Kening oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:215 year:2016 day:10 month:10 pages:592-599 extent:8 https://doi.org/10.1016/j.electacta.2016.08.088 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 215 2016 10 1010 592-599 8 045F 540 |
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10.1016/j.electacta.2016.08.088 doi GBVA2016021000010.pica (DE-627)ELV019799284 (ELSEVIER)S0013-4686(16)31812-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.00 bkl Feng, Jie verfasserin aut Development and performance of anode material based on A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ perovskites for solid oxide fuel cells 2016transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. A-site deficiency Elsevier Perovskite Elsevier Solid oxide fuel cells Elsevier Anode Elsevier Qiao, Jinshuo oth Wang, Wenyi oth Wang, Zhenhua oth Sun, Wang oth Sun, Kening oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:215 year:2016 day:10 month:10 pages:592-599 extent:8 https://doi.org/10.1016/j.electacta.2016.08.088 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 215 2016 10 1010 592-599 8 045F 540 |
| allfieldsGer |
10.1016/j.electacta.2016.08.088 doi GBVA2016021000010.pica (DE-627)ELV019799284 (ELSEVIER)S0013-4686(16)31812-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.00 bkl Feng, Jie verfasserin aut Development and performance of anode material based on A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ perovskites for solid oxide fuel cells 2016transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. A-site deficiency Elsevier Perovskite Elsevier Solid oxide fuel cells Elsevier Anode Elsevier Qiao, Jinshuo oth Wang, Wenyi oth Wang, Zhenhua oth Sun, Wang oth Sun, Kening oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:215 year:2016 day:10 month:10 pages:592-599 extent:8 https://doi.org/10.1016/j.electacta.2016.08.088 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 215 2016 10 1010 592-599 8 045F 540 |
| allfieldsSound |
10.1016/j.electacta.2016.08.088 doi GBVA2016021000010.pica (DE-627)ELV019799284 (ELSEVIER)S0013-4686(16)31812-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.00 bkl Feng, Jie verfasserin aut Development and performance of anode material based on A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ perovskites for solid oxide fuel cells 2016transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. A-site deficiency Elsevier Perovskite Elsevier Solid oxide fuel cells Elsevier Anode Elsevier Qiao, Jinshuo oth Wang, Wenyi oth Wang, Zhenhua oth Sun, Wang oth Sun, Kening oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:215 year:2016 day:10 month:10 pages:592-599 extent:8 https://doi.org/10.1016/j.electacta.2016.08.088 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 215 2016 10 1010 592-599 8 045F 540 |
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Enthalten in Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch New York, NY [u.a.] volume:215 year:2016 day:10 month:10 pages:592-599 extent:8 |
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Enthalten in Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch New York, NY [u.a.] volume:215 year:2016 day:10 month:10 pages:592-599 extent:8 |
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development and performance of anode material based on a-site deficient sr2-xfe1.4ni0.1mo0.5o6-δ perovskites for solid oxide fuel cells |
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Development and performance of anode material based on A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ perovskites for solid oxide fuel cells |
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Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. |
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Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. |
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Engineering of A-site deficiency in perovskites can be critical for designing new materials with required functional properties. In this article, A-site deficient Sr2-xFe1.4Ni0.1Mo0.5O6-δ (x=0-0.1, Sr2-xFNM) perovskites have been synthesized and characterized as anode materials for solid oxide fuel cells. X-ray photoelectron spectroscopy data indicate that Sr deficiency changes valence states of B-site cations. The introduction of A-site deficiency has shown to improve the chemical stability of the as-prepared materials under reducing conditions. With increasing of Sr deficiency, the conductivity in 5% H2/Ar increases markedly, reaching a peak value of 26.6Scm−1 at x=0.05. While further increasing of x reduces the conductivity by affecting the mobility of electronic charge carriers. The La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported cell with La0.6Sr0.4Fe0.8Co0.2O3 cathode and Sr1.95Fe1.4Ni0.1Mo0.5O6-δ anode demonstrates a maximum power density of 606mWcm−2 at 800°C operating in H2. Such designed A-site deficiency perovskite has the potential to be applied as SOFC anode materials. |
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