Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption
α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and...
Ausführliche Beschreibung
Autor*in: |
Sun, Suwen [verfasserIn] |
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Englisch |
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2017transfer abstract |
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Enthalten in: Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving - Lu, Li ELSEVIER, 2020, including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science, New York, NY [u.a.] |
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Übergeordnetes Werk: |
volume:194 ; year:2017 ; day:15 ; month:06 ; pages:1-8 ; extent:8 |
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DOI / URN: |
10.1016/j.matchemphys.2017.03.023 |
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520 | |a α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. | ||
520 | |a α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. | ||
650 | 7 | |a Adsorption |2 Elsevier | |
650 | 7 | |a Visible light |2 Elsevier | |
650 | 7 | |a α-Fe2O3/g-C3N4 |2 Elsevier | |
650 | 7 | |a Arsenite |2 Elsevier | |
650 | 7 | |a Photocatalytic oxidation |2 Elsevier | |
700 | 1 | |a Ji, Chunnuan |4 oth | |
700 | 1 | |a Wu, Lingling |4 oth | |
700 | 1 | |a Chi, Shenghua |4 oth | |
700 | 1 | |a Qu, Rongjun |4 oth | |
700 | 1 | |a Li, Yan |4 oth | |
700 | 1 | |a Lu, Yangxiao |4 oth | |
700 | 1 | |a Sun, Changmei |4 oth | |
700 | 1 | |a Xue, Zhongxin |4 oth | |
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10.1016/j.matchemphys.2017.03.023 doi GBV00000000000264A.pica (DE-627)ELV020127766 (ELSEVIER)S0254-0584(17)30228-6 DE-627 ger DE-627 rakwb eng 540 530 540 DE-600 530 DE-600 610 VZ 44.38 bkl 44.91 bkl Sun, Suwen verfasserin aut Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. Adsorption Elsevier Visible light Elsevier α-Fe2O3/g-C3N4 Elsevier Arsenite Elsevier Photocatalytic oxidation Elsevier Ji, Chunnuan oth Wu, Lingling oth Chi, Shenghua oth Qu, Rongjun oth Li, Yan oth Lu, Yangxiao oth Sun, Changmei oth Xue, Zhongxin oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:194 year:2017 day:15 month:06 pages:1-8 extent:8 https://doi.org/10.1016/j.matchemphys.2017.03.023 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 194 2017 15 0615 1-8 8 045F 540 |
spelling |
10.1016/j.matchemphys.2017.03.023 doi GBV00000000000264A.pica (DE-627)ELV020127766 (ELSEVIER)S0254-0584(17)30228-6 DE-627 ger DE-627 rakwb eng 540 530 540 DE-600 530 DE-600 610 VZ 44.38 bkl 44.91 bkl Sun, Suwen verfasserin aut Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. Adsorption Elsevier Visible light Elsevier α-Fe2O3/g-C3N4 Elsevier Arsenite Elsevier Photocatalytic oxidation Elsevier Ji, Chunnuan oth Wu, Lingling oth Chi, Shenghua oth Qu, Rongjun oth Li, Yan oth Lu, Yangxiao oth Sun, Changmei oth Xue, Zhongxin oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:194 year:2017 day:15 month:06 pages:1-8 extent:8 https://doi.org/10.1016/j.matchemphys.2017.03.023 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 194 2017 15 0615 1-8 8 045F 540 |
allfields_unstemmed |
10.1016/j.matchemphys.2017.03.023 doi GBV00000000000264A.pica (DE-627)ELV020127766 (ELSEVIER)S0254-0584(17)30228-6 DE-627 ger DE-627 rakwb eng 540 530 540 DE-600 530 DE-600 610 VZ 44.38 bkl 44.91 bkl Sun, Suwen verfasserin aut Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. Adsorption Elsevier Visible light Elsevier α-Fe2O3/g-C3N4 Elsevier Arsenite Elsevier Photocatalytic oxidation Elsevier Ji, Chunnuan oth Wu, Lingling oth Chi, Shenghua oth Qu, Rongjun oth Li, Yan oth Lu, Yangxiao oth Sun, Changmei oth Xue, Zhongxin oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:194 year:2017 day:15 month:06 pages:1-8 extent:8 https://doi.org/10.1016/j.matchemphys.2017.03.023 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 194 2017 15 0615 1-8 8 045F 540 |
allfieldsGer |
10.1016/j.matchemphys.2017.03.023 doi GBV00000000000264A.pica (DE-627)ELV020127766 (ELSEVIER)S0254-0584(17)30228-6 DE-627 ger DE-627 rakwb eng 540 530 540 DE-600 530 DE-600 610 VZ 44.38 bkl 44.91 bkl Sun, Suwen verfasserin aut Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. Adsorption Elsevier Visible light Elsevier α-Fe2O3/g-C3N4 Elsevier Arsenite Elsevier Photocatalytic oxidation Elsevier Ji, Chunnuan oth Wu, Lingling oth Chi, Shenghua oth Qu, Rongjun oth Li, Yan oth Lu, Yangxiao oth Sun, Changmei oth Xue, Zhongxin oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:194 year:2017 day:15 month:06 pages:1-8 extent:8 https://doi.org/10.1016/j.matchemphys.2017.03.023 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 194 2017 15 0615 1-8 8 045F 540 |
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10.1016/j.matchemphys.2017.03.023 doi GBV00000000000264A.pica (DE-627)ELV020127766 (ELSEVIER)S0254-0584(17)30228-6 DE-627 ger DE-627 rakwb eng 540 530 540 DE-600 530 DE-600 610 VZ 44.38 bkl 44.91 bkl Sun, Suwen verfasserin aut Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. Adsorption Elsevier Visible light Elsevier α-Fe2O3/g-C3N4 Elsevier Arsenite Elsevier Photocatalytic oxidation Elsevier Ji, Chunnuan oth Wu, Lingling oth Chi, Shenghua oth Qu, Rongjun oth Li, Yan oth Lu, Yangxiao oth Sun, Changmei oth Xue, Zhongxin oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:194 year:2017 day:15 month:06 pages:1-8 extent:8 https://doi.org/10.1016/j.matchemphys.2017.03.023 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 194 2017 15 0615 1-8 8 045F 540 |
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Enthalten in Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving New York, NY [u.a.] volume:194 year:2017 day:15 month:06 pages:1-8 extent:8 |
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Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving |
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Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption |
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facile one-pot construction of α-fe2o3/g-c3n4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption |
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Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption |
abstract |
α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. |
abstractGer |
α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. |
abstract_unstemmed |
α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated. |
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Facile one-pot construction of α-Fe2O3/g-C3N4 heterojunction for arsenic removal by synchronous visible light catalysis oxidation and adsorption |
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https://doi.org/10.1016/j.matchemphys.2017.03.023 |
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Ji, Chunnuan Wu, Lingling Chi, Shenghua Qu, Rongjun Li, Yan Lu, Yangxiao Sun, Changmei Xue, Zhongxin |
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A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">α-Fe2O3/g-C3N4 composites with heterojunction were prepared by facile one-pot synthesis using ferric chloride and dicyandiamide as precursors. The newly formed composites were applied to remove arsenic from aqueous solution for the first time through synchronous visible light catalysis oxidation and adsorption. α-Fe2O3/g-C3N4 composites were characterized by wide-angle X-ray powder diffraction, transmission electron microscopy, high-resolution transmission electron microscopy, X-ray photoelectron spectroscopy, UV–Vis diffuse reflectance spectroscopy, and BET surface analysis. Under visible light irradiation, As(III) was oxidized to As(V) efficiently on the surface of α-Fe2O3/g-C3N4. In addition, the oxidized arsenic could be adsorbed in situ, resulting in the effective arsenic removal. The enhancement of photocatalytic activity the composites was attributed to the construction of heterojunction between α-Fe2O3 and g-C3N4. A possible oxidation mechanism of the as-composites for As(III) under visible light irradiation was also elucidated.</subfield></datafield><datafield tag="650" ind1=" " ind2="7"><subfield code="a">Adsorption</subfield><subfield code="2">Elsevier</subfield></datafield><datafield tag="650" ind1=" " ind2="7"><subfield code="a">Visible light</subfield><subfield code="2">Elsevier</subfield></datafield><datafield tag="650" ind1=" " ind2="7"><subfield code="a">α-Fe2O3/g-C3N4</subfield><subfield code="2">Elsevier</subfield></datafield><datafield tag="650" ind1=" " ind2="7"><subfield code="a">Arsenite</subfield><subfield code="2">Elsevier</subfield></datafield><datafield tag="650" ind1=" " ind2="7"><subfield code="a">Photocatalytic oxidation</subfield><subfield code="2">Elsevier</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Ji, Chunnuan</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Wu, Lingling</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Chi, Shenghua</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Qu, Rongjun</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Li, Yan</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Lu, Yangxiao</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Sun, Changmei</subfield><subfield code="4">oth</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Xue, Zhongxin</subfield><subfield code="4">oth</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="n">Elsevier</subfield><subfield code="a">Lu, Li ELSEVIER</subfield><subfield code="t">Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving</subfield><subfield code="d">2020</subfield><subfield code="d">including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science</subfield><subfield code="g">New York, NY [u.a.]</subfield><subfield code="w">(DE-627)ELV005250781</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:194</subfield><subfield code="g">year:2017</subfield><subfield code="g">day:15</subfield><subfield code="g">month:06</subfield><subfield code="g">pages:1-8</subfield><subfield code="g">extent:8</subfield></datafield><datafield tag="856" ind1="4" ind2="0"><subfield code="u">https://doi.org/10.1016/j.matchemphys.2017.03.023</subfield><subfield code="3">Volltext</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ELV</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SYSFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-PHA</subfield></datafield><datafield tag="936" ind1="b" ind2="k"><subfield code="a">44.38</subfield><subfield code="j">Pharmakologie</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="936" ind1="b" ind2="k"><subfield code="a">44.91</subfield><subfield code="j">Psychiatrie</subfield><subfield code="j">Psychopathologie</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="951" ind1=" " ind2=" "><subfield code="a">AR</subfield></datafield><datafield tag="952" ind1=" " ind2=" "><subfield code="d">194</subfield><subfield code="j">2017</subfield><subfield code="b">15</subfield><subfield code="c">0615</subfield><subfield code="h">1-8</subfield><subfield code="g">8</subfield></datafield><datafield tag="953" ind1=" " ind2=" "><subfield code="2">045F</subfield><subfield code="a">540</subfield></datafield></record></collection>
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