Studies on intrinsic phase-dependent electrochemical properties of MnS nanocrystals as anodes for lithium-ion batteries
Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion b...
Ausführliche Beschreibung
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| Autor*in: |
Hao, Yong [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2017transfer abstract |
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| Umfang: |
8 |
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| Übergeordnetes Werk: |
Enthalten in: Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method - Xiao, Hong ELSEVIER, 2013, the international journal on the science and technology of electrochemical energy systems, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:338 ; year:2017 ; day:15 ; month:01 ; pages:9-16 ; extent:8 |
| Links: |
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| DOI / URN: |
10.1016/j.jpowsour.2016.11.032 |
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ELV020292163 |
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| 520 | |a Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. | ||
| 520 | |a Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. | ||
| 650 | 7 | |a Lithium-ion batteries |2 Elsevier | |
| 650 | 7 | |a Electrochemical performance |2 Elsevier | |
| 650 | 7 | |a Manganese sulfide nanocrystals |2 Elsevier | |
| 650 | 7 | |a Anode |2 Elsevier | |
| 650 | 7 | |a Capacity increase |2 Elsevier | |
| 700 | 1 | |a Chen, Chunhui |4 oth | |
| 700 | 1 | |a Yang, Xinyi |4 oth | |
| 700 | 1 | |a Xiao, Guanjun |4 oth | |
| 700 | 1 | |a Zou, Bo |4 oth | |
| 700 | 1 | |a Yang, Jianwen |4 oth | |
| 700 | 1 | |a Wang, Chunlei |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Xiao, Hong ELSEVIER |t Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |d 2013 |d the international journal on the science and technology of electrochemical energy systems |g New York, NY [u.a.] |w (DE-627)ELV00098745X |
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10.1016/j.jpowsour.2016.11.032 doi GBV00000000000050A.pica (DE-627)ELV020292163 (ELSEVIER)S0378-7753(16)31555-5 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hao, Yong verfasserin aut Studies on intrinsic phase-dependent electrochemical properties of MnS nanocrystals as anodes for lithium-ion batteries 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Lithium-ion batteries Elsevier Electrochemical performance Elsevier Manganese sulfide nanocrystals Elsevier Anode Elsevier Capacity increase Elsevier Chen, Chunhui oth Yang, Xinyi oth Xiao, Guanjun oth Zou, Bo oth Yang, Jianwen oth Wang, Chunlei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:338 year:2017 day:15 month:01 pages:9-16 extent:8 https://doi.org/10.1016/j.jpowsour.2016.11.032 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 338 2017 15 0115 9-16 8 045F 620 |
| spelling |
10.1016/j.jpowsour.2016.11.032 doi GBV00000000000050A.pica (DE-627)ELV020292163 (ELSEVIER)S0378-7753(16)31555-5 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hao, Yong verfasserin aut Studies on intrinsic phase-dependent electrochemical properties of MnS nanocrystals as anodes for lithium-ion batteries 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Lithium-ion batteries Elsevier Electrochemical performance Elsevier Manganese sulfide nanocrystals Elsevier Anode Elsevier Capacity increase Elsevier Chen, Chunhui oth Yang, Xinyi oth Xiao, Guanjun oth Zou, Bo oth Yang, Jianwen oth Wang, Chunlei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:338 year:2017 day:15 month:01 pages:9-16 extent:8 https://doi.org/10.1016/j.jpowsour.2016.11.032 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 338 2017 15 0115 9-16 8 045F 620 |
| allfields_unstemmed |
10.1016/j.jpowsour.2016.11.032 doi GBV00000000000050A.pica (DE-627)ELV020292163 (ELSEVIER)S0378-7753(16)31555-5 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hao, Yong verfasserin aut Studies on intrinsic phase-dependent electrochemical properties of MnS nanocrystals as anodes for lithium-ion batteries 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Lithium-ion batteries Elsevier Electrochemical performance Elsevier Manganese sulfide nanocrystals Elsevier Anode Elsevier Capacity increase Elsevier Chen, Chunhui oth Yang, Xinyi oth Xiao, Guanjun oth Zou, Bo oth Yang, Jianwen oth Wang, Chunlei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:338 year:2017 day:15 month:01 pages:9-16 extent:8 https://doi.org/10.1016/j.jpowsour.2016.11.032 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 338 2017 15 0115 9-16 8 045F 620 |
| allfieldsGer |
10.1016/j.jpowsour.2016.11.032 doi GBV00000000000050A.pica (DE-627)ELV020292163 (ELSEVIER)S0378-7753(16)31555-5 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hao, Yong verfasserin aut Studies on intrinsic phase-dependent electrochemical properties of MnS nanocrystals as anodes for lithium-ion batteries 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Lithium-ion batteries Elsevier Electrochemical performance Elsevier Manganese sulfide nanocrystals Elsevier Anode Elsevier Capacity increase Elsevier Chen, Chunhui oth Yang, Xinyi oth Xiao, Guanjun oth Zou, Bo oth Yang, Jianwen oth Wang, Chunlei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:338 year:2017 day:15 month:01 pages:9-16 extent:8 https://doi.org/10.1016/j.jpowsour.2016.11.032 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 338 2017 15 0115 9-16 8 045F 620 |
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10.1016/j.jpowsour.2016.11.032 doi GBV00000000000050A.pica (DE-627)ELV020292163 (ELSEVIER)S0378-7753(16)31555-5 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hao, Yong verfasserin aut Studies on intrinsic phase-dependent electrochemical properties of MnS nanocrystals as anodes for lithium-ion batteries 2017transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. Lithium-ion batteries Elsevier Electrochemical performance Elsevier Manganese sulfide nanocrystals Elsevier Anode Elsevier Capacity increase Elsevier Chen, Chunhui oth Yang, Xinyi oth Xiao, Guanjun oth Zou, Bo oth Yang, Jianwen oth Wang, Chunlei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:338 year:2017 day:15 month:01 pages:9-16 extent:8 https://doi.org/10.1016/j.jpowsour.2016.11.032 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 338 2017 15 0115 9-16 8 045F 620 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:338 year:2017 day:15 month:01 pages:9-16 extent:8 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:338 year:2017 day:15 month:01 pages:9-16 extent:8 |
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Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |
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However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. 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studies on intrinsic phase-dependent electrochemical properties of mns nanocrystals as anodes for lithium-ion batteries |
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Studies on intrinsic phase-dependent electrochemical properties of MnS nanocrystals as anodes for lithium-ion batteries |
| abstract |
Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. |
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Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. |
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Manganese sulfide (MnS), a member of transition metal sulfides, has been considered as a promising anode material for reversible Li storage due to its high theoretical capacity and structural advantages. However, the intrinsic electrochemical performance of MnS with different phases in lithium-ion batteries is yet to be fully investigated. Herein, high purity rock-salt (RS), zinc-blende (ZB) and wurtzite (WZ) MnS nanocrystals with different morphologies were successfully synthesized via a facile solvothermal method. The RS-MnS, ZB-MnS and WZ-MnS electrodes showed the capacities of 232.5 mAh g−1, 287.9 mAh g−1 and 79.8 mAh g−1 at the 600th cycle, respectively. ZB-MnS displayed the best performance in terms of specific capacity and cyclability in comparison to RS-MnS and WZ-MnS nanocrystals. Interestingly, all the three kinds of MnS electrodes exhibited an unusual phenomenon of capacity increase upon cycling along with reduced particle sizes and without change in crystallinity. The main contribution of capacity increase was ascribed to the decreased cell resistance and enhanced interfacial charge storage, which facilitated more effective Li+ diffusion into electrode materials. |
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Studies on intrinsic phase-dependent electrochemical properties of MnS nanocrystals as anodes for lithium-ion batteries |
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