Interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties
The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all...
Ausführliche Beschreibung
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| Autor*in: |
Nikogeorgos, Nikolaos [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2016transfer abstract |
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| Schlagwörter: |
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| Umfang: |
11 |
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| Übergeordnetes Werk: |
Enthalten in: Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study - Fitzgerald, Emily ELSEVIER, 2020, the international journal for the science and technology of polymers, Oxford |
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| Übergeordnetes Werk: |
volume:100 ; year:2016 ; day:25 ; month:09 ; pages:158-168 ; extent:11 |
| Links: |
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| DOI / URN: |
10.1016/j.polymer.2016.08.030 |
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| 520 | |a The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. | ||
| 520 | |a The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. | ||
| 650 | 7 | |a PLL |2 Elsevier | |
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| 700 | 1 | |a Lee, Seunghwan |4 oth | |
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10.1016/j.polymer.2016.08.030 doi GBVA2016023000001.pica (DE-627)ELV024906964 (ELSEVIER)S0032-3861(16)30687-5 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.63 bkl 44.69 bkl Nikogeorgos, Nikolaos verfasserin aut Interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties 2016transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. PLL Elsevier PEI Elsevier PAH Elsevier Mucins Elsevier Biolubrication Elsevier Mucoadhesion Elsevier Patil, Navinkumar J. oth Zappone, Bruno oth Lee, Seunghwan oth Enthalten in Elsevier Science Fitzgerald, Emily ELSEVIER Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study 2020 the international journal for the science and technology of polymers Oxford (DE-627)ELV005093368 volume:100 year:2016 day:25 month:09 pages:158-168 extent:11 https://doi.org/10.1016/j.polymer.2016.08.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.63 Krankenpflege VZ 44.69 Intensivmedizin VZ AR 100 2016 25 0925 158-168 11 045F 540 |
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10.1016/j.polymer.2016.08.030 doi GBVA2016023000001.pica (DE-627)ELV024906964 (ELSEVIER)S0032-3861(16)30687-5 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.63 bkl 44.69 bkl Nikogeorgos, Nikolaos verfasserin aut Interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties 2016transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. PLL Elsevier PEI Elsevier PAH Elsevier Mucins Elsevier Biolubrication Elsevier Mucoadhesion Elsevier Patil, Navinkumar J. oth Zappone, Bruno oth Lee, Seunghwan oth Enthalten in Elsevier Science Fitzgerald, Emily ELSEVIER Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study 2020 the international journal for the science and technology of polymers Oxford (DE-627)ELV005093368 volume:100 year:2016 day:25 month:09 pages:158-168 extent:11 https://doi.org/10.1016/j.polymer.2016.08.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.63 Krankenpflege VZ 44.69 Intensivmedizin VZ AR 100 2016 25 0925 158-168 11 045F 540 |
| allfields_unstemmed |
10.1016/j.polymer.2016.08.030 doi GBVA2016023000001.pica (DE-627)ELV024906964 (ELSEVIER)S0032-3861(16)30687-5 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.63 bkl 44.69 bkl Nikogeorgos, Nikolaos verfasserin aut Interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties 2016transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. PLL Elsevier PEI Elsevier PAH Elsevier Mucins Elsevier Biolubrication Elsevier Mucoadhesion Elsevier Patil, Navinkumar J. oth Zappone, Bruno oth Lee, Seunghwan oth Enthalten in Elsevier Science Fitzgerald, Emily ELSEVIER Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study 2020 the international journal for the science and technology of polymers Oxford (DE-627)ELV005093368 volume:100 year:2016 day:25 month:09 pages:158-168 extent:11 https://doi.org/10.1016/j.polymer.2016.08.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.63 Krankenpflege VZ 44.69 Intensivmedizin VZ AR 100 2016 25 0925 158-168 11 045F 540 |
| allfieldsGer |
10.1016/j.polymer.2016.08.030 doi GBVA2016023000001.pica (DE-627)ELV024906964 (ELSEVIER)S0032-3861(16)30687-5 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.63 bkl 44.69 bkl Nikogeorgos, Nikolaos verfasserin aut Interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties 2016transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. PLL Elsevier PEI Elsevier PAH Elsevier Mucins Elsevier Biolubrication Elsevier Mucoadhesion Elsevier Patil, Navinkumar J. oth Zappone, Bruno oth Lee, Seunghwan oth Enthalten in Elsevier Science Fitzgerald, Emily ELSEVIER Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study 2020 the international journal for the science and technology of polymers Oxford (DE-627)ELV005093368 volume:100 year:2016 day:25 month:09 pages:158-168 extent:11 https://doi.org/10.1016/j.polymer.2016.08.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.63 Krankenpflege VZ 44.69 Intensivmedizin VZ AR 100 2016 25 0925 158-168 11 045F 540 |
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10.1016/j.polymer.2016.08.030 doi GBVA2016023000001.pica (DE-627)ELV024906964 (ELSEVIER)S0032-3861(16)30687-5 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 44.63 bkl 44.69 bkl Nikogeorgos, Nikolaos verfasserin aut Interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties 2016transfer abstract 11 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. PLL Elsevier PEI Elsevier PAH Elsevier Mucins Elsevier Biolubrication Elsevier Mucoadhesion Elsevier Patil, Navinkumar J. oth Zappone, Bruno oth Lee, Seunghwan oth Enthalten in Elsevier Science Fitzgerald, Emily ELSEVIER Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study 2020 the international journal for the science and technology of polymers Oxford (DE-627)ELV005093368 volume:100 year:2016 day:25 month:09 pages:158-168 extent:11 https://doi.org/10.1016/j.polymer.2016.08.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.63 Krankenpflege VZ 44.69 Intensivmedizin VZ AR 100 2016 25 0925 158-168 11 045F 540 |
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Enthalten in Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study Oxford volume:100 year:2016 day:25 month:09 pages:158-168 extent:11 |
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Enthalten in Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study Oxford volume:100 year:2016 day:25 month:09 pages:158-168 extent:11 |
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Functional outcomes at 12 months for patients with traumatic brain injury, intracerebral haemorrhage and subarachnoid haemorrhage treated in an Australian neurocritical care unit: A prospective cohort study |
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interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties |
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Interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties |
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The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. |
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The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. |
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The interaction of porcine gastric mucin (PGM) with polycations possessing amine functional groups, including polyallylamine hydrochloride (PAH), poly-l-lysine (PLL) and polyethylenimine (PEI), was examined from a tribological standpoint at a self-mated polydimethylsiloxane (PDMS) interface. In all cases, PGM interacted with the cationic polymers, leading to a smaller size of the aggregates compared to PGM, surface charge compensation, and distortion of the PGM protein conformation. But, a synergistic lubrication effect was clearly observed only from the 1/1 (w/w) mixture of PGM with branched PEI (B-PEI) where the friction coefficient was reduced by two orders of magnitude compared to neat PGM or B-PEI in the speed range of 0.25–100 mm/s. This was attributed to the smallest hydrodynamic size and “sphere-like” conformation of B-PEI due to high degree of branching, which favors tenacious complexation with PGM, fast surface adsorption, and continuous reformation of the lubricating layer under cyclic tribostress in pin-on-disc tribometry. |
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Interaction of porcine gastric mucin with various polycations and its influence on the boundary lubrication properties |
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