An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport
We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to P...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
He, Yinghui [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2017transfer abstract |
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| Umfang: |
9 |
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| Übergeordnetes Werk: |
Enthalten in: Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands - saleh, Dalia I ELSEVIER, 2022, physics, materials and applications, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:49 ; year:2017 ; pages:406-414 ; extent:9 |
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| DOI / URN: |
10.1016/j.orgel.2017.07.016 |
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| 245 | 1 | 0 | |a An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport |
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| 520 | |a We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. | ||
| 520 | |a We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. | ||
| 650 | 7 | |a Ambipolar polymer |2 Elsevier | |
| 650 | 7 | |a Low off current |2 Elsevier | |
| 650 | 7 | |a Unipolar n-type OTFTs |2 Elsevier | |
| 650 | 7 | |a Amine-containing polymer |2 Elsevier | |
| 650 | 7 | |a Hole trapping |2 Elsevier | |
| 700 | 1 | |a Quinn, Jesse T.E. |4 oth | |
| 700 | 1 | |a Lee, Suhyun |4 oth | |
| 700 | 1 | |a Wang, Guan Ying |4 oth | |
| 700 | 1 | |a Li, Xu |4 oth | |
| 700 | 1 | |a Wang, Jinliang |4 oth | |
| 700 | 1 | |a Li, Yuning |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a saleh, Dalia I ELSEVIER |t Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |d 2022 |d physics, materials and applications |g Amsterdam [u.a.] |w (DE-627)ELV007843747 |
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10.1016/j.orgel.2017.07.016 doi GBV00000000000385.pica (DE-627)ELV025130978 (ELSEVIER)S1566-1199(17)30348-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl He, Yinghui verfasserin aut An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport 2017transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. Ambipolar polymer Elsevier Low off current Elsevier Unipolar n-type OTFTs Elsevier Amine-containing polymer Elsevier Hole trapping Elsevier Quinn, Jesse T.E. oth Lee, Suhyun oth Wang, Guan Ying oth Li, Xu oth Wang, Jinliang oth Li, Yuning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:49 year:2017 pages:406-414 extent:9 https://doi.org/10.1016/j.orgel.2017.07.016 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 49 2017 406-414 9 |
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10.1016/j.orgel.2017.07.016 doi GBV00000000000385.pica (DE-627)ELV025130978 (ELSEVIER)S1566-1199(17)30348-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl He, Yinghui verfasserin aut An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport 2017transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. Ambipolar polymer Elsevier Low off current Elsevier Unipolar n-type OTFTs Elsevier Amine-containing polymer Elsevier Hole trapping Elsevier Quinn, Jesse T.E. oth Lee, Suhyun oth Wang, Guan Ying oth Li, Xu oth Wang, Jinliang oth Li, Yuning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:49 year:2017 pages:406-414 extent:9 https://doi.org/10.1016/j.orgel.2017.07.016 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 49 2017 406-414 9 |
| allfields_unstemmed |
10.1016/j.orgel.2017.07.016 doi GBV00000000000385.pica (DE-627)ELV025130978 (ELSEVIER)S1566-1199(17)30348-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl He, Yinghui verfasserin aut An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport 2017transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. Ambipolar polymer Elsevier Low off current Elsevier Unipolar n-type OTFTs Elsevier Amine-containing polymer Elsevier Hole trapping Elsevier Quinn, Jesse T.E. oth Lee, Suhyun oth Wang, Guan Ying oth Li, Xu oth Wang, Jinliang oth Li, Yuning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:49 year:2017 pages:406-414 extent:9 https://doi.org/10.1016/j.orgel.2017.07.016 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 49 2017 406-414 9 |
| allfieldsGer |
10.1016/j.orgel.2017.07.016 doi GBV00000000000385.pica (DE-627)ELV025130978 (ELSEVIER)S1566-1199(17)30348-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl He, Yinghui verfasserin aut An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport 2017transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. Ambipolar polymer Elsevier Low off current Elsevier Unipolar n-type OTFTs Elsevier Amine-containing polymer Elsevier Hole trapping Elsevier Quinn, Jesse T.E. oth Lee, Suhyun oth Wang, Guan Ying oth Li, Xu oth Wang, Jinliang oth Li, Yuning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:49 year:2017 pages:406-414 extent:9 https://doi.org/10.1016/j.orgel.2017.07.016 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 49 2017 406-414 9 |
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10.1016/j.orgel.2017.07.016 doi GBV00000000000385.pica (DE-627)ELV025130978 (ELSEVIER)S1566-1199(17)30348-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl He, Yinghui verfasserin aut An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport 2017transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. Ambipolar polymer Elsevier Low off current Elsevier Unipolar n-type OTFTs Elsevier Amine-containing polymer Elsevier Hole trapping Elsevier Quinn, Jesse T.E. oth Lee, Suhyun oth Wang, Guan Ying oth Li, Xu oth Wang, Jinliang oth Li, Yuning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:49 year:2017 pages:406-414 extent:9 https://doi.org/10.1016/j.orgel.2017.07.016 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 49 2017 406-414 9 |
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English |
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Enthalten in Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands Amsterdam [u.a.] volume:49 year:2017 pages:406-414 extent:9 |
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Enthalten in Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands Amsterdam [u.a.] volume:49 year:2017 pages:406-414 extent:9 |
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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
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With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. 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An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport |
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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
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an aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport |
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An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport |
| abstract |
We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. |
| abstractGer |
We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. |
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We report the synthesis of an aromatic amine-containing polymer (PDPAT-12) and the use of this polymer as an effective additive to an ambipolar polymer semiconductor (PIBDFBT-e37) to realize unipolar n-type charge transport in organic thin film transistors (OTFTs). With 10 wt% PDPAT-12 addition to PIBDFBT-e37, the OTFTs achieved unipolar n-type charge transport with electron mobility of up to 0.42 cm2 V−1 s−1 in nitrogen and 0.19 cm2 V−1 s−1 in air. Moreover, the polymer blend demonstrated improved stability towards ambient air (retaining 50% of its initial electron mobility after exposed in air for 28 days) than the pristine PIBDFBT-e37 (retaining 13% of its initial electron mobility under the same conditions) and the PIBDFBT-e37:PEI (polyethylenimine) blend, which lost transistor behaviour almost instantly once exposed to ambient air. Our results show that the use of this aromatic amine-containing polymer as an additive can convert an ambipolar polymer into an n-type unipolar polymer in OTFTs with much improved air stability. |
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An aromatic amine-containing polymer as an additive to ambipolar polymer semiconductor realizing unipolar n-type charge transport |
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