Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol
Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Abd Hamid, S.B. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2017transfer abstract |
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| Umfang: |
5 |
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| Übergeordnetes Werk: |
Enthalten in: Using the Japanese version of the brief assessment of cognition in schizophrenia (BACS-J) to assess cognitive function in patients with REM sleep behavior disorder - Ubara, A. ELSEVIER, 2019, Amsterdam |
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| Übergeordnetes Werk: |
volume:94 ; year:2017 ; day:5 ; month:05 ; pages:18-22 ; extent:5 |
| Links: |
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| DOI / URN: |
10.1016/j.catcom.2017.02.006 |
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| 520 | |a Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. | ||
| 520 | |a Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. | ||
| 700 | 1 | |a Ambursa, Murtala M. |4 oth | |
| 700 | 1 | |a Sudarsanam, Putla |4 oth | |
| 700 | 1 | |a Voon, Lee Hwei |4 oth | |
| 700 | 1 | |a Bhargava, Suresh K. |4 oth | |
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10.1016/j.catcom.2017.02.006 doi GBVA2017006000012.pica (DE-627)ELV025136461 (ELSEVIER)S1566-7367(17)30051-1 DE-627 ger DE-627 rakwb eng 660 540 660 DE-600 540 DE-600 610 VZ 44.90 bkl Abd Hamid, S.B. verfasserin aut Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol 2017transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Ambursa, Murtala M. oth Sudarsanam, Putla oth Voon, Lee Hwei oth Bhargava, Suresh K. oth Enthalten in Elsevier Ubara, A. ELSEVIER Using the Japanese version of the brief assessment of cognition in schizophrenia (BACS-J) to assess cognitive function in patients with REM sleep behavior disorder 2019 Amsterdam (DE-627)ELV003313131 volume:94 year:2017 day:5 month:05 pages:18-22 extent:5 https://doi.org/10.1016/j.catcom.2017.02.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.90 Neurologie VZ AR 94 2017 5 0505 18-22 5 045F 660 |
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10.1016/j.catcom.2017.02.006 doi GBVA2017006000012.pica (DE-627)ELV025136461 (ELSEVIER)S1566-7367(17)30051-1 DE-627 ger DE-627 rakwb eng 660 540 660 DE-600 540 DE-600 610 VZ 44.90 bkl Abd Hamid, S.B. verfasserin aut Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol 2017transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Ambursa, Murtala M. oth Sudarsanam, Putla oth Voon, Lee Hwei oth Bhargava, Suresh K. oth Enthalten in Elsevier Ubara, A. ELSEVIER Using the Japanese version of the brief assessment of cognition in schizophrenia (BACS-J) to assess cognitive function in patients with REM sleep behavior disorder 2019 Amsterdam (DE-627)ELV003313131 volume:94 year:2017 day:5 month:05 pages:18-22 extent:5 https://doi.org/10.1016/j.catcom.2017.02.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.90 Neurologie VZ AR 94 2017 5 0505 18-22 5 045F 660 |
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10.1016/j.catcom.2017.02.006 doi GBVA2017006000012.pica (DE-627)ELV025136461 (ELSEVIER)S1566-7367(17)30051-1 DE-627 ger DE-627 rakwb eng 660 540 660 DE-600 540 DE-600 610 VZ 44.90 bkl Abd Hamid, S.B. verfasserin aut Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol 2017transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Ambursa, Murtala M. oth Sudarsanam, Putla oth Voon, Lee Hwei oth Bhargava, Suresh K. oth Enthalten in Elsevier Ubara, A. ELSEVIER Using the Japanese version of the brief assessment of cognition in schizophrenia (BACS-J) to assess cognitive function in patients with REM sleep behavior disorder 2019 Amsterdam (DE-627)ELV003313131 volume:94 year:2017 day:5 month:05 pages:18-22 extent:5 https://doi.org/10.1016/j.catcom.2017.02.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.90 Neurologie VZ AR 94 2017 5 0505 18-22 5 045F 660 |
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10.1016/j.catcom.2017.02.006 doi GBVA2017006000012.pica (DE-627)ELV025136461 (ELSEVIER)S1566-7367(17)30051-1 DE-627 ger DE-627 rakwb eng 660 540 660 DE-600 540 DE-600 610 VZ 44.90 bkl Abd Hamid, S.B. verfasserin aut Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol 2017transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Ambursa, Murtala M. oth Sudarsanam, Putla oth Voon, Lee Hwei oth Bhargava, Suresh K. oth Enthalten in Elsevier Ubara, A. ELSEVIER Using the Japanese version of the brief assessment of cognition in schizophrenia (BACS-J) to assess cognitive function in patients with REM sleep behavior disorder 2019 Amsterdam (DE-627)ELV003313131 volume:94 year:2017 day:5 month:05 pages:18-22 extent:5 https://doi.org/10.1016/j.catcom.2017.02.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.90 Neurologie VZ AR 94 2017 5 0505 18-22 5 045F 660 |
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10.1016/j.catcom.2017.02.006 doi GBVA2017006000012.pica (DE-627)ELV025136461 (ELSEVIER)S1566-7367(17)30051-1 DE-627 ger DE-627 rakwb eng 660 540 660 DE-600 540 DE-600 610 VZ 44.90 bkl Abd Hamid, S.B. verfasserin aut Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol 2017transfer abstract 5 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. Ambursa, Murtala M. oth Sudarsanam, Putla oth Voon, Lee Hwei oth Bhargava, Suresh K. oth Enthalten in Elsevier Ubara, A. ELSEVIER Using the Japanese version of the brief assessment of cognition in schizophrenia (BACS-J) to assess cognitive function in patients with REM sleep behavior disorder 2019 Amsterdam (DE-627)ELV003313131 volume:94 year:2017 day:5 month:05 pages:18-22 extent:5 https://doi.org/10.1016/j.catcom.2017.02.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.90 Neurologie VZ AR 94 2017 5 0505 18-22 5 045F 660 |
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Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol |
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Using the Japanese version of the brief assessment of cognition in schizophrenia (BACS-J) to assess cognitive function in patients with REM sleep behavior disorder |
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effect of ti loading on structure-activity properties of cu-ni/ti-mcm-41 catalysts in hydrodeoxygenation of guaiacol |
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Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol |
| abstract |
Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. |
| abstractGer |
Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. |
| abstract_unstemmed |
Various Cu-Ni/Ti-MCM-41 catalysts by varying Ti amount (Ti/Si=10, 20 and 30%) were synthesized for hydrodeoxygenation of guaiacol and characterized by XRD, N2 adsorption-desorption, NH3-TPD, H2-TPR and Raman spectroscopy. The Ti loading shows an adverse effect on the catalyst surface area. But, more number of acidic sites (5173.55μmol/g) were found for 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst. The 20% Ti loaded Cu-Ni/Ti-MCM-41 catalyst shows a high guaiacol conversion (74.2%) and cyclohexane selectivity (48.81%) which is due to abundant acid and redox sites: acid sites initiate removal of oxygen via dehydration, while hydrogenation of guaiacol to cyclohexane is promoted by redox sites. |
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Effect of Ti loading on structure-activity properties of Cu-Ni/Ti-MCM-41 catalysts in hydrodeoxygenation of guaiacol |
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