Superhydrophobic membranes via facile bio-inspired mineralization for vacuum membrane distillation
Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Zhong, Wenwei [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2017transfer abstract |
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| Schlagwörter: |
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| Umfang: |
10 |
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| Übergeordnetes Werk: |
Enthalten in: Steering charge kinetics in W - Yue, Xin-Zheng ELSEVIER, 2019, the official journal of the North American Membrane Society, New York, NY [u.a.] |
|---|---|
| Übergeordnetes Werk: |
volume:540 ; year:2017 ; day:15 ; month:10 ; pages:98-107 ; extent:10 |
| Links: |
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| DOI / URN: |
10.1016/j.memsci.2017.06.033 |
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| 520 | |a Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. | ||
| 520 | |a Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. | ||
| 650 | 7 | |a Membrane wetting |2 Elsevier | |
| 650 | 7 | |a Surface modification |2 Elsevier | |
| 650 | 7 | |a Superhydrophobic |2 Elsevier | |
| 650 | 7 | |a Vacuum membrane distillation |2 Elsevier | |
| 650 | 7 | |a Polydopamine |2 Elsevier | |
| 700 | 1 | |a Hou, Jingwei |4 oth | |
| 700 | 1 | |a Yang, Hao-Cheng |4 oth | |
| 700 | 1 | |a Chen, Vicki |4 oth | |
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10.1016/j.memsci.2017.06.033 doi GBV00000000000355.pica (DE-627)ELV025325507 (ELSEVIER)S0376-7388(17)30737-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Zhong, Wenwei verfasserin aut Superhydrophobic membranes via facile bio-inspired mineralization for vacuum membrane distillation 2017transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Membrane wetting Elsevier Surface modification Elsevier Superhydrophobic Elsevier Vacuum membrane distillation Elsevier Polydopamine Elsevier Hou, Jingwei oth Yang, Hao-Cheng oth Chen, Vicki oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:540 year:2017 day:15 month:10 pages:98-107 extent:10 https://doi.org/10.1016/j.memsci.2017.06.033 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 540 2017 15 1015 98-107 10 |
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10.1016/j.memsci.2017.06.033 doi GBV00000000000355.pica (DE-627)ELV025325507 (ELSEVIER)S0376-7388(17)30737-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Zhong, Wenwei verfasserin aut Superhydrophobic membranes via facile bio-inspired mineralization for vacuum membrane distillation 2017transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Membrane wetting Elsevier Surface modification Elsevier Superhydrophobic Elsevier Vacuum membrane distillation Elsevier Polydopamine Elsevier Hou, Jingwei oth Yang, Hao-Cheng oth Chen, Vicki oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:540 year:2017 day:15 month:10 pages:98-107 extent:10 https://doi.org/10.1016/j.memsci.2017.06.033 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 540 2017 15 1015 98-107 10 |
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10.1016/j.memsci.2017.06.033 doi GBV00000000000355.pica (DE-627)ELV025325507 (ELSEVIER)S0376-7388(17)30737-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Zhong, Wenwei verfasserin aut Superhydrophobic membranes via facile bio-inspired mineralization for vacuum membrane distillation 2017transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Membrane wetting Elsevier Surface modification Elsevier Superhydrophobic Elsevier Vacuum membrane distillation Elsevier Polydopamine Elsevier Hou, Jingwei oth Yang, Hao-Cheng oth Chen, Vicki oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:540 year:2017 day:15 month:10 pages:98-107 extent:10 https://doi.org/10.1016/j.memsci.2017.06.033 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 540 2017 15 1015 98-107 10 |
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10.1016/j.memsci.2017.06.033 doi GBV00000000000355.pica (DE-627)ELV025325507 (ELSEVIER)S0376-7388(17)30737-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Zhong, Wenwei verfasserin aut Superhydrophobic membranes via facile bio-inspired mineralization for vacuum membrane distillation 2017transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Membrane wetting Elsevier Surface modification Elsevier Superhydrophobic Elsevier Vacuum membrane distillation Elsevier Polydopamine Elsevier Hou, Jingwei oth Yang, Hao-Cheng oth Chen, Vicki oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:540 year:2017 day:15 month:10 pages:98-107 extent:10 https://doi.org/10.1016/j.memsci.2017.06.033 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 540 2017 15 1015 98-107 10 |
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10.1016/j.memsci.2017.06.033 doi GBV00000000000355.pica (DE-627)ELV025325507 (ELSEVIER)S0376-7388(17)30737-8 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Zhong, Wenwei verfasserin aut Superhydrophobic membranes via facile bio-inspired mineralization for vacuum membrane distillation 2017transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. Membrane wetting Elsevier Surface modification Elsevier Superhydrophobic Elsevier Vacuum membrane distillation Elsevier Polydopamine Elsevier Hou, Jingwei oth Yang, Hao-Cheng oth Chen, Vicki oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:540 year:2017 day:15 month:10 pages:98-107 extent:10 https://doi.org/10.1016/j.memsci.2017.06.033 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 540 2017 15 1015 98-107 10 |
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Superhydrophobic membranes via facile bio-inspired mineralization for vacuum membrane distillation |
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Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. |
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Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. |
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Growing interests have been shown on the application of vacuum membrane distillation (VMD) for desalination and concentrated effluent treatment due to its high mass transfer efficiency. However, VMD is more prone to severe membrane wetting, potentially due to the high-pressure difference across the membrane. Anti-wetting strategies such as frequent cleaning to remove the crystals and surface modification of the membrane to improve the intrinsic anti-wetting property are often investigated. The usual approach to enhance the surface hydrophobicity is to introduce a nanostructured surface or/and to reduce the surface energy by functionalisation. This work demonstrated a facile process to introduce a superhydrophobic layer on polypropylene hollow fiber membranes via a mussel-inspired modification technique. The membranes were deposited by polydopamine/polyethyleneimine, followed by the surface silicification and subsequent fluorination. We examined the surface morphologies, chemistry and wettability after each step of surface modification. The surface functional coating is ultrathin, which imposed a negligible effect on the membrane pore size. The final modified membranes exhibited comparable mass transfer with the virgin membrane, but superior wetting resistance in 35g/L NaCl solution for long term operation with the permeate conductivity < 10µS/cm for 50h. It also showed excellent cleaning efficiency in the long-term treatment of brackish groundwater concentrate. |
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