Formation of Dimethyl Carbonate on Nature Clay Supported Bimetallic Copper-Nickel Catalysts
Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differentia...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Zhou, Yingjie [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2015transfer abstract |
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| Schlagwörter: |
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| Umfang: |
9 |
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| Übergeordnetes Werk: |
Enthalten in: Self-assembled 3D hierarchical MnCO - Rajendiran, Rajmohan ELSEVIER, 2020, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:103 ; year:2015 ; day:15 ; month:09 ; pages:925-933 ; extent:9 |
| Links: |
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| DOI / URN: |
10.1016/j.jclepro.2014.08.075 |
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| 520 | |a Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. | ||
| 520 | |a Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. | ||
| 650 | 7 | |a Dimethyl carbonate |2 Elsevier | |
| 650 | 7 | |a Carbon dioxide |2 Elsevier | |
| 650 | 7 | |a Halloysite nanotubes |2 Elsevier | |
| 650 | 7 | |a Bimetallic catalyst |2 Elsevier | |
| 700 | 1 | |a Wang, Shuanjin |4 oth | |
| 700 | 1 | |a Xiao, Min |4 oth | |
| 700 | 1 | |a Han, Dongmei |4 oth | |
| 700 | 1 | |a Lu, Yixin |4 oth | |
| 700 | 1 | |a Meng, Yuezhong |4 oth | |
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10.1016/j.jclepro.2014.08.075 doi GBVA2015016000025.pica (DE-627)ELV029136342 (ELSEVIER)S0959-6526(14)00898-1 DE-627 ger DE-627 rakwb eng 690 330 690 DE-600 330 DE-600 540 VZ 35.18 bkl Zhou, Yingjie verfasserin aut Formation of Dimethyl Carbonate on Nature Clay Supported Bimetallic Copper-Nickel Catalysts 2015transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Dimethyl carbonate Elsevier Carbon dioxide Elsevier Halloysite nanotubes Elsevier Bimetallic catalyst Elsevier Wang, Shuanjin oth Xiao, Min oth Han, Dongmei oth Lu, Yixin oth Meng, Yuezhong oth Enthalten in Elsevier Science Rajendiran, Rajmohan ELSEVIER Self-assembled 3D hierarchical MnCO 2020 Amsterdam [u.a.] (DE-627)ELV003750353 volume:103 year:2015 day:15 month:09 pages:925-933 extent:9 https://doi.org/10.1016/j.jclepro.2014.08.075 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 35.18 Kolloidchemie Grenzflächenchemie VZ AR 103 2015 15 0915 925-933 9 045F 690 |
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10.1016/j.jclepro.2014.08.075 doi GBVA2015016000025.pica (DE-627)ELV029136342 (ELSEVIER)S0959-6526(14)00898-1 DE-627 ger DE-627 rakwb eng 690 330 690 DE-600 330 DE-600 540 VZ 35.18 bkl Zhou, Yingjie verfasserin aut Formation of Dimethyl Carbonate on Nature Clay Supported Bimetallic Copper-Nickel Catalysts 2015transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Dimethyl carbonate Elsevier Carbon dioxide Elsevier Halloysite nanotubes Elsevier Bimetallic catalyst Elsevier Wang, Shuanjin oth Xiao, Min oth Han, Dongmei oth Lu, Yixin oth Meng, Yuezhong oth Enthalten in Elsevier Science Rajendiran, Rajmohan ELSEVIER Self-assembled 3D hierarchical MnCO 2020 Amsterdam [u.a.] (DE-627)ELV003750353 volume:103 year:2015 day:15 month:09 pages:925-933 extent:9 https://doi.org/10.1016/j.jclepro.2014.08.075 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 35.18 Kolloidchemie Grenzflächenchemie VZ AR 103 2015 15 0915 925-933 9 045F 690 |
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10.1016/j.jclepro.2014.08.075 doi GBVA2015016000025.pica (DE-627)ELV029136342 (ELSEVIER)S0959-6526(14)00898-1 DE-627 ger DE-627 rakwb eng 690 330 690 DE-600 330 DE-600 540 VZ 35.18 bkl Zhou, Yingjie verfasserin aut Formation of Dimethyl Carbonate on Nature Clay Supported Bimetallic Copper-Nickel Catalysts 2015transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Dimethyl carbonate Elsevier Carbon dioxide Elsevier Halloysite nanotubes Elsevier Bimetallic catalyst Elsevier Wang, Shuanjin oth Xiao, Min oth Han, Dongmei oth Lu, Yixin oth Meng, Yuezhong oth Enthalten in Elsevier Science Rajendiran, Rajmohan ELSEVIER Self-assembled 3D hierarchical MnCO 2020 Amsterdam [u.a.] (DE-627)ELV003750353 volume:103 year:2015 day:15 month:09 pages:925-933 extent:9 https://doi.org/10.1016/j.jclepro.2014.08.075 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 35.18 Kolloidchemie Grenzflächenchemie VZ AR 103 2015 15 0915 925-933 9 045F 690 |
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10.1016/j.jclepro.2014.08.075 doi GBVA2015016000025.pica (DE-627)ELV029136342 (ELSEVIER)S0959-6526(14)00898-1 DE-627 ger DE-627 rakwb eng 690 330 690 DE-600 330 DE-600 540 VZ 35.18 bkl Zhou, Yingjie verfasserin aut Formation of Dimethyl Carbonate on Nature Clay Supported Bimetallic Copper-Nickel Catalysts 2015transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Dimethyl carbonate Elsevier Carbon dioxide Elsevier Halloysite nanotubes Elsevier Bimetallic catalyst Elsevier Wang, Shuanjin oth Xiao, Min oth Han, Dongmei oth Lu, Yixin oth Meng, Yuezhong oth Enthalten in Elsevier Science Rajendiran, Rajmohan ELSEVIER Self-assembled 3D hierarchical MnCO 2020 Amsterdam [u.a.] (DE-627)ELV003750353 volume:103 year:2015 day:15 month:09 pages:925-933 extent:9 https://doi.org/10.1016/j.jclepro.2014.08.075 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 35.18 Kolloidchemie Grenzflächenchemie VZ AR 103 2015 15 0915 925-933 9 045F 690 |
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10.1016/j.jclepro.2014.08.075 doi GBVA2015016000025.pica (DE-627)ELV029136342 (ELSEVIER)S0959-6526(14)00898-1 DE-627 ger DE-627 rakwb eng 690 330 690 DE-600 330 DE-600 540 VZ 35.18 bkl Zhou, Yingjie verfasserin aut Formation of Dimethyl Carbonate on Nature Clay Supported Bimetallic Copper-Nickel Catalysts 2015transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. Dimethyl carbonate Elsevier Carbon dioxide Elsevier Halloysite nanotubes Elsevier Bimetallic catalyst Elsevier Wang, Shuanjin oth Xiao, Min oth Han, Dongmei oth Lu, Yixin oth Meng, Yuezhong oth Enthalten in Elsevier Science Rajendiran, Rajmohan ELSEVIER Self-assembled 3D hierarchical MnCO 2020 Amsterdam [u.a.] (DE-627)ELV003750353 volume:103 year:2015 day:15 month:09 pages:925-933 extent:9 https://doi.org/10.1016/j.jclepro.2014.08.075 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 35.18 Kolloidchemie Grenzflächenchemie VZ AR 103 2015 15 0915 925-933 9 045F 690 |
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Enthalten in Self-assembled 3D hierarchical MnCO Amsterdam [u.a.] volume:103 year:2015 day:15 month:09 pages:925-933 extent:9 |
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Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. |
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Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. |
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Halloysite nanotubes supported Cu–Ni bimetallic catalysts were synthesized and applied to the direct formation of dimethyl carbonate (DMC) from methanol and CO2. Halloystite nanotubes (HNTs), K treated HNTs (KHNTs) and the synthesized catalysts were characterized by thermogravimetric and differential thermalgravimetric analysis (TG-DTA), temperature programmed reduction (TPR), X-ray photoelectron spectrum (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), X-ray powder diffraction (XRD), and temperature programmed desorption (TPD) techniques. The catalyst activities were evaluated in a continuous fixed-bed tubular microreactor under 1.2 MPa at 130 °C. The effects of the metal weight loadings on the catalytic performances and surface acid–base properties were studied. It was found that moderately acid–base balance on the catalysts surface were important for the DMC yield. |
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