Comprehensive review of methane conversion in solid oxide fuel cells: Prospects for efficient electricity generation from natural gas
Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly...
Ausführliche Beschreibung
Autor*in: |
Gür, Turgut M. [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
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2016transfer abstract |
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Umfang: |
64 |
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Übergeordnetes Werk: |
Enthalten in: A study on nanoindentation and tribological behaviour of multifunctional ZnO/PMMA nanocomposite - 2013transfer abstract, an international review journal, Amsterdam [u.a.] |
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Übergeordnetes Werk: |
volume:54 ; year:2016 ; pages:1-64 ; extent:64 |
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DOI / URN: |
10.1016/j.pecs.2015.10.004 |
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520 | |a Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. | ||
520 | |a Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. | ||
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10.1016/j.pecs.2015.10.004 doi GBVA2016012000023.pica (DE-627)ELV035349522 (ELSEVIER)S0360-1285(15)30049-6 DE-627 ger DE-627 rakwb eng 620 660 620 DE-600 660 DE-600 530 VZ 600 VZ 670 VZ 630 580 VZ BIODIV DE-30 fid 48.00 bkl Gür, Turgut M. verfasserin aut Comprehensive review of methane conversion in solid oxide fuel cells: Prospects for efficient electricity generation from natural gas 2016transfer abstract 64 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Enthalten in Elsevier Science A study on nanoindentation and tribological behaviour of multifunctional ZnO/PMMA nanocomposite 2013transfer abstract an international review journal Amsterdam [u.a.] (DE-627)ELV011493593 volume:54 year:2016 pages:1-64 extent:64 https://doi.org/10.1016/j.pecs.2015.10.004 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 54 2016 1-64 64 045F 620 |
spelling |
10.1016/j.pecs.2015.10.004 doi GBVA2016012000023.pica (DE-627)ELV035349522 (ELSEVIER)S0360-1285(15)30049-6 DE-627 ger DE-627 rakwb eng 620 660 620 DE-600 660 DE-600 530 VZ 600 VZ 670 VZ 630 580 VZ BIODIV DE-30 fid 48.00 bkl Gür, Turgut M. verfasserin aut Comprehensive review of methane conversion in solid oxide fuel cells: Prospects for efficient electricity generation from natural gas 2016transfer abstract 64 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Enthalten in Elsevier Science A study on nanoindentation and tribological behaviour of multifunctional ZnO/PMMA nanocomposite 2013transfer abstract an international review journal Amsterdam [u.a.] (DE-627)ELV011493593 volume:54 year:2016 pages:1-64 extent:64 https://doi.org/10.1016/j.pecs.2015.10.004 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 54 2016 1-64 64 045F 620 |
allfields_unstemmed |
10.1016/j.pecs.2015.10.004 doi GBVA2016012000023.pica (DE-627)ELV035349522 (ELSEVIER)S0360-1285(15)30049-6 DE-627 ger DE-627 rakwb eng 620 660 620 DE-600 660 DE-600 530 VZ 600 VZ 670 VZ 630 580 VZ BIODIV DE-30 fid 48.00 bkl Gür, Turgut M. verfasserin aut Comprehensive review of methane conversion in solid oxide fuel cells: Prospects for efficient electricity generation from natural gas 2016transfer abstract 64 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Enthalten in Elsevier Science A study on nanoindentation and tribological behaviour of multifunctional ZnO/PMMA nanocomposite 2013transfer abstract an international review journal Amsterdam [u.a.] (DE-627)ELV011493593 volume:54 year:2016 pages:1-64 extent:64 https://doi.org/10.1016/j.pecs.2015.10.004 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 54 2016 1-64 64 045F 620 |
allfieldsGer |
10.1016/j.pecs.2015.10.004 doi GBVA2016012000023.pica (DE-627)ELV035349522 (ELSEVIER)S0360-1285(15)30049-6 DE-627 ger DE-627 rakwb eng 620 660 620 DE-600 660 DE-600 530 VZ 600 VZ 670 VZ 630 580 VZ BIODIV DE-30 fid 48.00 bkl Gür, Turgut M. verfasserin aut Comprehensive review of methane conversion in solid oxide fuel cells: Prospects for efficient electricity generation from natural gas 2016transfer abstract 64 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Enthalten in Elsevier Science A study on nanoindentation and tribological behaviour of multifunctional ZnO/PMMA nanocomposite 2013transfer abstract an international review journal Amsterdam [u.a.] (DE-627)ELV011493593 volume:54 year:2016 pages:1-64 extent:64 https://doi.org/10.1016/j.pecs.2015.10.004 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 54 2016 1-64 64 045F 620 |
allfieldsSound |
10.1016/j.pecs.2015.10.004 doi GBVA2016012000023.pica (DE-627)ELV035349522 (ELSEVIER)S0360-1285(15)30049-6 DE-627 ger DE-627 rakwb eng 620 660 620 DE-600 660 DE-600 530 VZ 600 VZ 670 VZ 630 580 VZ BIODIV DE-30 fid 48.00 bkl Gür, Turgut M. verfasserin aut Comprehensive review of methane conversion in solid oxide fuel cells: Prospects for efficient electricity generation from natural gas 2016transfer abstract 64 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. Enthalten in Elsevier Science A study on nanoindentation and tribological behaviour of multifunctional ZnO/PMMA nanocomposite 2013transfer abstract an international review journal Amsterdam [u.a.] (DE-627)ELV011493593 volume:54 year:2016 pages:1-64 extent:64 https://doi.org/10.1016/j.pecs.2015.10.004 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 54 2016 1-64 64 045F 620 |
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comprehensive review of methane conversion in solid oxide fuel cells: prospects for efficient electricity generation from natural gas |
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Comprehensive review of methane conversion in solid oxide fuel cells: Prospects for efficient electricity generation from natural gas |
abstract |
Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. |
abstractGer |
Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. |
abstract_unstemmed |
Natural gas is an important energy resource for electric power generation and other energy needs. Recent discoveries of vast reserves of shale gas greatly increased its abundance while lowering its cost. Combined with its significantly smaller carbon-footprint than coal, natural gas has increasingly become the preferred choice to generate electrical power even at the expense of converting existing coal fired power plants to run on natural gas. However, most natural gas combustion-based power plants currently operate at efficiencies in the low 30%. Conversion of natural gas in solid oxide fuel cells (SOFC) promises to increase system level conversion efficiencies to above 60%, doubling the current efficiencies and significantly reducing the CO2 emissions by a factor of 2. Such dramatic improvements in conversion efficiency and ease of CO2 capture are currently out of reach for the combustion-based power generation technologies. Equally importantly, the CO2 produced from methane conversion leaves the fuel cell in a highly concentrated form. As nitrogen is blocked off by the impervious ceramic electrolyte of the SOFC from entering the process stream, methane oxidation produces a flue stream that is primarily made of the oxidation products CO2 and steam. The latter can easily be condensed out to capture CO2, thus eliminating the need for expensive and energy intensive post separation operations otherwise required to separate CO2 from N2 for storage purposes. So if successfully developed and deployed widely, natural gas conversion in SOFCs will greatly reduce CO2 emissions, help mitigate climate change, and minimize the environmental impact of power generation. |
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Comprehensive review of methane conversion in solid oxide fuel cells: Prospects for efficient electricity generation from natural gas |
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