Effects of H2O and CO2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames
The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flam...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Xu, Huanhuan [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2017transfer abstract |
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| Umfang: |
12 |
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| Übergeordnetes Werk: |
Enthalten in: Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments - Lloyd, C.E.M. ELSEVIER, 2014, the journal of the Combustion Institute, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:177 ; year:2017 ; pages:67-78 ; extent:12 |
| Links: |
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| DOI / URN: |
10.1016/j.combustflame.2016.12.001 |
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ELV036108294 |
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| 520 | |a The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. | ||
| 520 | |a The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. | ||
| 700 | 1 | |a Liu, Fengshan |4 oth | |
| 700 | 1 | |a Sun, Shaozeng |4 oth | |
| 700 | 1 | |a Zhao, Yijun |4 oth | |
| 700 | 1 | |a Meng, Shun |4 oth | |
| 700 | 1 | |a Tang, Wenbo |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a Lloyd, C.E.M. ELSEVIER |t Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments |d 2014 |d the journal of the Combustion Institute |g Amsterdam [u.a.] |w (DE-627)ELV018057144 |
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10.1016/j.combustflame.2016.12.001 doi GBV00000000000101A.pica (DE-627)ELV036108294 (ELSEVIER)S0010-2180(16)30364-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 610 VZ 74.00 bkl 44.73 bkl Xu, Huanhuan verfasserin aut Effects of H2O and CO2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames 2017transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. Liu, Fengshan oth Sun, Shaozeng oth Zhao, Yijun oth Meng, Shun oth Tang, Wenbo oth Enthalten in Elsevier Science Lloyd, C.E.M. ELSEVIER Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments 2014 the journal of the Combustion Institute Amsterdam [u.a.] (DE-627)ELV018057144 volume:177 year:2017 pages:67-78 extent:12 https://doi.org/10.1016/j.combustflame.2016.12.001 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_70 74.00 Geographie Anthropogeographie: Allgemeines VZ 44.73 Geomedizin VZ AR 177 2017 67-78 12 045F 620 |
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10.1016/j.combustflame.2016.12.001 doi GBV00000000000101A.pica (DE-627)ELV036108294 (ELSEVIER)S0010-2180(16)30364-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 610 VZ 74.00 bkl 44.73 bkl Xu, Huanhuan verfasserin aut Effects of H2O and CO2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames 2017transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. Liu, Fengshan oth Sun, Shaozeng oth Zhao, Yijun oth Meng, Shun oth Tang, Wenbo oth Enthalten in Elsevier Science Lloyd, C.E.M. ELSEVIER Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments 2014 the journal of the Combustion Institute Amsterdam [u.a.] (DE-627)ELV018057144 volume:177 year:2017 pages:67-78 extent:12 https://doi.org/10.1016/j.combustflame.2016.12.001 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_70 74.00 Geographie Anthropogeographie: Allgemeines VZ 44.73 Geomedizin VZ AR 177 2017 67-78 12 045F 620 |
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10.1016/j.combustflame.2016.12.001 doi GBV00000000000101A.pica (DE-627)ELV036108294 (ELSEVIER)S0010-2180(16)30364-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 610 VZ 74.00 bkl 44.73 bkl Xu, Huanhuan verfasserin aut Effects of H2O and CO2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames 2017transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. Liu, Fengshan oth Sun, Shaozeng oth Zhao, Yijun oth Meng, Shun oth Tang, Wenbo oth Enthalten in Elsevier Science Lloyd, C.E.M. ELSEVIER Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments 2014 the journal of the Combustion Institute Amsterdam [u.a.] (DE-627)ELV018057144 volume:177 year:2017 pages:67-78 extent:12 https://doi.org/10.1016/j.combustflame.2016.12.001 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_70 74.00 Geographie Anthropogeographie: Allgemeines VZ 44.73 Geomedizin VZ AR 177 2017 67-78 12 045F 620 |
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10.1016/j.combustflame.2016.12.001 doi GBV00000000000101A.pica (DE-627)ELV036108294 (ELSEVIER)S0010-2180(16)30364-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 610 VZ 74.00 bkl 44.73 bkl Xu, Huanhuan verfasserin aut Effects of H2O and CO2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames 2017transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. Liu, Fengshan oth Sun, Shaozeng oth Zhao, Yijun oth Meng, Shun oth Tang, Wenbo oth Enthalten in Elsevier Science Lloyd, C.E.M. ELSEVIER Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments 2014 the journal of the Combustion Institute Amsterdam [u.a.] (DE-627)ELV018057144 volume:177 year:2017 pages:67-78 extent:12 https://doi.org/10.1016/j.combustflame.2016.12.001 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_70 74.00 Geographie Anthropogeographie: Allgemeines VZ 44.73 Geomedizin VZ AR 177 2017 67-78 12 045F 620 |
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10.1016/j.combustflame.2016.12.001 doi GBV00000000000101A.pica (DE-627)ELV036108294 (ELSEVIER)S0010-2180(16)30364-9 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 610 VZ 74.00 bkl 44.73 bkl Xu, Huanhuan verfasserin aut Effects of H2O and CO2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames 2017transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. Liu, Fengshan oth Sun, Shaozeng oth Zhao, Yijun oth Meng, Shun oth Tang, Wenbo oth Enthalten in Elsevier Science Lloyd, C.E.M. ELSEVIER Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments 2014 the journal of the Combustion Institute Amsterdam [u.a.] (DE-627)ELV018057144 volume:177 year:2017 pages:67-78 extent:12 https://doi.org/10.1016/j.combustflame.2016.12.001 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_70 74.00 Geographie Anthropogeographie: Allgemeines VZ 44.73 Geomedizin VZ AR 177 2017 67-78 12 045F 620 |
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Enthalten in Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments Amsterdam [u.a.] volume:177 year:2017 pages:67-78 extent:12 |
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Methods for detecting change in hydrochemical time series in response to targeted pollutant mitigation in river catchments |
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effects of h2o and co2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames |
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Effects of H2O and CO2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames |
| abstract |
The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. |
| abstractGer |
The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. |
| abstract_unstemmed |
The effects of up to 30% H2O and CO2 replacement of N2 in air on the structure and shape of laminar coflow syngas (COH2) diffusion flames were experimentally and numerically studied. Temperatures along the flame centerline were measured using a type-B thermocouple. The OH*-chemiluminescence and flame luminance were captured respectively by an intensified CCD camera and a CCD camera to determine the flame height and radii. The syngas diffusion flames were numerically modeled using detailed thermal and transport properties and the chemical reaction mechanism of Davis et al. (2005). Four pairs of artificial species were introduced in additional numerical calculations to isolate the chemical, thermal, transport, and radiative effects of H2O and CO2. The experimental and numerical results show that H2O and CO2 replacement of N2 in the oxidizer reduce the peak flame temperature, but they influence the flame centerline temperature distributions differently. The thermal and radiative effects of both H2O and CO2 addition decrease the flame temperatures. The chemical and transport effects of CO2 and H2O affect flame temperatures differently. H2O addition promotes the OH concentration though H+O2 =O+OH and O+H2O=2OH, while CO2 addition decreases the OH concentration by suppressing those reactions. The higher concentrations of OH under H2O addition signify higher combustion intensity and hence lead to decreased flame height and radius. In contrast, the addition of CO2 suppresses flame temperature and the overall combustion process, resulting in increased flame height and radius. |
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Effects of H2O and CO2 diluted oxidizer on the structure and shape of laminar coflow syngas diffusion flames |
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