Catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor
The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficienc...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
ZHOU, Fu-xun [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2013transfer abstract |
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| Schlagwörter: |
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| Umfang: |
7 |
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| Übergeordnetes Werk: |
Enthalten in: Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis - Habara, Seiji ELSEVIER, 2015, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:41 ; year:2013 ; number:5 ; pages:523-529 ; extent:7 |
| Links: |
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| DOI / URN: |
10.1016/S1872-5813(13)60028-6 |
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ELV038759985 |
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| 245 | 1 | 0 | |a Catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor |
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| 520 | |a The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. | ||
| 520 | |a The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. | ||
| 650 | 7 | |a fluidized bed reactor |2 Elsevier | |
| 650 | 7 | |a deoxidization |2 Elsevier | |
| 650 | 7 | |a catalytic combustion |2 Elsevier | |
| 650 | 7 | |a coal mine methane |2 Elsevier | |
| 700 | 1 | |a ZHAO, Jian-tao |4 oth | |
| 700 | 1 | |a ZHANG, Lei |4 oth | |
| 700 | 1 | |a WU, Zhi-wei |4 oth | |
| 700 | 1 | |a WANG, Jian-guo |4 oth | |
| 700 | 1 | |a FANG, Yi-tian |4 oth | |
| 700 | 1 | |a QIN, Zhang-feng |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Habara, Seiji ELSEVIER |t Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis |d 2015 |g Amsterdam [u.a.] |w (DE-627)ELV013083767 |
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10.1016/S1872-5813(13)60028-6 doi GBVA2013009000012.pica (DE-627)ELV038759985 (ELSEVIER)S1872-5813(13)60028-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 600 690 VZ 51.00 bkl 51.32 bkl ZHOU, Fu-xun verfasserin aut Catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor 2013transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. fluidized bed reactor Elsevier deoxidization Elsevier catalytic combustion Elsevier coal mine methane Elsevier ZHAO, Jian-tao oth ZHANG, Lei oth WU, Zhi-wei oth WANG, Jian-guo oth FANG, Yi-tian oth QIN, Zhang-feng oth Enthalten in Elsevier Habara, Seiji ELSEVIER Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis 2015 Amsterdam [u.a.] (DE-627)ELV013083767 volume:41 year:2013 number:5 pages:523-529 extent:7 https://doi.org/10.1016/S1872-5813(13)60028-6 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.00 Werkstoffkunde: Allgemeines VZ 51.32 Werkstoffmechanik VZ AR 41 2013 5 523-529 7 045F 540 |
| spelling |
10.1016/S1872-5813(13)60028-6 doi GBVA2013009000012.pica (DE-627)ELV038759985 (ELSEVIER)S1872-5813(13)60028-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 600 690 VZ 51.00 bkl 51.32 bkl ZHOU, Fu-xun verfasserin aut Catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor 2013transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. fluidized bed reactor Elsevier deoxidization Elsevier catalytic combustion Elsevier coal mine methane Elsevier ZHAO, Jian-tao oth ZHANG, Lei oth WU, Zhi-wei oth WANG, Jian-guo oth FANG, Yi-tian oth QIN, Zhang-feng oth Enthalten in Elsevier Habara, Seiji ELSEVIER Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis 2015 Amsterdam [u.a.] (DE-627)ELV013083767 volume:41 year:2013 number:5 pages:523-529 extent:7 https://doi.org/10.1016/S1872-5813(13)60028-6 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.00 Werkstoffkunde: Allgemeines VZ 51.32 Werkstoffmechanik VZ AR 41 2013 5 523-529 7 045F 540 |
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10.1016/S1872-5813(13)60028-6 doi GBVA2013009000012.pica (DE-627)ELV038759985 (ELSEVIER)S1872-5813(13)60028-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 600 690 VZ 51.00 bkl 51.32 bkl ZHOU, Fu-xun verfasserin aut Catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor 2013transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. fluidized bed reactor Elsevier deoxidization Elsevier catalytic combustion Elsevier coal mine methane Elsevier ZHAO, Jian-tao oth ZHANG, Lei oth WU, Zhi-wei oth WANG, Jian-guo oth FANG, Yi-tian oth QIN, Zhang-feng oth Enthalten in Elsevier Habara, Seiji ELSEVIER Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis 2015 Amsterdam [u.a.] (DE-627)ELV013083767 volume:41 year:2013 number:5 pages:523-529 extent:7 https://doi.org/10.1016/S1872-5813(13)60028-6 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.00 Werkstoffkunde: Allgemeines VZ 51.32 Werkstoffmechanik VZ AR 41 2013 5 523-529 7 045F 540 |
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10.1016/S1872-5813(13)60028-6 doi GBVA2013009000012.pica (DE-627)ELV038759985 (ELSEVIER)S1872-5813(13)60028-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 600 690 VZ 51.00 bkl 51.32 bkl ZHOU, Fu-xun verfasserin aut Catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor 2013transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. fluidized bed reactor Elsevier deoxidization Elsevier catalytic combustion Elsevier coal mine methane Elsevier ZHAO, Jian-tao oth ZHANG, Lei oth WU, Zhi-wei oth WANG, Jian-guo oth FANG, Yi-tian oth QIN, Zhang-feng oth Enthalten in Elsevier Habara, Seiji ELSEVIER Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis 2015 Amsterdam [u.a.] (DE-627)ELV013083767 volume:41 year:2013 number:5 pages:523-529 extent:7 https://doi.org/10.1016/S1872-5813(13)60028-6 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.00 Werkstoffkunde: Allgemeines VZ 51.32 Werkstoffmechanik VZ AR 41 2013 5 523-529 7 045F 540 |
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10.1016/S1872-5813(13)60028-6 doi GBVA2013009000012.pica (DE-627)ELV038759985 (ELSEVIER)S1872-5813(13)60028-6 DE-627 ger DE-627 rakwb eng 540 540 DE-600 610 VZ 600 690 VZ 51.00 bkl 51.32 bkl ZHOU, Fu-xun verfasserin aut Catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor 2013transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. fluidized bed reactor Elsevier deoxidization Elsevier catalytic combustion Elsevier coal mine methane Elsevier ZHAO, Jian-tao oth ZHANG, Lei oth WU, Zhi-wei oth WANG, Jian-guo oth FANG, Yi-tian oth QIN, Zhang-feng oth Enthalten in Elsevier Habara, Seiji ELSEVIER Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis 2015 Amsterdam [u.a.] (DE-627)ELV013083767 volume:41 year:2013 number:5 pages:523-529 extent:7 https://doi.org/10.1016/S1872-5813(13)60028-6 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.00 Werkstoffkunde: Allgemeines VZ 51.32 Werkstoffmechanik VZ AR 41 2013 5 523-529 7 045F 540 |
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Enthalten in Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis Amsterdam [u.a.] volume:41 year:2013 number:5 pages:523-529 extent:7 |
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Late Restenosis After Paclitaxel-Coated Balloon Angioplasty Occurs in Patients With Drug-Eluting Stent Restenosis |
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catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor |
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Catalytic deoxygenating characteristics of oxygen-bearing coal mine methane in the fluidized bed reactor |
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The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. |
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The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. |
| abstract_unstemmed |
The catalytic deoxygenating experiment of oxygen-bearing coal mine methane (CMM) was carried out in a bench-scale fluidized bed reactor with the spherical Cu-based catalyst. The effects of the bed temperature, the particle size and the space velocity were investigated on the oxygen removal efficiency and CO2 selectivity. The rise of bed temperature could promote the oxygen conversion due to the high activity of the catalyst. The O2 conversion could reach more than 95% when the temperature was above 450°C. The smaller particle size was beneficial to the CO2 selectivity of the catalyst because of the decrease in inner diffusion resistance. The lower space velocity also could improve the oxygen removal efficiency when the bed temperature was below 450°C although the improvement almost disappears above 450°C due to the increase catalytic combustion rate. Additionally, by adjusting the CH4/Air ratio, the catalytic deoxygenation adaptability of the fluidized bed reactor and the catalyst were evaluated for the variable oxygen content in CMM. The results indicate that the process has a perfect oxygen removal performance with the O2 concentration less than 0.2% and the CO2 selectivity more than 98% for the O2 content from 5% to 15% in the simulated CMM. |
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