Electrochemiluminescent resonance energy transfer of polymer dots for aptasensing
This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-color...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Sun, Feng [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018transfer abstract |
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| Schlagwörter: |
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| Umfang: |
7 |
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| Übergeordnetes Werk: |
Enthalten in: Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines - Costanigro, Marco ELSEVIER, 2019, the principal international journal devoted to research, design development and application of biosensors and bioelectronics, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:100 ; year:2018 ; day:15 ; month:02 ; pages:28-34 ; extent:7 |
| Links: |
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| DOI / URN: |
10.1016/j.bios.2017.08.047 |
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ELV04082537X |
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| 245 | 1 | 0 | |a Electrochemiluminescent resonance energy transfer of polymer dots for aptasensing |
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| 520 | |a This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. | ||
| 520 | |a This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. | ||
| 650 | 7 | |a Lead cation |2 Elsevier | |
| 650 | 7 | |a Signal switch |2 Elsevier | |
| 650 | 7 | |a Aggregation-induced emission |2 Elsevier | |
| 650 | 7 | |a Electrochemiluminescence |2 Elsevier | |
| 650 | 7 | |a Polymer dots |2 Elsevier | |
| 650 | 7 | |a Aptasensor |2 Elsevier | |
| 700 | 1 | |a Wang, Ziyu |4 oth | |
| 700 | 1 | |a Feng, Yaqiang |4 oth | |
| 700 | 1 | |a Cheng, Yixiang |4 oth | |
| 700 | 1 | |a Ju, Huangxian |4 oth | |
| 700 | 1 | |a Quan, Yiwu |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a Costanigro, Marco ELSEVIER |t Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines |d 2019 |d the principal international journal devoted to research, design development and application of biosensors and bioelectronics |g Amsterdam [u.a.] |w (DE-627)ELV001931067 |
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10.1016/j.bios.2017.08.047 doi GBV00000000000361.pica (DE-627)ELV04082537X (ELSEVIER)S0956-5663(17)30583-3 DE-627 ger DE-627 rakwb eng 630 640 VZ 49.00 bkl Sun, Feng verfasserin aut Electrochemiluminescent resonance energy transfer of polymer dots for aptasensing 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. Lead cation Elsevier Signal switch Elsevier Aggregation-induced emission Elsevier Electrochemiluminescence Elsevier Polymer dots Elsevier Aptasensor Elsevier Wang, Ziyu oth Feng, Yaqiang oth Cheng, Yixiang oth Ju, Huangxian oth Quan, Yiwu oth Enthalten in Elsevier Science Costanigro, Marco ELSEVIER Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines 2019 the principal international journal devoted to research, design development and application of biosensors and bioelectronics Amsterdam [u.a.] (DE-627)ELV001931067 volume:100 year:2018 day:15 month:02 pages:28-34 extent:7 https://doi.org/10.1016/j.bios.2017.08.047 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 49.00 Hauswirtschaft: Allgemeines VZ AR 100 2018 15 0215 28-34 7 |
| spelling |
10.1016/j.bios.2017.08.047 doi GBV00000000000361.pica (DE-627)ELV04082537X (ELSEVIER)S0956-5663(17)30583-3 DE-627 ger DE-627 rakwb eng 630 640 VZ 49.00 bkl Sun, Feng verfasserin aut Electrochemiluminescent resonance energy transfer of polymer dots for aptasensing 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. Lead cation Elsevier Signal switch Elsevier Aggregation-induced emission Elsevier Electrochemiluminescence Elsevier Polymer dots Elsevier Aptasensor Elsevier Wang, Ziyu oth Feng, Yaqiang oth Cheng, Yixiang oth Ju, Huangxian oth Quan, Yiwu oth Enthalten in Elsevier Science Costanigro, Marco ELSEVIER Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines 2019 the principal international journal devoted to research, design development and application of biosensors and bioelectronics Amsterdam [u.a.] (DE-627)ELV001931067 volume:100 year:2018 day:15 month:02 pages:28-34 extent:7 https://doi.org/10.1016/j.bios.2017.08.047 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 49.00 Hauswirtschaft: Allgemeines VZ AR 100 2018 15 0215 28-34 7 |
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10.1016/j.bios.2017.08.047 doi GBV00000000000361.pica (DE-627)ELV04082537X (ELSEVIER)S0956-5663(17)30583-3 DE-627 ger DE-627 rakwb eng 630 640 VZ 49.00 bkl Sun, Feng verfasserin aut Electrochemiluminescent resonance energy transfer of polymer dots for aptasensing 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. Lead cation Elsevier Signal switch Elsevier Aggregation-induced emission Elsevier Electrochemiluminescence Elsevier Polymer dots Elsevier Aptasensor Elsevier Wang, Ziyu oth Feng, Yaqiang oth Cheng, Yixiang oth Ju, Huangxian oth Quan, Yiwu oth Enthalten in Elsevier Science Costanigro, Marco ELSEVIER Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines 2019 the principal international journal devoted to research, design development and application of biosensors and bioelectronics Amsterdam [u.a.] (DE-627)ELV001931067 volume:100 year:2018 day:15 month:02 pages:28-34 extent:7 https://doi.org/10.1016/j.bios.2017.08.047 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 49.00 Hauswirtschaft: Allgemeines VZ AR 100 2018 15 0215 28-34 7 |
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10.1016/j.bios.2017.08.047 doi GBV00000000000361.pica (DE-627)ELV04082537X (ELSEVIER)S0956-5663(17)30583-3 DE-627 ger DE-627 rakwb eng 630 640 VZ 49.00 bkl Sun, Feng verfasserin aut Electrochemiluminescent resonance energy transfer of polymer dots for aptasensing 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. Lead cation Elsevier Signal switch Elsevier Aggregation-induced emission Elsevier Electrochemiluminescence Elsevier Polymer dots Elsevier Aptasensor Elsevier Wang, Ziyu oth Feng, Yaqiang oth Cheng, Yixiang oth Ju, Huangxian oth Quan, Yiwu oth Enthalten in Elsevier Science Costanigro, Marco ELSEVIER Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines 2019 the principal international journal devoted to research, design development and application of biosensors and bioelectronics Amsterdam [u.a.] (DE-627)ELV001931067 volume:100 year:2018 day:15 month:02 pages:28-34 extent:7 https://doi.org/10.1016/j.bios.2017.08.047 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 49.00 Hauswirtschaft: Allgemeines VZ AR 100 2018 15 0215 28-34 7 |
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10.1016/j.bios.2017.08.047 doi GBV00000000000361.pica (DE-627)ELV04082537X (ELSEVIER)S0956-5663(17)30583-3 DE-627 ger DE-627 rakwb eng 630 640 VZ 49.00 bkl Sun, Feng verfasserin aut Electrochemiluminescent resonance energy transfer of polymer dots for aptasensing 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. Lead cation Elsevier Signal switch Elsevier Aggregation-induced emission Elsevier Electrochemiluminescence Elsevier Polymer dots Elsevier Aptasensor Elsevier Wang, Ziyu oth Feng, Yaqiang oth Cheng, Yixiang oth Ju, Huangxian oth Quan, Yiwu oth Enthalten in Elsevier Science Costanigro, Marco ELSEVIER Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines 2019 the principal international journal devoted to research, design development and application of biosensors and bioelectronics Amsterdam [u.a.] (DE-627)ELV001931067 volume:100 year:2018 day:15 month:02 pages:28-34 extent:7 https://doi.org/10.1016/j.bios.2017.08.047 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 49.00 Hauswirtschaft: Allgemeines VZ AR 100 2018 15 0215 28-34 7 |
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Enthalten in Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines Amsterdam [u.a.] volume:100 year:2018 day:15 month:02 pages:28-34 extent:7 |
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Vertical differentiation via multi-tier geographical indications and the consumer perception of quality: The case of Chianti wines |
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Electrochemiluminescent resonance energy transfer of polymer dots for aptasensing |
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This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. |
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This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. |
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This work designed a three-component polymer for the preparation of polymer dots (Pdots). The polymer contained 9-(diphenylmethylene)-9H-fluorene (DPF), 9,9-dioctyl-9H-fluorene (DOF) and 1,1′-binaphthyl moieties, and was synthesized via Pd-catalyzed Suzuki reaction. It exhibited obvious yellow-colored aggregation-induced emission (AIE) for fluorescence enhancement at 543nm via an intramolecular fluorescence resonance energy transfer from DOF moiety to DPF moiety. The Pdots prepared by nanoprecipitation could be conveniently cast on electrode surface and showed a stable anodic electrochemiluminescence (ECL) emission in the presence of triethylamine as a co-reactant. The ECL emission could be effectively quenched by rhodamine B via resonance energy transfer, which led to an “off-on” switch for the design of ECL sensing methodology. Using Pb2+ as a target model, an ECL aptasensor for the detection of trace Pb2+ was proposed, which showed a linear range of 100pM to 1.0μM with a detection limit down to 38.0pM This work demonstrated the first Pdots prepared with AIE-active polymer for highly efficient ECL sensing. |
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