Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer
Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar...
Ausführliche Beschreibung
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Sun, Ziqi [verfasserIn] |
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Englisch |
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2018transfer abstract |
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8 |
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Enthalten in: Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands - saleh, Dalia I ELSEVIER, 2022, physics, materials and applications, Amsterdam [u.a.] |
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Übergeordnetes Werk: |
volume:52 ; year:2018 ; pages:309-316 ; extent:8 |
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DOI / URN: |
10.1016/j.orgel.2017.11.013 |
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ELV041251342 |
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245 | 1 | 9 | |a Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer |
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520 | |a Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. | ||
520 | |a Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. | ||
650 | 7 | |a Hole transport layer |2 Elsevier | |
650 | 7 | |a Light-harvesting |2 Elsevier | |
650 | 7 | |a Perovskite solar cells |2 Elsevier | |
650 | 7 | |a AuAg@AuAg |2 Elsevier | |
650 | 7 | |a Charge transport |2 Elsevier | |
650 | 7 | |a Core-shell alloy nanocrystals |2 Elsevier | |
700 | 1 | |a Xiahou, Yujiao |4 oth | |
700 | 1 | |a Cao, Tiantian |4 oth | |
700 | 1 | |a Zhang, Kaicheng |4 oth | |
700 | 1 | |a Wang, Zhaowei |4 oth | |
700 | 1 | |a Huang, Peng |4 oth | |
700 | 1 | |a Zhu, Kai |4 oth | |
700 | 1 | |a Yuan, Ligang |4 oth | |
700 | 1 | |a Zhou, Yi |4 oth | |
700 | 1 | |a Song, Bo |4 oth | |
700 | 1 | |a Xia, Haibing |4 oth | |
700 | 1 | |a Chen, Ning |4 oth | |
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10.1016/j.orgel.2017.11.013 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV041251342 (ELSEVIER)S1566-1199(17)30545-1 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Sun, Ziqi verfasserin aut Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Hole transport layer Elsevier Light-harvesting Elsevier Perovskite solar cells Elsevier AuAg@AuAg Elsevier Charge transport Elsevier Core-shell alloy nanocrystals Elsevier Xiahou, Yujiao oth Cao, Tiantian oth Zhang, Kaicheng oth Wang, Zhaowei oth Huang, Peng oth Zhu, Kai oth Yuan, Ligang oth Zhou, Yi oth Song, Bo oth Xia, Haibing oth Chen, Ning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:52 year:2018 pages:309-316 extent:8 https://doi.org/10.1016/j.orgel.2017.11.013 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 52 2018 309-316 8 |
spelling |
10.1016/j.orgel.2017.11.013 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV041251342 (ELSEVIER)S1566-1199(17)30545-1 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Sun, Ziqi verfasserin aut Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Hole transport layer Elsevier Light-harvesting Elsevier Perovskite solar cells Elsevier AuAg@AuAg Elsevier Charge transport Elsevier Core-shell alloy nanocrystals Elsevier Xiahou, Yujiao oth Cao, Tiantian oth Zhang, Kaicheng oth Wang, Zhaowei oth Huang, Peng oth Zhu, Kai oth Yuan, Ligang oth Zhou, Yi oth Song, Bo oth Xia, Haibing oth Chen, Ning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:52 year:2018 pages:309-316 extent:8 https://doi.org/10.1016/j.orgel.2017.11.013 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 52 2018 309-316 8 |
allfields_unstemmed |
10.1016/j.orgel.2017.11.013 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV041251342 (ELSEVIER)S1566-1199(17)30545-1 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Sun, Ziqi verfasserin aut Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Hole transport layer Elsevier Light-harvesting Elsevier Perovskite solar cells Elsevier AuAg@AuAg Elsevier Charge transport Elsevier Core-shell alloy nanocrystals Elsevier Xiahou, Yujiao oth Cao, Tiantian oth Zhang, Kaicheng oth Wang, Zhaowei oth Huang, Peng oth Zhu, Kai oth Yuan, Ligang oth Zhou, Yi oth Song, Bo oth Xia, Haibing oth Chen, Ning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:52 year:2018 pages:309-316 extent:8 https://doi.org/10.1016/j.orgel.2017.11.013 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 52 2018 309-316 8 |
allfieldsGer |
10.1016/j.orgel.2017.11.013 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV041251342 (ELSEVIER)S1566-1199(17)30545-1 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Sun, Ziqi verfasserin aut Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Hole transport layer Elsevier Light-harvesting Elsevier Perovskite solar cells Elsevier AuAg@AuAg Elsevier Charge transport Elsevier Core-shell alloy nanocrystals Elsevier Xiahou, Yujiao oth Cao, Tiantian oth Zhang, Kaicheng oth Wang, Zhaowei oth Huang, Peng oth Zhu, Kai oth Yuan, Ligang oth Zhou, Yi oth Song, Bo oth Xia, Haibing oth Chen, Ning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:52 year:2018 pages:309-316 extent:8 https://doi.org/10.1016/j.orgel.2017.11.013 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 52 2018 309-316 8 |
allfieldsSound |
10.1016/j.orgel.2017.11.013 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV041251342 (ELSEVIER)S1566-1199(17)30545-1 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Sun, Ziqi verfasserin aut Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. Hole transport layer Elsevier Light-harvesting Elsevier Perovskite solar cells Elsevier AuAg@AuAg Elsevier Charge transport Elsevier Core-shell alloy nanocrystals Elsevier Xiahou, Yujiao oth Cao, Tiantian oth Zhang, Kaicheng oth Wang, Zhaowei oth Huang, Peng oth Zhu, Kai oth Yuan, Ligang oth Zhou, Yi oth Song, Bo oth Xia, Haibing oth Chen, Ning oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:52 year:2018 pages:309-316 extent:8 https://doi.org/10.1016/j.orgel.2017.11.013 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 52 2018 309-316 8 |
language |
English |
source |
Enthalten in Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands Amsterdam [u.a.] volume:52 year:2018 pages:309-316 extent:8 |
sourceStr |
Enthalten in Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands Amsterdam [u.a.] volume:52 year:2018 pages:309-316 extent:8 |
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Hole transport layer Light-harvesting Perovskite solar cells AuAg@AuAg Charge transport Core-shell alloy nanocrystals |
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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
authorswithroles_txt_mv |
Sun, Ziqi @@aut@@ Xiahou, Yujiao @@oth@@ Cao, Tiantian @@oth@@ Zhang, Kaicheng @@oth@@ Wang, Zhaowei @@oth@@ Huang, Peng @@oth@@ Zhu, Kai @@oth@@ Yuan, Ligang @@oth@@ Zhou, Yi @@oth@@ Song, Bo @@oth@@ Xia, Haibing @@oth@@ Chen, Ning @@oth@@ |
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2018-01-01T00:00:00Z |
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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
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p-i-n type perovskite solar cells by doping auagauag core-shell alloy nanocrystals into pedot:pss layer |
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Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer |
abstract |
Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. |
abstractGer |
Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. |
abstract_unstemmed |
Metal nanocrystals have shown great potential in the application of solar cell devices, which is ascribed to their enhancement in light-harvesting, due to the plasmonic effects. Herein, we applied AuAgAuAg (AuAg) core-shell alloy nanocrystals (ANCs) into PEDOT:PSS layer of the p-i-n perovskite solar cells (pero-SCs) as dopant for the first time. The devices based on AuAg ANCs doped PEDOT:PSS reached a champion power conversion efficiency of 16.76%, showing a 28% increase compared with that of the devices based on non-doped PEDOT:PSS (13.14%). Further device characterizations, including incident photon-to-current efficiency, UV–vis absorption spectra, photoluminescence and alternating current impedance spectroscopy, suggested that the significant increase of device performance could mainly attribute to better light harvesting by the scattering effect of AuAg ANCs and better charge transport of the modified PEDOT:PSS layer. This study provides a new doping material in PEDOT:PSS to enhance the light harvesting, which leads to a significant improvement on the performance of pero-SCs. |
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title_short |
Enhanced p-i-n type perovskite solar cells by doping AuAgAuAg core-shell alloy nanocrystals into PEDOT:PSS layer |
url |
https://doi.org/10.1016/j.orgel.2017.11.013 |
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Xiahou, Yujiao Cao, Tiantian Zhang, Kaicheng Wang, Zhaowei Huang, Peng Zhu, Kai Yuan, Ligang Zhou, Yi Song, Bo Xia, Haibing Chen, Ning |
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Xiahou, Yujiao Cao, Tiantian Zhang, Kaicheng Wang, Zhaowei Huang, Peng Zhu, Kai Yuan, Ligang Zhou, Yi Song, Bo Xia, Haibing Chen, Ning |
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