Performance enhancement of mesoporous TiO<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by ZnS ultrathin-interfacial modification layer
Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic laye...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Shaikh, Shoyebmohamad F. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018transfer abstract |
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| Umfang: |
10 |
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| Übergeordnetes Werk: |
Enthalten in: Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners - Jacobs, Jacquelyn A. ELSEVIER, 2017, JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics, Lausanne |
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| Übergeordnetes Werk: |
volume:738 ; year:2018 ; day:25 ; month:03 ; pages:405-414 ; extent:10 |
| Links: |
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| DOI / URN: |
10.1016/j.jallcom.2017.12.199 |
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| 520 | |a Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. | ||
| 520 | |a Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. | ||
| 650 | 7 | |a Organometal halide perovskite |2 Elsevier | |
| 650 | 7 | |a Interfacial modification |2 Elsevier | |
| 650 | 7 | |a Ultraviolet photoelectron spectroscopy |2 Elsevier | |
| 650 | 7 | |a X-ray photoelectron spectroscopy |2 Elsevier | |
| 700 | 1 | |a Kwon, Hyeok-Chan |4 oth | |
| 700 | 1 | |a Yang, Wooseok |4 oth | |
| 700 | 1 | |a Mane, Rajaram S. |4 oth | |
| 700 | 1 | |a Moon, Jooho |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Jacobs, Jacquelyn A. ELSEVIER |t Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners |d 2017 |d JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics |g Lausanne |w (DE-627)ELV001115774 |
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10.1016/j.jallcom.2017.12.199 doi GBV00000000000359.pica (DE-627)ELV04159553X (ELSEVIER)S0925-8388(17)34395-5 DE-627 ger DE-627 rakwb eng 630 VZ Shaikh, Shoyebmohamad F. verfasserin aut Performance enhancement of mesoporous TiO<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by ZnS ultrathin-interfacial modification layer 2018transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Organometal halide perovskite Elsevier Interfacial modification Elsevier Ultraviolet photoelectron spectroscopy Elsevier X-ray photoelectron spectroscopy Elsevier Kwon, Hyeok-Chan oth Yang, Wooseok oth Mane, Rajaram S. oth Moon, Jooho oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:738 year:2018 day:25 month:03 pages:405-414 extent:10 https://doi.org/10.1016/j.jallcom.2017.12.199 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 738 2018 25 0325 405-414 10 |
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10.1016/j.jallcom.2017.12.199 doi GBV00000000000359.pica (DE-627)ELV04159553X (ELSEVIER)S0925-8388(17)34395-5 DE-627 ger DE-627 rakwb eng 630 VZ Shaikh, Shoyebmohamad F. verfasserin aut Performance enhancement of mesoporous TiO<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by ZnS ultrathin-interfacial modification layer 2018transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Organometal halide perovskite Elsevier Interfacial modification Elsevier Ultraviolet photoelectron spectroscopy Elsevier X-ray photoelectron spectroscopy Elsevier Kwon, Hyeok-Chan oth Yang, Wooseok oth Mane, Rajaram S. oth Moon, Jooho oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:738 year:2018 day:25 month:03 pages:405-414 extent:10 https://doi.org/10.1016/j.jallcom.2017.12.199 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 738 2018 25 0325 405-414 10 |
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10.1016/j.jallcom.2017.12.199 doi GBV00000000000359.pica (DE-627)ELV04159553X (ELSEVIER)S0925-8388(17)34395-5 DE-627 ger DE-627 rakwb eng 630 VZ Shaikh, Shoyebmohamad F. verfasserin aut Performance enhancement of mesoporous TiO<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by ZnS ultrathin-interfacial modification layer 2018transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Organometal halide perovskite Elsevier Interfacial modification Elsevier Ultraviolet photoelectron spectroscopy Elsevier X-ray photoelectron spectroscopy Elsevier Kwon, Hyeok-Chan oth Yang, Wooseok oth Mane, Rajaram S. oth Moon, Jooho oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:738 year:2018 day:25 month:03 pages:405-414 extent:10 https://doi.org/10.1016/j.jallcom.2017.12.199 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 738 2018 25 0325 405-414 10 |
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10.1016/j.jallcom.2017.12.199 doi GBV00000000000359.pica (DE-627)ELV04159553X (ELSEVIER)S0925-8388(17)34395-5 DE-627 ger DE-627 rakwb eng 630 VZ Shaikh, Shoyebmohamad F. verfasserin aut Performance enhancement of mesoporous TiO<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by ZnS ultrathin-interfacial modification layer 2018transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Organometal halide perovskite Elsevier Interfacial modification Elsevier Ultraviolet photoelectron spectroscopy Elsevier X-ray photoelectron spectroscopy Elsevier Kwon, Hyeok-Chan oth Yang, Wooseok oth Mane, Rajaram S. oth Moon, Jooho oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:738 year:2018 day:25 month:03 pages:405-414 extent:10 https://doi.org/10.1016/j.jallcom.2017.12.199 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 738 2018 25 0325 405-414 10 |
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10.1016/j.jallcom.2017.12.199 doi GBV00000000000359.pica (DE-627)ELV04159553X (ELSEVIER)S0925-8388(17)34395-5 DE-627 ger DE-627 rakwb eng 630 VZ Shaikh, Shoyebmohamad F. verfasserin aut Performance enhancement of mesoporous TiO<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by ZnS ultrathin-interfacial modification layer 2018transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. Organometal halide perovskite Elsevier Interfacial modification Elsevier Ultraviolet photoelectron spectroscopy Elsevier X-ray photoelectron spectroscopy Elsevier Kwon, Hyeok-Chan oth Yang, Wooseok oth Mane, Rajaram S. oth Moon, Jooho oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:738 year:2018 day:25 month:03 pages:405-414 extent:10 https://doi.org/10.1016/j.jallcom.2017.12.199 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 738 2018 25 0325 405-414 10 |
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Enthalten in Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners Lausanne volume:738 year:2018 day:25 month:03 pages:405-414 extent:10 |
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Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. 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Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners |
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performance enhancement of mesoporous tio<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by zns ultrathin-interfacial modification layer |
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Performance enhancement of mesoporous TiO<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by ZnS ultrathin-interfacial modification layer |
| abstract |
Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. |
| abstractGer |
Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. |
| abstract_unstemmed |
Interfacial modification (IM) plays a vital role in boosting the performance of perovskite solar cells. Herein, we demonstrate a new strategy in which zinc sulfide (ZnS) is used as an interfacial modifier between mesoporous-TiO2 (mp-TiO2) and a CH3NH3PbI3 absorber layer via the successive ionic layer adsorption and reaction method. The layer thickness of ZnS was optimized, and its effects on the conduction band position, interfacial charge recombination, and photovoltaic performance were investigated. Our results revealed that an ultrathin ZnS layer on mp-TiO2 helps in suppressing backflow of electrons, effectively reducing interfacial charge recombination and facilitating electron transfer. Our best performing perovskite solar cell device using the mp-TiO2-ZnS achieved a power conversion efficiency of 14.9%, with an open-circuit voltage of 1.02 V, short-circuit current density of 19.05 mA cm−2, and fill factor of 75.43%. Our simple ZnS IM approach proves that interface engineering could be a key strategy in improving the performance of perovskite solar cells. |
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Performance enhancement of mesoporous TiO<ce:inf loc="post">2</ce:inf>-based perovskite solar cells by ZnS ultrathin-interfacial modification layer |
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