Dendrite-free Li metal anode enabled by a 3D free-standing lithiophilic nitrogen-enriched carbon sponge
Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Hou, Guangmei [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018transfer abstract |
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| Umfang: |
8 |
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| Übergeordnetes Werk: |
Enthalten in: Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method - Xiao, Hong ELSEVIER, 2013, the international journal on the science and technology of electrochemical energy systems, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:386 ; year:2018 ; day:15 ; month:05 ; pages:77-84 ; extent:8 |
| Links: |
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| DOI / URN: |
10.1016/j.jpowsour.2018.03.049 |
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ELV042578574 |
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| 245 | 1 | 0 | |a Dendrite-free Li metal anode enabled by a 3D free-standing lithiophilic nitrogen-enriched carbon sponge |
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| 520 | |a Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. | ||
| 520 | |a Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. | ||
| 650 | 7 | |a Li dendrites |2 Elsevier | |
| 650 | 7 | |a Free-standing |2 Elsevier | |
| 650 | 7 | |a Lithiophilic matrix |2 Elsevier | |
| 650 | 7 | |a Battery |2 Elsevier | |
| 650 | 7 | |a Li metal anode |2 Elsevier | |
| 700 | 1 | |a Ren, Xiaohua |4 oth | |
| 700 | 1 | |a Ma, Xiaoxin |4 oth | |
| 700 | 1 | |a Zhang, Le |4 oth | |
| 700 | 1 | |a Zhai, Wei |4 oth | |
| 700 | 1 | |a Ai, Qing |4 oth | |
| 700 | 1 | |a Xu, Xiaoyan |4 oth | |
| 700 | 1 | |a Zhang, Lin |4 oth | |
| 700 | 1 | |a Si, Pengchao |4 oth | |
| 700 | 1 | |a Feng, Jinkui |4 oth | |
| 700 | 1 | |a Ding, Fei |4 oth | |
| 700 | 1 | |a Ci, Lijie |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Xiao, Hong ELSEVIER |t Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |d 2013 |d the international journal on the science and technology of electrochemical energy systems |g New York, NY [u.a.] |w (DE-627)ELV00098745X |
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10.1016/j.jpowsour.2018.03.049 doi GBV00000000000189A.pica (DE-627)ELV042578574 (ELSEVIER)S0378-7753(18)30283-0 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hou, Guangmei verfasserin aut Dendrite-free Li metal anode enabled by a 3D free-standing lithiophilic nitrogen-enriched carbon sponge 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Li dendrites Elsevier Free-standing Elsevier Lithiophilic matrix Elsevier Battery Elsevier Li metal anode Elsevier Ren, Xiaohua oth Ma, Xiaoxin oth Zhang, Le oth Zhai, Wei oth Ai, Qing oth Xu, Xiaoyan oth Zhang, Lin oth Si, Pengchao oth Feng, Jinkui oth Ding, Fei oth Ci, Lijie oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:386 year:2018 day:15 month:05 pages:77-84 extent:8 https://doi.org/10.1016/j.jpowsour.2018.03.049 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 386 2018 15 0515 77-84 8 045F 620 |
| spelling |
10.1016/j.jpowsour.2018.03.049 doi GBV00000000000189A.pica (DE-627)ELV042578574 (ELSEVIER)S0378-7753(18)30283-0 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hou, Guangmei verfasserin aut Dendrite-free Li metal anode enabled by a 3D free-standing lithiophilic nitrogen-enriched carbon sponge 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Li dendrites Elsevier Free-standing Elsevier Lithiophilic matrix Elsevier Battery Elsevier Li metal anode Elsevier Ren, Xiaohua oth Ma, Xiaoxin oth Zhang, Le oth Zhai, Wei oth Ai, Qing oth Xu, Xiaoyan oth Zhang, Lin oth Si, Pengchao oth Feng, Jinkui oth Ding, Fei oth Ci, Lijie oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:386 year:2018 day:15 month:05 pages:77-84 extent:8 https://doi.org/10.1016/j.jpowsour.2018.03.049 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 386 2018 15 0515 77-84 8 045F 620 |
| allfields_unstemmed |
10.1016/j.jpowsour.2018.03.049 doi GBV00000000000189A.pica (DE-627)ELV042578574 (ELSEVIER)S0378-7753(18)30283-0 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hou, Guangmei verfasserin aut Dendrite-free Li metal anode enabled by a 3D free-standing lithiophilic nitrogen-enriched carbon sponge 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Li dendrites Elsevier Free-standing Elsevier Lithiophilic matrix Elsevier Battery Elsevier Li metal anode Elsevier Ren, Xiaohua oth Ma, Xiaoxin oth Zhang, Le oth Zhai, Wei oth Ai, Qing oth Xu, Xiaoyan oth Zhang, Lin oth Si, Pengchao oth Feng, Jinkui oth Ding, Fei oth Ci, Lijie oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:386 year:2018 day:15 month:05 pages:77-84 extent:8 https://doi.org/10.1016/j.jpowsour.2018.03.049 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 386 2018 15 0515 77-84 8 045F 620 |
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10.1016/j.jpowsour.2018.03.049 doi GBV00000000000189A.pica (DE-627)ELV042578574 (ELSEVIER)S0378-7753(18)30283-0 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hou, Guangmei verfasserin aut Dendrite-free Li metal anode enabled by a 3D free-standing lithiophilic nitrogen-enriched carbon sponge 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Li dendrites Elsevier Free-standing Elsevier Lithiophilic matrix Elsevier Battery Elsevier Li metal anode Elsevier Ren, Xiaohua oth Ma, Xiaoxin oth Zhang, Le oth Zhai, Wei oth Ai, Qing oth Xu, Xiaoyan oth Zhang, Lin oth Si, Pengchao oth Feng, Jinkui oth Ding, Fei oth Ci, Lijie oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:386 year:2018 day:15 month:05 pages:77-84 extent:8 https://doi.org/10.1016/j.jpowsour.2018.03.049 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 386 2018 15 0515 77-84 8 045F 620 |
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10.1016/j.jpowsour.2018.03.049 doi GBV00000000000189A.pica (DE-627)ELV042578574 (ELSEVIER)S0378-7753(18)30283-0 DE-627 ger DE-627 rakwb eng 620 620 DE-600 690 VZ 50.92 bkl Hou, Guangmei verfasserin aut Dendrite-free Li metal anode enabled by a 3D free-standing lithiophilic nitrogen-enriched carbon sponge 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. Li dendrites Elsevier Free-standing Elsevier Lithiophilic matrix Elsevier Battery Elsevier Li metal anode Elsevier Ren, Xiaohua oth Ma, Xiaoxin oth Zhang, Le oth Zhai, Wei oth Ai, Qing oth Xu, Xiaoyan oth Zhang, Lin oth Si, Pengchao oth Feng, Jinkui oth Ding, Fei oth Ci, Lijie oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:386 year:2018 day:15 month:05 pages:77-84 extent:8 https://doi.org/10.1016/j.jpowsour.2018.03.049 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 386 2018 15 0515 77-84 8 045F 620 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:386 year:2018 day:15 month:05 pages:77-84 extent:8 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:386 year:2018 day:15 month:05 pages:77-84 extent:8 |
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Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |
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Hou, Guangmei @@aut@@ Ren, Xiaohua @@oth@@ Ma, Xiaoxin @@oth@@ Zhang, Le @@oth@@ Zhai, Wei @@oth@@ Ai, Qing @@oth@@ Xu, Xiaoyan @@oth@@ Zhang, Lin @@oth@@ Si, Pengchao @@oth@@ Feng, Jinkui @@oth@@ Ding, Fei @@oth@@ Ci, Lijie @@oth@@ |
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However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. 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Dendrite-free Li metal anode enabled by a 3D free-standing lithiophilic nitrogen-enriched carbon sponge |
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Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. |
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Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. |
| abstract_unstemmed |
Lithium metal is considered as the ultimate anode material for high-energy Li battery systems. However, the commercial application of lithium anode is impeded by issues with safety and low coulombic efficiency induced by Li dendrite growth. Herein, a free-standing three-dimensional nitrogen-enriched graphitic carbon sponge with a high nitrogen content is proposed as a multifunctional current collect for Lithium accommodation. The abundant lithiophilic N-containing functional groups are served as preferred nucleation sites to guide a uniform Li deposition. In addition, the nitrogen-enriched graphitic carbon sponge with a high specific surface area can effectively reduce the local current density. As a result of the synergistic effect, the nitrogen-enriched graphitic carbon sponge electrode realizes a long-term stable cycling without dendrites formation. Notably, the as-obtained composite electrode can deliver an ultra-high specific capacity of ∼3175 mA h g−1. The nitrogen-enriched graphitic carbon sponge might provide innovative insights to design a superior matrix for dendrite-free Li anode. |
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Ren, Xiaohua Ma, Xiaoxin Zhang, Le Zhai, Wei Ai, Qing Xu, Xiaoyan Zhang, Lin Si, Pengchao Feng, Jinkui Ding, Fei Ci, Lijie |
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Ren, Xiaohua Ma, Xiaoxin Zhang, Le Zhai, Wei Ai, Qing Xu, Xiaoyan Zhang, Lin Si, Pengchao Feng, Jinkui Ding, Fei Ci, Lijie |
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