Photoelectrochemical water splitting with tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod in photoelectrochemical cell
Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure na...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Bashiri, Robabeh [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018transfer abstract |
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| Umfang: |
8 |
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| Übergeordnetes Werk: |
Enthalten in: Sodium atom beam collisions with the liquid glycerol surface: Mass effects of deuteration - Wiens, Justin P. ELSEVIER, 2019, advancing the science and technology of diamond, diamond-like carbon, silicon carbides and Group 3 nitride materials, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:85 ; year:2018 ; pages:5-12 ; extent:8 |
| Links: |
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| DOI / URN: |
10.1016/j.diamond.2018.03.019 |
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ELV042988543 |
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| 520 | |a Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. | ||
| 520 | |a Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. | ||
| 700 | 1 | |a Mohamed, Norani Muti |4 oth | |
| 700 | 1 | |a Suhaimi, Nur Amirah |4 oth | |
| 700 | 1 | |a Shahid, Muhammad Umair |4 oth | |
| 700 | 1 | |a Kait, Chong Fai |4 oth | |
| 700 | 1 | |a Sufian, Suriati |4 oth | |
| 700 | 1 | |a Khatani, Mehboob |4 oth | |
| 700 | 1 | |a Mumtaz, Asad |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a Wiens, Justin P. ELSEVIER |t Sodium atom beam collisions with the liquid glycerol surface: Mass effects of deuteration |d 2019 |d advancing the science and technology of diamond, diamond-like carbon, silicon carbides and Group 3 nitride materials |g Amsterdam [u.a.] |w (DE-627)ELV002660938 |
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10.1016/j.diamond.2018.03.019 doi GBV00000000000226A.pica (DE-627)ELV042988543 (ELSEVIER)S0925-9635(17)30604-0 DE-627 ger DE-627 rakwb eng 550 670 550 DE-600 670 DE-600 540 VZ 35.10 bkl Bashiri, Robabeh verfasserin aut Photoelectrochemical water splitting with tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod in photoelectrochemical cell 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Mohamed, Norani Muti oth Suhaimi, Nur Amirah oth Shahid, Muhammad Umair oth Kait, Chong Fai oth Sufian, Suriati oth Khatani, Mehboob oth Mumtaz, Asad oth Enthalten in Elsevier Science Wiens, Justin P. ELSEVIER Sodium atom beam collisions with the liquid glycerol surface: Mass effects of deuteration 2019 advancing the science and technology of diamond, diamond-like carbon, silicon carbides and Group 3 nitride materials Amsterdam [u.a.] (DE-627)ELV002660938 volume:85 year:2018 pages:5-12 extent:8 https://doi.org/10.1016/j.diamond.2018.03.019 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.10 Physikalische Chemie: Allgemeines VZ AR 85 2018 5-12 8 045F 550 |
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10.1016/j.diamond.2018.03.019 doi GBV00000000000226A.pica (DE-627)ELV042988543 (ELSEVIER)S0925-9635(17)30604-0 DE-627 ger DE-627 rakwb eng 550 670 550 DE-600 670 DE-600 540 VZ 35.10 bkl Bashiri, Robabeh verfasserin aut Photoelectrochemical water splitting with tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod in photoelectrochemical cell 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Mohamed, Norani Muti oth Suhaimi, Nur Amirah oth Shahid, Muhammad Umair oth Kait, Chong Fai oth Sufian, Suriati oth Khatani, Mehboob oth Mumtaz, Asad oth Enthalten in Elsevier Science Wiens, Justin P. ELSEVIER Sodium atom beam collisions with the liquid glycerol surface: Mass effects of deuteration 2019 advancing the science and technology of diamond, diamond-like carbon, silicon carbides and Group 3 nitride materials Amsterdam [u.a.] (DE-627)ELV002660938 volume:85 year:2018 pages:5-12 extent:8 https://doi.org/10.1016/j.diamond.2018.03.019 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.10 Physikalische Chemie: Allgemeines VZ AR 85 2018 5-12 8 045F 550 |
| allfields_unstemmed |
10.1016/j.diamond.2018.03.019 doi GBV00000000000226A.pica (DE-627)ELV042988543 (ELSEVIER)S0925-9635(17)30604-0 DE-627 ger DE-627 rakwb eng 550 670 550 DE-600 670 DE-600 540 VZ 35.10 bkl Bashiri, Robabeh verfasserin aut Photoelectrochemical water splitting with tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod in photoelectrochemical cell 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Mohamed, Norani Muti oth Suhaimi, Nur Amirah oth Shahid, Muhammad Umair oth Kait, Chong Fai oth Sufian, Suriati oth Khatani, Mehboob oth Mumtaz, Asad oth Enthalten in Elsevier Science Wiens, Justin P. ELSEVIER Sodium atom beam collisions with the liquid glycerol surface: Mass effects of deuteration 2019 advancing the science and technology of diamond, diamond-like carbon, silicon carbides and Group 3 nitride materials Amsterdam [u.a.] (DE-627)ELV002660938 volume:85 year:2018 pages:5-12 extent:8 https://doi.org/10.1016/j.diamond.2018.03.019 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.10 Physikalische Chemie: Allgemeines VZ AR 85 2018 5-12 8 045F 550 |
| allfieldsGer |
10.1016/j.diamond.2018.03.019 doi GBV00000000000226A.pica (DE-627)ELV042988543 (ELSEVIER)S0925-9635(17)30604-0 DE-627 ger DE-627 rakwb eng 550 670 550 DE-600 670 DE-600 540 VZ 35.10 bkl Bashiri, Robabeh verfasserin aut Photoelectrochemical water splitting with tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod in photoelectrochemical cell 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Mohamed, Norani Muti oth Suhaimi, Nur Amirah oth Shahid, Muhammad Umair oth Kait, Chong Fai oth Sufian, Suriati oth Khatani, Mehboob oth Mumtaz, Asad oth Enthalten in Elsevier Science Wiens, Justin P. ELSEVIER Sodium atom beam collisions with the liquid glycerol surface: Mass effects of deuteration 2019 advancing the science and technology of diamond, diamond-like carbon, silicon carbides and Group 3 nitride materials Amsterdam [u.a.] (DE-627)ELV002660938 volume:85 year:2018 pages:5-12 extent:8 https://doi.org/10.1016/j.diamond.2018.03.019 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.10 Physikalische Chemie: Allgemeines VZ AR 85 2018 5-12 8 045F 550 |
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10.1016/j.diamond.2018.03.019 doi GBV00000000000226A.pica (DE-627)ELV042988543 (ELSEVIER)S0925-9635(17)30604-0 DE-627 ger DE-627 rakwb eng 550 670 550 DE-600 670 DE-600 540 VZ 35.10 bkl Bashiri, Robabeh verfasserin aut Photoelectrochemical water splitting with tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod in photoelectrochemical cell 2018transfer abstract 8 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. Mohamed, Norani Muti oth Suhaimi, Nur Amirah oth Shahid, Muhammad Umair oth Kait, Chong Fai oth Sufian, Suriati oth Khatani, Mehboob oth Mumtaz, Asad oth Enthalten in Elsevier Science Wiens, Justin P. ELSEVIER Sodium atom beam collisions with the liquid glycerol surface: Mass effects of deuteration 2019 advancing the science and technology of diamond, diamond-like carbon, silicon carbides and Group 3 nitride materials Amsterdam [u.a.] (DE-627)ELV002660938 volume:85 year:2018 pages:5-12 extent:8 https://doi.org/10.1016/j.diamond.2018.03.019 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.10 Physikalische Chemie: Allgemeines VZ AR 85 2018 5-12 8 045F 550 |
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Photoelectrochemical water splitting with tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod in photoelectrochemical cell |
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Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. |
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Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. |
| abstract_unstemmed |
Solar hydrogen production through water photosplitting in photoelectrochemical (PEC) cell is one of the most desirable, cost-effective and environmentally friendly processes. However, it is still suffering from the low photoconversion efficiency. A novel tailored TiO2/SrTiO3g-C3N4 heterostructure nanorod was synthesized to investigate the photocatalytic hydrogen production under visible light condition in glycerol-based PEC cell. A series of TiO2 and TiO2/SrTiO3 nanorod were grown on F-doped SnO2 glass (FTO) substrate by hydrothermal method and then were modified using graphitic carbon nitride g-C3N4 via the chemical bath deposition technique. The samples were characterized using X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), high-resolution transmission electron microscopy (HRTEM), diffuse reflectance UV–Vis spectroscopy (DR-UV–Vis), and Fourier transform infrared (FTIR) to explore the physicochemical properties of the prepared photocatalysts. The prepared TiO2/SrTiO3@g-C3N4 served as the efficient photoanode with maximum produced hydrogen of 73 μmol/cm2 compared to others. This photocatalyst had more uniformed structures and shifted more absorbance to the visible region as presented in FESEM and DR-UV–Vis. Therefore, high performance of this photocatalyst can be ascribed to the close interfacial connections between g-C3N4 and TiO2/SrTiO3 where the photo-generated electron and holes were effectively separated. |
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