Mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices
Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are inves...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Han, Pengxian [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018transfer abstract |
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| Schlagwörter: |
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| Umfang: |
7 |
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| Übergeordnetes Werk: |
Enthalten in: Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method - Xiao, Hong ELSEVIER, 2013, the international journal on the science and technology of electrochemical energy systems, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:393 ; year:2018 ; day:31 ; month:07 ; pages:145-151 ; extent:7 |
| Links: |
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| DOI / URN: |
10.1016/j.jpowsour.2018.05.021 |
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| 520 | |a Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. | ||
| 520 | |a Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. | ||
| 650 | 7 | |a Lithium ion battery |2 Elsevier | |
| 650 | 7 | |a Mesocarbon microbead |2 Elsevier | |
| 650 | 7 | |a Pre-lithiation |2 Elsevier | |
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| 700 | 1 | |a Yue, Liping |4 oth | |
| 700 | 1 | |a Zhao, Jingwen |4 oth | |
| 700 | 1 | |a Zhou, Xinhong |4 oth | |
| 700 | 1 | |a Cui, Guanglei |4 oth | |
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10.1016/j.jpowsour.2018.05.021 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001222.pica (DE-627)ELV043495532 (ELSEVIER)S0378-7753(18)30482-8 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Han, Pengxian verfasserin aut Mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Lithium ion battery Elsevier Mesocarbon microbead Elsevier Pre-lithiation Elsevier Dual-carbon Elsevier Han, Xiaoqi oth Yao, Jianhua oth Yue, Liping oth Zhao, Jingwen oth Zhou, Xinhong oth Cui, Guanglei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:393 year:2018 day:31 month:07 pages:145-151 extent:7 https://doi.org/10.1016/j.jpowsour.2018.05.021 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 393 2018 31 0731 145-151 7 |
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10.1016/j.jpowsour.2018.05.021 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001222.pica (DE-627)ELV043495532 (ELSEVIER)S0378-7753(18)30482-8 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Han, Pengxian verfasserin aut Mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Lithium ion battery Elsevier Mesocarbon microbead Elsevier Pre-lithiation Elsevier Dual-carbon Elsevier Han, Xiaoqi oth Yao, Jianhua oth Yue, Liping oth Zhao, Jingwen oth Zhou, Xinhong oth Cui, Guanglei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:393 year:2018 day:31 month:07 pages:145-151 extent:7 https://doi.org/10.1016/j.jpowsour.2018.05.021 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 393 2018 31 0731 145-151 7 |
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10.1016/j.jpowsour.2018.05.021 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001222.pica (DE-627)ELV043495532 (ELSEVIER)S0378-7753(18)30482-8 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Han, Pengxian verfasserin aut Mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Lithium ion battery Elsevier Mesocarbon microbead Elsevier Pre-lithiation Elsevier Dual-carbon Elsevier Han, Xiaoqi oth Yao, Jianhua oth Yue, Liping oth Zhao, Jingwen oth Zhou, Xinhong oth Cui, Guanglei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:393 year:2018 day:31 month:07 pages:145-151 extent:7 https://doi.org/10.1016/j.jpowsour.2018.05.021 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 393 2018 31 0731 145-151 7 |
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10.1016/j.jpowsour.2018.05.021 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001222.pica (DE-627)ELV043495532 (ELSEVIER)S0378-7753(18)30482-8 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Han, Pengxian verfasserin aut Mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Lithium ion battery Elsevier Mesocarbon microbead Elsevier Pre-lithiation Elsevier Dual-carbon Elsevier Han, Xiaoqi oth Yao, Jianhua oth Yue, Liping oth Zhao, Jingwen oth Zhou, Xinhong oth Cui, Guanglei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:393 year:2018 day:31 month:07 pages:145-151 extent:7 https://doi.org/10.1016/j.jpowsour.2018.05.021 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 393 2018 31 0731 145-151 7 |
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10.1016/j.jpowsour.2018.05.021 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001222.pica (DE-627)ELV043495532 (ELSEVIER)S0378-7753(18)30482-8 DE-627 ger DE-627 rakwb eng 690 VZ 50.92 bkl Han, Pengxian verfasserin aut Mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices 2018transfer abstract 7 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. Lithium ion battery Elsevier Mesocarbon microbead Elsevier Pre-lithiation Elsevier Dual-carbon Elsevier Han, Xiaoqi oth Yao, Jianhua oth Yue, Liping oth Zhao, Jingwen oth Zhou, Xinhong oth Cui, Guanglei oth Enthalten in Elsevier Xiao, Hong ELSEVIER Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method 2013 the international journal on the science and technology of electrochemical energy systems New York, NY [u.a.] (DE-627)ELV00098745X volume:393 year:2018 day:31 month:07 pages:145-151 extent:7 https://doi.org/10.1016/j.jpowsour.2018.05.021 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.92 Meerestechnik VZ AR 393 2018 31 0731 145-151 7 |
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Enthalten in Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method New York, NY [u.a.] volume:393 year:2018 day:31 month:07 pages:145-151 extent:7 |
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Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |
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Numerical modeling of wave–current forces acting on horizontal cylinder of marine structures by VOF method |
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mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices |
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Mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices |
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Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. |
| abstractGer |
Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. |
| abstract_unstemmed |
Recently, the low cost energy devices with high energy density and high power density are becoming more and more important in the field of electric vehicles. In this work, the electrochemical intercalation/deintercalation behaviors of PF6ˉ into graphitic mesocarbon microbead (MCMB) cathode are investigated in the electrolyte of 1 M LiPF6 in the mixed solvent of ethylmethyl carbonate and sulfolane. The charge storage mechanisms related to surface-limited capacitive and diffusion-controlled intercalation capacity are also studied by cyclic voltammetry measurements, which indicates that both the intercalation reaction and the capacitive reaction contribute to the overall capacity. Furthermore, dual-carbon batteries comprising MCMB cathode and pre-lithiated MCMB anode are unprecedentedly demonstrated in the form of aluminum pouch cells with laminated structure and exhibit an encouraging energy density of 47.9 Wh kg−1 at the power density of 583.6 W kg−1 based on the overall mass of the battery. Finally, electrochemical impedance spectroscopy is used to differentiate the resistance variation of MCMB cathode and MCMB anode before and after 3000 cycles. The continuous intercalation/deintercalation of PF6ˉ into MCMB cathode lead to the exfoliation of the active material and the increase of internal resistance. |
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Mesocarbon microbead based dual-carbon batteries towards low cost energy storage devices |
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Han, Xiaoqi Yao, Jianhua Yue, Liping Zhao, Jingwen Zhou, Xinhong Cui, Guanglei |
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