Nickel phosphate as advanced promising electrochemical catalyst for the electro-oxidation of methanol
Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commer...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Song, Xueying [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018transfer abstract |
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| Umfang: |
12 |
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| Übergeordnetes Werk: |
Enthalten in: External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs - Dedhia, Kavita ELSEVIER, 2018, official journal of the International Association for Hydrogen Energy, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:43 ; year:2018 ; number:27 ; day:5 ; month:07 ; pages:12091-12102 ; extent:12 |
| Links: |
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| DOI / URN: |
10.1016/j.ijhydene.2018.04.165 |
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| 520 | |a Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. | ||
| 520 | |a Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. | ||
| 650 | 7 | |a Electrocatalysis |2 Elsevier | |
| 650 | 7 | |a Methanol oxidation |2 Elsevier | |
| 650 | 7 | |a Nickel phosphate |2 Elsevier | |
| 700 | 1 | |a Sun, Qian |4 oth | |
| 700 | 1 | |a Gao, Li |4 oth | |
| 700 | 1 | |a Chen, Wei |4 oth | |
| 700 | 1 | |a Wu, Yufeng |4 oth | |
| 700 | 1 | |a Li, Yamin |4 oth | |
| 700 | 1 | |a Mao, Liqun |4 oth | |
| 700 | 1 | |a Yang, Jing-He |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Dedhia, Kavita ELSEVIER |t External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs |d 2018 |d official journal of the International Association for Hydrogen Energy |g New York, NY [u.a.] |w (DE-627)ELV000127019 |
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10.1016/j.ijhydene.2018.04.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000886.pica (DE-627)ELV043554911 (ELSEVIER)S0360-3199(18)31354-5 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Song, Xueying verfasserin aut Nickel phosphate as advanced promising electrochemical catalyst for the electro-oxidation of methanol 2018transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Electrocatalysis Elsevier Methanol oxidation Elsevier Nickel phosphate Elsevier Sun, Qian oth Gao, Li oth Chen, Wei oth Wu, Yufeng oth Li, Yamin oth Mao, Liqun oth Yang, Jing-He oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:43 year:2018 number:27 day:5 month:07 pages:12091-12102 extent:12 https://doi.org/10.1016/j.ijhydene.2018.04.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 43 2018 27 5 0705 12091-12102 12 |
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10.1016/j.ijhydene.2018.04.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000886.pica (DE-627)ELV043554911 (ELSEVIER)S0360-3199(18)31354-5 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Song, Xueying verfasserin aut Nickel phosphate as advanced promising electrochemical catalyst for the electro-oxidation of methanol 2018transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Electrocatalysis Elsevier Methanol oxidation Elsevier Nickel phosphate Elsevier Sun, Qian oth Gao, Li oth Chen, Wei oth Wu, Yufeng oth Li, Yamin oth Mao, Liqun oth Yang, Jing-He oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:43 year:2018 number:27 day:5 month:07 pages:12091-12102 extent:12 https://doi.org/10.1016/j.ijhydene.2018.04.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 43 2018 27 5 0705 12091-12102 12 |
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10.1016/j.ijhydene.2018.04.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000886.pica (DE-627)ELV043554911 (ELSEVIER)S0360-3199(18)31354-5 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Song, Xueying verfasserin aut Nickel phosphate as advanced promising electrochemical catalyst for the electro-oxidation of methanol 2018transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Electrocatalysis Elsevier Methanol oxidation Elsevier Nickel phosphate Elsevier Sun, Qian oth Gao, Li oth Chen, Wei oth Wu, Yufeng oth Li, Yamin oth Mao, Liqun oth Yang, Jing-He oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:43 year:2018 number:27 day:5 month:07 pages:12091-12102 extent:12 https://doi.org/10.1016/j.ijhydene.2018.04.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 43 2018 27 5 0705 12091-12102 12 |
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10.1016/j.ijhydene.2018.04.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000886.pica (DE-627)ELV043554911 (ELSEVIER)S0360-3199(18)31354-5 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Song, Xueying verfasserin aut Nickel phosphate as advanced promising electrochemical catalyst for the electro-oxidation of methanol 2018transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Electrocatalysis Elsevier Methanol oxidation Elsevier Nickel phosphate Elsevier Sun, Qian oth Gao, Li oth Chen, Wei oth Wu, Yufeng oth Li, Yamin oth Mao, Liqun oth Yang, Jing-He oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:43 year:2018 number:27 day:5 month:07 pages:12091-12102 extent:12 https://doi.org/10.1016/j.ijhydene.2018.04.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 43 2018 27 5 0705 12091-12102 12 |
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10.1016/j.ijhydene.2018.04.165 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000886.pica (DE-627)ELV043554911 (ELSEVIER)S0360-3199(18)31354-5 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Song, Xueying verfasserin aut Nickel phosphate as advanced promising electrochemical catalyst for the electro-oxidation of methanol 2018transfer abstract 12 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. Electrocatalysis Elsevier Methanol oxidation Elsevier Nickel phosphate Elsevier Sun, Qian oth Gao, Li oth Chen, Wei oth Wu, Yufeng oth Li, Yamin oth Mao, Liqun oth Yang, Jing-He oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:43 year:2018 number:27 day:5 month:07 pages:12091-12102 extent:12 https://doi.org/10.1016/j.ijhydene.2018.04.165 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 43 2018 27 5 0705 12091-12102 12 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:43 year:2018 number:27 day:5 month:07 pages:12091-12102 extent:12 |
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nickel phosphate as advanced promising electrochemical catalyst for the electro-oxidation of methanol |
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Nickel phosphate as advanced promising electrochemical catalyst for the electro-oxidation of methanol |
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Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. |
| abstractGer |
Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. |
| abstract_unstemmed |
Mesoporous nickel phosphate nanotube (Meso NiPO NT) and mesoporous nickel phosphate nanosheet (Meso NiPO NS) are developed as catalysts for electrochemical methanol oxidation. Conventional mesoporous nickel phosphate which is composed of stacked nanocrystals (Meso NiPO), microporous VSB-5 and commercial nickel oxide (NiO) are used as control materials. Notably, both Meso NiPO NT (40.83 mA cm−2) and Meso NiPO NS (44.97 mA cm−2) exhibit much higher oxidation current density than VSB-5 (13.41 mA cm−2), Meso NiPO (19.85 mA cm−2) and commercial NiO (0.87 mA cm−2). As for the durability test on these materials modified fluorine-doped tin dioxide transparent conductive glass (FTO) electrodes, Meso NiPO NT displays the most stable performance and still retains 91.3% electrochemical activity, which perhaps benefit from its nanotube structure and large specific surface area (99.6 m2/g). Moreover, Meso NiPO NT has higher activity and more excellent stability than many of the previously reported nickel-based materials, suggesting a potential development for direct methanol fuel cells. |
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Sun, Qian Gao, Li Chen, Wei Wu, Yufeng Li, Yamin Mao, Liqun Yang, Jing-He |
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