Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions
Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Gao, Zhiqiang [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018transfer abstract |
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| Umfang: |
9 |
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| Übergeordnetes Werk: |
Enthalten in: Dynamic patterns of open review process - Zhao, Zhi-Dan ELSEVIER, 2021, an international journal sponsored by the American Carbon Society, Amsterdam [u.a.] |
|---|---|
| Übergeordnetes Werk: |
volume:139 ; year:2018 ; pages:369-377 ; extent:9 |
| Links: |
|---|
| DOI / URN: |
10.1016/j.carbon.2018.07.006 |
|---|
| Katalog-ID: |
ELV044293100 |
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| 245 | 1 | 0 | |a Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions |
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| 520 | |a Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. | ||
| 520 | |a Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. | ||
| 700 | 1 | |a Li, Miaomiao |4 oth | |
| 700 | 1 | |a Wang, Jiayu |4 oth | |
| 700 | 1 | |a Zhu, Jixin |4 oth | |
| 700 | 1 | |a Zhao, Xianmin |4 oth | |
| 700 | 1 | |a Huang, Huajie |4 oth | |
| 700 | 1 | |a Zhang, Jianfeng |4 oth | |
| 700 | 1 | |a Wu, Yuping |4 oth | |
| 700 | 1 | |a Fu, Yongsheng |4 oth | |
| 700 | 1 | |a Wang, Xin |4 oth | |
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10.1016/j.carbon.2018.07.006 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV044293100 (ELSEVIER)S0008-6223(18)30648-1 DE-627 ger DE-627 rakwb eng 500 VZ 33.25 bkl 31.00 bkl Gao, Zhiqiang verfasserin aut Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions 2018transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Li, Miaomiao oth Wang, Jiayu oth Zhu, Jixin oth Zhao, Xianmin oth Huang, Huajie oth Zhang, Jianfeng oth Wu, Yuping oth Fu, Yongsheng oth Wang, Xin oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:139 year:2018 pages:369-377 extent:9 https://doi.org/10.1016/j.carbon.2018.07.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 139 2018 369-377 9 |
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10.1016/j.carbon.2018.07.006 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV044293100 (ELSEVIER)S0008-6223(18)30648-1 DE-627 ger DE-627 rakwb eng 500 VZ 33.25 bkl 31.00 bkl Gao, Zhiqiang verfasserin aut Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions 2018transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Li, Miaomiao oth Wang, Jiayu oth Zhu, Jixin oth Zhao, Xianmin oth Huang, Huajie oth Zhang, Jianfeng oth Wu, Yuping oth Fu, Yongsheng oth Wang, Xin oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:139 year:2018 pages:369-377 extent:9 https://doi.org/10.1016/j.carbon.2018.07.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 139 2018 369-377 9 |
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10.1016/j.carbon.2018.07.006 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV044293100 (ELSEVIER)S0008-6223(18)30648-1 DE-627 ger DE-627 rakwb eng 500 VZ 33.25 bkl 31.00 bkl Gao, Zhiqiang verfasserin aut Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions 2018transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Li, Miaomiao oth Wang, Jiayu oth Zhu, Jixin oth Zhao, Xianmin oth Huang, Huajie oth Zhang, Jianfeng oth Wu, Yuping oth Fu, Yongsheng oth Wang, Xin oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:139 year:2018 pages:369-377 extent:9 https://doi.org/10.1016/j.carbon.2018.07.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 139 2018 369-377 9 |
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10.1016/j.carbon.2018.07.006 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV044293100 (ELSEVIER)S0008-6223(18)30648-1 DE-627 ger DE-627 rakwb eng 500 VZ 33.25 bkl 31.00 bkl Gao, Zhiqiang verfasserin aut Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions 2018transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Li, Miaomiao oth Wang, Jiayu oth Zhu, Jixin oth Zhao, Xianmin oth Huang, Huajie oth Zhang, Jianfeng oth Wu, Yuping oth Fu, Yongsheng oth Wang, Xin oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:139 year:2018 pages:369-377 extent:9 https://doi.org/10.1016/j.carbon.2018.07.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 139 2018 369-377 9 |
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10.1016/j.carbon.2018.07.006 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001218.pica (DE-627)ELV044293100 (ELSEVIER)S0008-6223(18)30648-1 DE-627 ger DE-627 rakwb eng 500 VZ 33.25 bkl 31.00 bkl Gao, Zhiqiang verfasserin aut Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions 2018transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. Li, Miaomiao oth Wang, Jiayu oth Zhu, Jixin oth Zhao, Xianmin oth Huang, Huajie oth Zhang, Jianfeng oth Wu, Yuping oth Fu, Yongsheng oth Wang, Xin oth Enthalten in Elsevier Science Zhao, Zhi-Dan ELSEVIER Dynamic patterns of open review process 2021 an international journal sponsored by the American Carbon Society Amsterdam [u.a.] (DE-627)ELV006580718 volume:139 year:2018 pages:369-377 extent:9 https://doi.org/10.1016/j.carbon.2018.07.006 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OPC-MAT 33.25 Thermodynamik statistische Physik VZ 31.00 Mathematik: Allgemeines VZ AR 139 2018 369-377 9 |
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Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions |
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Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions |
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Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. |
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Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. |
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Although electrocatalytic hydrogen evolution and methanol oxidation have long been regarded as promising technologies for future energy production and conversion, the incapability of the electrode catalysts poses a major impediment to their large-scale commercialization. Herein, we present a facile co-assembly approach to the fabrication of Pt nanocrystals grown on 3D architectures built from ultrathin graphene and MoS2 nanosheets. By virtue of their unique textural features, such as large specific surface area, 3D cross-linked porous framework, homogeneous distribution of Pt nanoparticles, and excellent electron conductivity, the resulting Pt/graphene-MoS2 architectures possess multifunctional catalytic activities toward hydrogen evolution and methanol oxidation reactions, accompanied by high durability and strong poison tolerance, which significantly outperform those for conventional Pt/carbon black, Pt/graphene, and Pt/MoS2 catalysts. It is believed that such a simple bottom-up design concept can open up new possibilities for the up-scale synthesis of various 3D hybrid architectures with metals or metal oxides for energy-related applications. |
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Pt nanocrystals grown on three-dimensional architectures made from graphene and MoS2 nanosheets: Highly efficient multifunctional electrocatalysts toward hydrogen evolution and methanol oxidation reactions |
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