Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells
Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafe...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Li, Songjun [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2018transfer abstract |
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| Umfang: |
6 |
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| Übergeordnetes Werk: |
Enthalten in: Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands - saleh, Dalia I ELSEVIER, 2022, physics, materials and applications, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:59 ; year:2018 ; pages:1-6 ; extent:6 |
| Links: |
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| DOI / URN: |
10.1016/j.orgel.2018.04.030 |
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ELV045033137 |
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| 245 | 1 | 0 | |a Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells |
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| 520 | |a Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. | ||
| 520 | |a Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. | ||
| 650 | 7 | |a PEDOT |2 Elsevier | |
| 650 | 7 | |a Stability |2 Elsevier | |
| 650 | 7 | |a Doping |2 Elsevier | |
| 650 | 7 | |a Charge recombination |2 Elsevier | |
| 650 | 7 | |a Electropolymerization |2 Elsevier | |
| 650 | 7 | |a Si/organic solar cells |2 Elsevier | |
| 700 | 1 | |a Chen, Ling |4 oth | |
| 700 | 1 | |a Zhang, Kan |4 oth | |
| 700 | 1 | |a Wu, Shuping |4 oth | |
| 700 | 1 | |a Shen, Xiaojuan |4 oth | |
| 700 | 1 | |a Zhao, Jie |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a saleh, Dalia I ELSEVIER |t Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |d 2022 |d physics, materials and applications |g Amsterdam [u.a.] |w (DE-627)ELV007843747 |
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10.1016/j.orgel.2018.04.030 doi GBV00000000000676.pica (DE-627)ELV045033137 (ELSEVIER)S1566-1199(18)30194-0 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Li, Songjun verfasserin aut Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells 2018transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. PEDOT Elsevier Stability Elsevier Doping Elsevier Charge recombination Elsevier Electropolymerization Elsevier Si/organic solar cells Elsevier Chen, Ling oth Zhang, Kan oth Wu, Shuping oth Shen, Xiaojuan oth Zhao, Jie oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:59 year:2018 pages:1-6 extent:6 https://doi.org/10.1016/j.orgel.2018.04.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 59 2018 1-6 6 |
| spelling |
10.1016/j.orgel.2018.04.030 doi GBV00000000000676.pica (DE-627)ELV045033137 (ELSEVIER)S1566-1199(18)30194-0 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Li, Songjun verfasserin aut Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells 2018transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. PEDOT Elsevier Stability Elsevier Doping Elsevier Charge recombination Elsevier Electropolymerization Elsevier Si/organic solar cells Elsevier Chen, Ling oth Zhang, Kan oth Wu, Shuping oth Shen, Xiaojuan oth Zhao, Jie oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:59 year:2018 pages:1-6 extent:6 https://doi.org/10.1016/j.orgel.2018.04.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 59 2018 1-6 6 |
| allfields_unstemmed |
10.1016/j.orgel.2018.04.030 doi GBV00000000000676.pica (DE-627)ELV045033137 (ELSEVIER)S1566-1199(18)30194-0 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Li, Songjun verfasserin aut Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells 2018transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. PEDOT Elsevier Stability Elsevier Doping Elsevier Charge recombination Elsevier Electropolymerization Elsevier Si/organic solar cells Elsevier Chen, Ling oth Zhang, Kan oth Wu, Shuping oth Shen, Xiaojuan oth Zhao, Jie oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:59 year:2018 pages:1-6 extent:6 https://doi.org/10.1016/j.orgel.2018.04.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 59 2018 1-6 6 |
| allfieldsGer |
10.1016/j.orgel.2018.04.030 doi GBV00000000000676.pica (DE-627)ELV045033137 (ELSEVIER)S1566-1199(18)30194-0 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Li, Songjun verfasserin aut Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells 2018transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. PEDOT Elsevier Stability Elsevier Doping Elsevier Charge recombination Elsevier Electropolymerization Elsevier Si/organic solar cells Elsevier Chen, Ling oth Zhang, Kan oth Wu, Shuping oth Shen, Xiaojuan oth Zhao, Jie oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:59 year:2018 pages:1-6 extent:6 https://doi.org/10.1016/j.orgel.2018.04.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 59 2018 1-6 6 |
| allfieldsSound |
10.1016/j.orgel.2018.04.030 doi GBV00000000000676.pica (DE-627)ELV045033137 (ELSEVIER)S1566-1199(18)30194-0 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Li, Songjun verfasserin aut Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells 2018transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. PEDOT Elsevier Stability Elsevier Doping Elsevier Charge recombination Elsevier Electropolymerization Elsevier Si/organic solar cells Elsevier Chen, Ling oth Zhang, Kan oth Wu, Shuping oth Shen, Xiaojuan oth Zhao, Jie oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:59 year:2018 pages:1-6 extent:6 https://doi.org/10.1016/j.orgel.2018.04.030 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 59 2018 1-6 6 |
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English |
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Enthalten in Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands Amsterdam [u.a.] volume:59 year:2018 pages:1-6 extent:6 |
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Enthalten in Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands Amsterdam [u.a.] volume:59 year:2018 pages:1-6 extent:6 |
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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
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Li, Songjun ddc 540 bkl 35.00 Elsevier PEDOT Elsevier Stability Elsevier Doping Elsevier Charge recombination Elsevier Electropolymerization Elsevier Si/organic solar cells Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells |
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doped the electropolymerized pedot for high performance and air stable si/organic solar cells |
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Doped the electropolymerized PEDOT for high performance and air stable Si/organic solar cells |
| abstract |
Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. |
| abstractGer |
Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. |
| abstract_unstemmed |
Poly(3,4-ethylenedioxythiophene) (PEDOT) has been electropolymerized on the Si wafer through a non-aqueous galvanostatic method, which is employed to fabricate the Si/organic solar cell for the first time. Surface morphology, film thickness as well as the sheet resistance of the PEDOT-coated Si wafer are investigated by controlling the polymerization time, and the best electropolymerization time for the Si/PEDOT device performance is 8 s. However, the pristine PEDOT film shows low carrier concentration, and the low work function is not suitable for the fabrication of high performance solar cells. Interestingly, after optimizing the PEDOT-coated Si wafer with hydrochloroplatinic acid (H2PtCl6) solution, the work function of the PEDOT film is enhanced, which raises the barrier height (ΦSBH) as well as Vbi between the Si and PEDOT interface. Additionally, the sheet resistance of the PEDOT layer is reduced. Both of them are beneficial for the better charge transfer and collection. As a result, the efficiency of 7.36% has been achieved by the Si/PEDOT devices, which is much higher than that of the control ones, ∼5.49%. More importantly, due to the stable PEDOT, the Si/PEDOT solar cell shows excellent stability. These results point out a new route to develop low-cost, high performance and high stability Si/organic hybrid solar cells. |
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