High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture
Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matr...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Li, Peng [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019transfer abstract |
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| Schlagwörter: |
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| Umfang: |
10 |
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| Übergeordnetes Werk: |
Enthalten in: Nonlinear relationship between monetary policy and stock returns: Evidence from the U.S. - Chauvet, Marcelle ELSEVIER, 2022, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:165 ; year:2019 ; day:15 ; month:02 ; pages:486-495 ; extent:10 |
| Links: |
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| DOI / URN: |
10.1016/j.actamat.2018.12.024 |
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ELV045493324 |
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| 245 | 1 | 0 | |a High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture |
| 264 | 1 | |c 2019transfer abstract | |
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| 520 | |a Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. | ||
| 520 | |a Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. | ||
| 650 | 7 | |a Polymorphic phase boundary |2 Elsevier | |
| 650 | 7 | |a Crystallographic texture |2 Elsevier | |
| 650 | 7 | |a Piezoelectricity |2 Elsevier | |
| 650 | 7 | |a Potassium-sodium niobate |2 Elsevier | |
| 700 | 1 | |a Huan, Yu |4 oth | |
| 700 | 1 | |a Yang, Weiwei |4 oth | |
| 700 | 1 | |a Zhu, Fangyuan |4 oth | |
| 700 | 1 | |a Li, Xiaolong |4 oth | |
| 700 | 1 | |a Zhang, Xingmin |4 oth | |
| 700 | 1 | |a Shen, Bo |4 oth | |
| 700 | 1 | |a Zhai, Jiwei |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier Science |a Chauvet, Marcelle ELSEVIER |t Nonlinear relationship between monetary policy and stock returns: Evidence from the U.S. |d 2022 |g Amsterdam [u.a.] |w (DE-627)ELV009239057 |
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10.1016/j.actamat.2018.12.024 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001731.pica (DE-627)ELV045493324 (ELSEVIER)S1359-6454(18)30966-2 DE-627 ger DE-627 rakwb eng 330 VZ Li, Peng verfasserin aut High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Polymorphic phase boundary Elsevier Crystallographic texture Elsevier Piezoelectricity Elsevier Potassium-sodium niobate Elsevier Huan, Yu oth Yang, Weiwei oth Zhu, Fangyuan oth Li, Xiaolong oth Zhang, Xingmin oth Shen, Bo oth Zhai, Jiwei oth Enthalten in Elsevier Science Chauvet, Marcelle ELSEVIER Nonlinear relationship between monetary policy and stock returns: Evidence from the U.S. 2022 Amsterdam [u.a.] (DE-627)ELV009239057 volume:165 year:2019 day:15 month:02 pages:486-495 extent:10 https://doi.org/10.1016/j.actamat.2018.12.024 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U AR 165 2019 15 0215 486-495 10 |
| spelling |
10.1016/j.actamat.2018.12.024 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001731.pica (DE-627)ELV045493324 (ELSEVIER)S1359-6454(18)30966-2 DE-627 ger DE-627 rakwb eng 330 VZ Li, Peng verfasserin aut High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Polymorphic phase boundary Elsevier Crystallographic texture Elsevier Piezoelectricity Elsevier Potassium-sodium niobate Elsevier Huan, Yu oth Yang, Weiwei oth Zhu, Fangyuan oth Li, Xiaolong oth Zhang, Xingmin oth Shen, Bo oth Zhai, Jiwei oth Enthalten in Elsevier Science Chauvet, Marcelle ELSEVIER Nonlinear relationship between monetary policy and stock returns: Evidence from the U.S. 2022 Amsterdam [u.a.] (DE-627)ELV009239057 volume:165 year:2019 day:15 month:02 pages:486-495 extent:10 https://doi.org/10.1016/j.actamat.2018.12.024 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U AR 165 2019 15 0215 486-495 10 |
| allfields_unstemmed |
10.1016/j.actamat.2018.12.024 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001731.pica (DE-627)ELV045493324 (ELSEVIER)S1359-6454(18)30966-2 DE-627 ger DE-627 rakwb eng 330 VZ Li, Peng verfasserin aut High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Polymorphic phase boundary Elsevier Crystallographic texture Elsevier Piezoelectricity Elsevier Potassium-sodium niobate Elsevier Huan, Yu oth Yang, Weiwei oth Zhu, Fangyuan oth Li, Xiaolong oth Zhang, Xingmin oth Shen, Bo oth Zhai, Jiwei oth Enthalten in Elsevier Science Chauvet, Marcelle ELSEVIER Nonlinear relationship between monetary policy and stock returns: Evidence from the U.S. 2022 Amsterdam [u.a.] (DE-627)ELV009239057 volume:165 year:2019 day:15 month:02 pages:486-495 extent:10 https://doi.org/10.1016/j.actamat.2018.12.024 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U AR 165 2019 15 0215 486-495 10 |
| allfieldsGer |
10.1016/j.actamat.2018.12.024 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001731.pica (DE-627)ELV045493324 (ELSEVIER)S1359-6454(18)30966-2 DE-627 ger DE-627 rakwb eng 330 VZ Li, Peng verfasserin aut High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Polymorphic phase boundary Elsevier Crystallographic texture Elsevier Piezoelectricity Elsevier Potassium-sodium niobate Elsevier Huan, Yu oth Yang, Weiwei oth Zhu, Fangyuan oth Li, Xiaolong oth Zhang, Xingmin oth Shen, Bo oth Zhai, Jiwei oth Enthalten in Elsevier Science Chauvet, Marcelle ELSEVIER Nonlinear relationship between monetary policy and stock returns: Evidence from the U.S. 2022 Amsterdam [u.a.] (DE-627)ELV009239057 volume:165 year:2019 day:15 month:02 pages:486-495 extent:10 https://doi.org/10.1016/j.actamat.2018.12.024 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U AR 165 2019 15 0215 486-495 10 |
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10.1016/j.actamat.2018.12.024 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001731.pica (DE-627)ELV045493324 (ELSEVIER)S1359-6454(18)30966-2 DE-627 ger DE-627 rakwb eng 330 VZ Li, Peng verfasserin aut High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. Polymorphic phase boundary Elsevier Crystallographic texture Elsevier Piezoelectricity Elsevier Potassium-sodium niobate Elsevier Huan, Yu oth Yang, Weiwei oth Zhu, Fangyuan oth Li, Xiaolong oth Zhang, Xingmin oth Shen, Bo oth Zhai, Jiwei oth Enthalten in Elsevier Science Chauvet, Marcelle ELSEVIER Nonlinear relationship between monetary policy and stock returns: Evidence from the U.S. 2022 Amsterdam [u.a.] (DE-627)ELV009239057 volume:165 year:2019 day:15 month:02 pages:486-495 extent:10 https://doi.org/10.1016/j.actamat.2018.12.024 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U AR 165 2019 15 0215 486-495 10 |
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high-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture |
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High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture |
| abstract |
Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. |
| abstractGer |
Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. |
| abstract_unstemmed |
Lead-free piezoelectric ceramics are urgently needed in the field of electromechanical conversion devices due to the restriction on the use of lead-based ceramics. In this study, the polymorphic phase boundary (PPB) were tuned by incorporating different concentration of (Bi0.5K0.5)HfO3 into the matrix (K0.5Na0.5)(Nb0.965Sb0.035)O3 CaZrO3, and the c crystallographic texture was realized by templated grain growth method. The maximal d 33 (∼550 pC/N) and k p (∼72%) were achieved in the c textured ceramics with composition around rhombohedral-orthorhombic-tetragonal (R-O-T) phase boundary. It is proposed that the enhanced piezoelectricity should be ascribed to several combined effects, which primarily contain the R-O-T phase boundary facilitating polarization rotation, the crystallographic orientation induced intrinsic piezoelectric anisotropy, electric-field-induced lattice distortion and phase transitions, and NaNbO3 seed-crystal-driven nanodomain structures. This work provides an effective solution to enhance piezoelectric properties by simultaneous tailoring polymorphic phase boundary and using crystallographic texture in potassium-sodium niobate based piezoelectric ceramics. We believe that the simple solution and design principle can also be applied to other piezoelectric ceramic systems, no matter lead-based or lead-free. |
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High-performance potassium-sodium niobate lead-free piezoelectric ceramics based on polymorphic phase boundary and crystallographic texture |
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