Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu
Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between M...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Talic, Belma [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019transfer abstract |
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| Umfang: |
9 |
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| Übergeordnetes Werk: |
Enthalten in: P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION - Garg, A. ELSEVIER, 2014, diffusion and reactions, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:332 ; year:2019 ; pages:16-24 ; extent:9 |
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| DOI / URN: |
10.1016/j.ssi.2019.01.008 |
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| 520 | |a Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. | ||
| 520 | |a Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. | ||
| 700 | 1 | |a Hendriksen, Peter Vang |4 oth | |
| 700 | 1 | |a Wiik, Kjell |4 oth | |
| 700 | 1 | |a Lein, Hilde Lea |4 oth | |
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10.1016/j.ssi.2019.01.008 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000831.pica (DE-627)ELV045820414 (ELSEVIER)S0167-2738(18)30584-8 DE-627 ger DE-627 rakwb eng 610 VZ 610 VZ 44.44 bkl Talic, Belma verfasserin aut Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu 2019transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Hendriksen, Peter Vang oth Wiik, Kjell oth Lein, Hilde Lea oth Enthalten in Elsevier Science Garg, A. ELSEVIER P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION 2014 diffusion and reactions Amsterdam [u.a.] (DE-627)ELV012106844 volume:332 year:2019 pages:16-24 extent:9 https://doi.org/10.1016/j.ssi.2019.01.008 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_21 GBV_ILN_78 44.44 Parasitologie Medizin VZ AR 332 2019 16-24 9 |
| spelling |
10.1016/j.ssi.2019.01.008 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000831.pica (DE-627)ELV045820414 (ELSEVIER)S0167-2738(18)30584-8 DE-627 ger DE-627 rakwb eng 610 VZ 610 VZ 44.44 bkl Talic, Belma verfasserin aut Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu 2019transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Hendriksen, Peter Vang oth Wiik, Kjell oth Lein, Hilde Lea oth Enthalten in Elsevier Science Garg, A. ELSEVIER P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION 2014 diffusion and reactions Amsterdam [u.a.] (DE-627)ELV012106844 volume:332 year:2019 pages:16-24 extent:9 https://doi.org/10.1016/j.ssi.2019.01.008 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_21 GBV_ILN_78 44.44 Parasitologie Medizin VZ AR 332 2019 16-24 9 |
| allfields_unstemmed |
10.1016/j.ssi.2019.01.008 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000831.pica (DE-627)ELV045820414 (ELSEVIER)S0167-2738(18)30584-8 DE-627 ger DE-627 rakwb eng 610 VZ 610 VZ 44.44 bkl Talic, Belma verfasserin aut Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu 2019transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Hendriksen, Peter Vang oth Wiik, Kjell oth Lein, Hilde Lea oth Enthalten in Elsevier Science Garg, A. ELSEVIER P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION 2014 diffusion and reactions Amsterdam [u.a.] (DE-627)ELV012106844 volume:332 year:2019 pages:16-24 extent:9 https://doi.org/10.1016/j.ssi.2019.01.008 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_21 GBV_ILN_78 44.44 Parasitologie Medizin VZ AR 332 2019 16-24 9 |
| allfieldsGer |
10.1016/j.ssi.2019.01.008 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000831.pica (DE-627)ELV045820414 (ELSEVIER)S0167-2738(18)30584-8 DE-627 ger DE-627 rakwb eng 610 VZ 610 VZ 44.44 bkl Talic, Belma verfasserin aut Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu 2019transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Hendriksen, Peter Vang oth Wiik, Kjell oth Lein, Hilde Lea oth Enthalten in Elsevier Science Garg, A. ELSEVIER P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION 2014 diffusion and reactions Amsterdam [u.a.] (DE-627)ELV012106844 volume:332 year:2019 pages:16-24 extent:9 https://doi.org/10.1016/j.ssi.2019.01.008 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_21 GBV_ILN_78 44.44 Parasitologie Medizin VZ AR 332 2019 16-24 9 |
| allfieldsSound |
10.1016/j.ssi.2019.01.008 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000831.pica (DE-627)ELV045820414 (ELSEVIER)S0167-2738(18)30584-8 DE-627 ger DE-627 rakwb eng 610 VZ 610 VZ 44.44 bkl Talic, Belma verfasserin aut Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu 2019transfer abstract 9 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. Hendriksen, Peter Vang oth Wiik, Kjell oth Lein, Hilde Lea oth Enthalten in Elsevier Science Garg, A. ELSEVIER P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION 2014 diffusion and reactions Amsterdam [u.a.] (DE-627)ELV012106844 volume:332 year:2019 pages:16-24 extent:9 https://doi.org/10.1016/j.ssi.2019.01.008 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_21 GBV_ILN_78 44.44 Parasitologie Medizin VZ AR 332 2019 16-24 9 |
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Enthalten in P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION Amsterdam [u.a.] volume:332 year:2019 pages:16-24 extent:9 |
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Enthalten in P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION Amsterdam [u.a.] volume:332 year:2019 pages:16-24 extent:9 |
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P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION |
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P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION |
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P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION |
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Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu |
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Talic, Belma |
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P616 TGFβ1 STIMULATION OF HUMAN BONE MARROW MESENCHYMAL STEM CELLS (MSC) ENHANCES THEIR HEPATIC ENGRAFTMENT AND THERAPEUTIC EFFECT IN INJURED LIVER VIA UPREGULATION OF CXCR3 FUNCTION |
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diffusion couple study of the interaction between cr2o3 and mnco2o4 doped with fe and cu |
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Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu |
| abstract |
Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. |
| abstractGer |
Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. |
| abstract_unstemmed |
Manganese cobalt spinel oxides are promising coating materials for the protection of ferritic stainless steel interconnects in solid oxide fuel cell (SOFC) stacks. The interaction between such coatings and the steel is here studied using diffusion couples as a model system. The interaction between MnCo2O4, MnCo1.7Fe0.3O4 and MnCo1.7Cu0.3O4 spinels and Cr2O3 was studied in air at 900 °C. In all cases, a reaction layer rich in Co and Cr formed at the interfaces. Using Pt-particles to mark the original interface reveals that the reaction layers grow by diffusion of Co (and Mn) from the spinel oxides to the Cr2O3/reaction layer interface. The growth of the reaction layers followed parabolic kinetics with rate constants of 1.3 × 10−5 μm2 s−1 for the MnCo2O4/Cr2O3 couple, 8.6 × 10−6 μm2 s−1 for the MnCo1.7Fe0.3O4/Cr2O3 couple, and finally 1.2 × 10−4 μm2 s−1 for the MnCo1.7Cu0.3O4/Cr2O3 couple. |
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Diffusion couple study of the interaction between Cr2O3 and MnCo2O4 doped with Fe and Cu |
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