Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications
Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membrane...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Ding, Liming [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019transfer abstract |
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| Schlagwörter: |
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| Umfang: |
10 |
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| Übergeordnetes Werk: |
Enthalten in: Steering charge kinetics in W - Yue, Xin-Zheng ELSEVIER, 2019, the official journal of the North American Membrane Society, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:578 ; year:2019 ; day:15 ; month:05 ; pages:126-135 ; extent:10 |
| Links: |
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| DOI / URN: |
10.1016/j.memsci.2019.02.050 |
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| 245 | 1 | 0 | |a Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications |
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| 520 | |a Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. | ||
| 520 | |a Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. | ||
| 650 | 7 | |a Vanaduim redox flow battery |2 Elsevier | |
| 650 | 7 | |a Enhance proton conductivity |2 Elsevier | |
| 650 | 7 | |a Sulfonated polybenzimidazoles |2 Elsevier | |
| 650 | 7 | |a Proton exchange membrane |2 Elsevier | |
| 700 | 1 | |a Song, Xipeng |4 oth | |
| 700 | 1 | |a Wang, Lihua |4 oth | |
| 700 | 1 | |a Zhao, Zhiping |4 oth | |
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10.1016/j.memsci.2019.02.050 doi GBV00000000000729.pica (DE-627)ELV04598171X (ELSEVIER)S0376-7388(18)33434-3 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Ding, Liming verfasserin aut Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Vanaduim redox flow battery Elsevier Enhance proton conductivity Elsevier Sulfonated polybenzimidazoles Elsevier Proton exchange membrane Elsevier Song, Xipeng oth Wang, Lihua oth Zhao, Zhiping oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:578 year:2019 day:15 month:05 pages:126-135 extent:10 https://doi.org/10.1016/j.memsci.2019.02.050 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 578 2019 15 0515 126-135 10 |
| spelling |
10.1016/j.memsci.2019.02.050 doi GBV00000000000729.pica (DE-627)ELV04598171X (ELSEVIER)S0376-7388(18)33434-3 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Ding, Liming verfasserin aut Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Vanaduim redox flow battery Elsevier Enhance proton conductivity Elsevier Sulfonated polybenzimidazoles Elsevier Proton exchange membrane Elsevier Song, Xipeng oth Wang, Lihua oth Zhao, Zhiping oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:578 year:2019 day:15 month:05 pages:126-135 extent:10 https://doi.org/10.1016/j.memsci.2019.02.050 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 578 2019 15 0515 126-135 10 |
| allfields_unstemmed |
10.1016/j.memsci.2019.02.050 doi GBV00000000000729.pica (DE-627)ELV04598171X (ELSEVIER)S0376-7388(18)33434-3 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Ding, Liming verfasserin aut Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Vanaduim redox flow battery Elsevier Enhance proton conductivity Elsevier Sulfonated polybenzimidazoles Elsevier Proton exchange membrane Elsevier Song, Xipeng oth Wang, Lihua oth Zhao, Zhiping oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:578 year:2019 day:15 month:05 pages:126-135 extent:10 https://doi.org/10.1016/j.memsci.2019.02.050 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 578 2019 15 0515 126-135 10 |
| allfieldsGer |
10.1016/j.memsci.2019.02.050 doi GBV00000000000729.pica (DE-627)ELV04598171X (ELSEVIER)S0376-7388(18)33434-3 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Ding, Liming verfasserin aut Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Vanaduim redox flow battery Elsevier Enhance proton conductivity Elsevier Sulfonated polybenzimidazoles Elsevier Proton exchange membrane Elsevier Song, Xipeng oth Wang, Lihua oth Zhao, Zhiping oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:578 year:2019 day:15 month:05 pages:126-135 extent:10 https://doi.org/10.1016/j.memsci.2019.02.050 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 578 2019 15 0515 126-135 10 |
| allfieldsSound |
10.1016/j.memsci.2019.02.050 doi GBV00000000000729.pica (DE-627)ELV04598171X (ELSEVIER)S0376-7388(18)33434-3 DE-627 ger DE-627 rakwb eng 540 VZ 35.17 bkl 58.50 bkl 43.12 bkl Ding, Liming verfasserin aut Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. Vanaduim redox flow battery Elsevier Enhance proton conductivity Elsevier Sulfonated polybenzimidazoles Elsevier Proton exchange membrane Elsevier Song, Xipeng oth Wang, Lihua oth Zhao, Zhiping oth Enthalten in Elsevier Yue, Xin-Zheng ELSEVIER Steering charge kinetics in W 2019 the official journal of the North American Membrane Society New York, NY [u.a.] (DE-627)ELV002478420 volume:578 year:2019 day:15 month:05 pages:126-135 extent:10 https://doi.org/10.1016/j.memsci.2019.02.050 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.17 Katalyse VZ 58.50 Umwelttechnik: Allgemeines VZ 43.12 Umweltchemie VZ AR 578 2019 15 0515 126-135 10 |
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But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. 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enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications |
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Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications |
| abstract |
Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. |
| abstractGer |
Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. |
| abstract_unstemmed |
Acid doped polybenzimidazole membrane can transport protons and is a potential proton exchange membrane for vanadium redox flow battery applications. But the proton conductivity of polybenzimidazole membranes is just moderate; the vanadium redox flow battery assembled with polybenzimidazole membranes usual cannot achieve satisfactory voltage efficiency. Therefore, the main aim of this study is to prepare high proton conductivity polybenzimidazole membranes. A series of sulfonated polybenzimidazoles with different sulfonation degree are synthesized. The 5-sulfoisophthalic acid monosodium salt is introduced not only to control the sulfonation degree of the polymer but also to enhance the hydrophilicity of polybenzimidazole and further increase the proton conductivity of polybenzimidazole membrane. The physicochemical properties and single cell performance of sulfonated polybenzimidazoles membranes are thoroughly assessed. The results indicate that the water uptake of membranes are enhanced as the sulfonation degree increases and is superior to increase the proton conductivity. But sulfonate can also form hydrogen bonds with the basic groups N= in imidazole rings and block the protons transport. Ultimately, sulfonated polybenzimidazole membrane with the sulfonation degree of 30% exhibites the highest proton conductivity as well as energy efficiency. |
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Enhancing proton conductivity of polybenzimidazole membranes by introducing sulfonate for vanadium redox flow batteries applications |
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