Bi<ce:inf loc="post">2</ce:inf>S<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed Bi<ce:inf loc="post">2</ce:inf>WO<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity
Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution....
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Xu, Xiaoming [verfasserIn] |
|---|
| Format: |
E-Artikel |
|---|---|
| Sprache: |
Englisch |
| Erschienen: |
2019transfer abstract |
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| Umfang: |
13 |
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| Übergeordnetes Werk: |
Enthalten in: Characterising shape patterns using features derived from best-fitting ellipsoids - Gontar, Amelia ELSEVIER, 2018, a journal devoted to applied physics and chemistry of surfaces and interfaces, Amsterdam |
|---|---|
| Übergeordnetes Werk: |
volume:479 ; year:2019 ; day:15 ; month:06 ; pages:410-422 ; extent:13 |
| Links: |
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| DOI / URN: |
10.1016/j.apsusc.2019.02.086 |
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| 520 | |a Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. | ||
| 520 | |a Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. | ||
| 700 | 1 | |a Meng, Lingjun |4 oth | |
| 700 | 1 | |a Li, Yong |4 oth | |
| 700 | 1 | |a Sun, Cheng |4 oth | |
| 700 | 1 | |a Yang, Shaogui |4 oth | |
| 700 | 1 | |a He, Huan |4 oth | |
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10.1016/j.apsusc.2019.02.086 doi GBV00000000000590.pica (DE-627)ELV046500170 (ELSEVIER)S0169-4332(19)30428-3 DE-627 ger DE-627 rakwb eng 000 150 VZ 54.74 bkl Xu, Xiaoming verfasserin aut Bi<ce:inf loc="post">2</ce:inf>S<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed Bi<ce:inf loc="post">2</ce:inf>WO<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity 2019transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Meng, Lingjun oth Li, Yong oth Sun, Cheng oth Yang, Shaogui oth He, Huan oth Enthalten in Elsevier Gontar, Amelia ELSEVIER Characterising shape patterns using features derived from best-fitting ellipsoids 2018 a journal devoted to applied physics and chemistry of surfaces and interfaces Amsterdam (DE-627)ELV000097942 volume:479 year:2019 day:15 month:06 pages:410-422 extent:13 https://doi.org/10.1016/j.apsusc.2019.02.086 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.74 Maschinelles Sehen VZ AR 479 2019 15 0615 410-422 13 |
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10.1016/j.apsusc.2019.02.086 doi GBV00000000000590.pica (DE-627)ELV046500170 (ELSEVIER)S0169-4332(19)30428-3 DE-627 ger DE-627 rakwb eng 000 150 VZ 54.74 bkl Xu, Xiaoming verfasserin aut Bi<ce:inf loc="post">2</ce:inf>S<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed Bi<ce:inf loc="post">2</ce:inf>WO<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity 2019transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Meng, Lingjun oth Li, Yong oth Sun, Cheng oth Yang, Shaogui oth He, Huan oth Enthalten in Elsevier Gontar, Amelia ELSEVIER Characterising shape patterns using features derived from best-fitting ellipsoids 2018 a journal devoted to applied physics and chemistry of surfaces and interfaces Amsterdam (DE-627)ELV000097942 volume:479 year:2019 day:15 month:06 pages:410-422 extent:13 https://doi.org/10.1016/j.apsusc.2019.02.086 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.74 Maschinelles Sehen VZ AR 479 2019 15 0615 410-422 13 |
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10.1016/j.apsusc.2019.02.086 doi GBV00000000000590.pica (DE-627)ELV046500170 (ELSEVIER)S0169-4332(19)30428-3 DE-627 ger DE-627 rakwb eng 000 150 VZ 54.74 bkl Xu, Xiaoming verfasserin aut Bi<ce:inf loc="post">2</ce:inf>S<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed Bi<ce:inf loc="post">2</ce:inf>WO<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity 2019transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Meng, Lingjun oth Li, Yong oth Sun, Cheng oth Yang, Shaogui oth He, Huan oth Enthalten in Elsevier Gontar, Amelia ELSEVIER Characterising shape patterns using features derived from best-fitting ellipsoids 2018 a journal devoted to applied physics and chemistry of surfaces and interfaces Amsterdam (DE-627)ELV000097942 volume:479 year:2019 day:15 month:06 pages:410-422 extent:13 https://doi.org/10.1016/j.apsusc.2019.02.086 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.74 Maschinelles Sehen VZ AR 479 2019 15 0615 410-422 13 |
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10.1016/j.apsusc.2019.02.086 doi GBV00000000000590.pica (DE-627)ELV046500170 (ELSEVIER)S0169-4332(19)30428-3 DE-627 ger DE-627 rakwb eng 000 150 VZ 54.74 bkl Xu, Xiaoming verfasserin aut Bi<ce:inf loc="post">2</ce:inf>S<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed Bi<ce:inf loc="post">2</ce:inf>WO<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity 2019transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Meng, Lingjun oth Li, Yong oth Sun, Cheng oth Yang, Shaogui oth He, Huan oth Enthalten in Elsevier Gontar, Amelia ELSEVIER Characterising shape patterns using features derived from best-fitting ellipsoids 2018 a journal devoted to applied physics and chemistry of surfaces and interfaces Amsterdam (DE-627)ELV000097942 volume:479 year:2019 day:15 month:06 pages:410-422 extent:13 https://doi.org/10.1016/j.apsusc.2019.02.086 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.74 Maschinelles Sehen VZ AR 479 2019 15 0615 410-422 13 |
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10.1016/j.apsusc.2019.02.086 doi GBV00000000000590.pica (DE-627)ELV046500170 (ELSEVIER)S0169-4332(19)30428-3 DE-627 ger DE-627 rakwb eng 000 150 VZ 54.74 bkl Xu, Xiaoming verfasserin aut Bi<ce:inf loc="post">2</ce:inf>S<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed Bi<ce:inf loc="post">2</ce:inf>WO<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity 2019transfer abstract 13 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. Meng, Lingjun oth Li, Yong oth Sun, Cheng oth Yang, Shaogui oth He, Huan oth Enthalten in Elsevier Gontar, Amelia ELSEVIER Characterising shape patterns using features derived from best-fitting ellipsoids 2018 a journal devoted to applied physics and chemistry of surfaces and interfaces Amsterdam (DE-627)ELV000097942 volume:479 year:2019 day:15 month:06 pages:410-422 extent:13 https://doi.org/10.1016/j.apsusc.2019.02.086 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 54.74 Maschinelles Sehen VZ AR 479 2019 15 0615 410-422 13 |
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Bi<ce:inf loc="post">2</ce:inf>S<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed Bi<ce:inf loc="post">2</ce:inf>WO<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity |
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bi<ce:inf loc="post">2</ce:inf>s<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed bi<ce:inf loc="post">2</ce:inf>wo<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity |
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Bi<ce:inf loc="post">2</ce:inf>S<ce:inf loc="post">3</ce:inf> nanoribbons-hybridized {001} facets exposed Bi<ce:inf loc="post">2</ce:inf>WO<ce:inf loc="post">6</ce:inf> ultrathin nanosheets with enhanced visible light photocatalytic activity |
| abstract |
Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. |
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Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. |
| abstract_unstemmed |
Bi2S3 nanoribbons were dispersed in situ on Bi2WO6 ultrathin nanosheets with exposed {001} facet via a simple one-set hydrothermal route forming Bi2S3/Bi2WO6 heterojunctions with high active surface, in which the quantity of Bi2S3 nanoribbons was tuned by changing the amount of thiourea in solution. The obtained composites were characterized by various measurements and their photocatalytic activities under visible-light irradiation were also investigated. The 7%-Bi2S3/Bi2WO6 nanocomposites exhibited excellent photocatalytic activities in degradation of ofloxacin (OFL). A plausible degradation pathway for OFL was proposed via combining LC-MS and GC–MS detections with Gaussian calculations. The probable photocatalytic and formation mechanism of catalysts were discussed on the basis of the obtained experimental results and density function theory (DFT) calculations. An enhanced photocatalytic mechanism attributed to the synergistic effect between the exposed {001} facet and heterojunction with shape-crystalline integrity, significantly improving band structure and visible light absorption, increasing reactive sites, and suppressing the recombination of charges. The findings provide new insights for designing highly active and stable heterojunction catalysts to remove environmental pollutants and promote solar energy conversion efficiently. |
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Meng, Lingjun Li, Yong Sun, Cheng Yang, Shaogui He, Huan |
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