Ag loaded B-doped-g C3N4 nanosheet with efficient properties for photocatalysis
Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Thorat, Nirmala [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019transfer abstract |
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| Schlagwörter: |
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| Umfang: |
10 |
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| Übergeordnetes Werk: |
Enthalten in: Cohort, signaling, and early-career dynamics: The hidden significance of class in black-white earnings inequality - Ren, Chunhui ELSEVIER, 2022, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:247 ; year:2019 ; day:1 ; month:10 ; pages:57-66 ; extent:10 |
| Links: |
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| DOI / URN: |
10.1016/j.jenvman.2019.06.043 |
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ELV047568984 |
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| 520 | |a Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. | ||
| 520 | |a Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. | ||
| 650 | 7 | |a B doping |2 Elsevier | |
| 650 | 7 | |a Ag nanoparticle |2 Elsevier | |
| 650 | 7 | |a Recombination rate |2 Elsevier | |
| 650 | 7 | |a Plasmonic |2 Elsevier | |
| 650 | 7 | |a g-C3N4 nanosheet |2 Elsevier | |
| 650 | 7 | |a Graphitic carbon nitride |2 Elsevier | |
| 700 | 1 | |a Yadav, Asha |4 oth | |
| 700 | 1 | |a Yadav, Manisha |4 oth | |
| 700 | 1 | |a Gupta, Suraj |4 oth | |
| 700 | 1 | |a Varma, Ranjana |4 oth | |
| 700 | 1 | |a Pillai, Saju |4 oth | |
| 700 | 1 | |a Fernandes, Rohan |4 oth | |
| 700 | 1 | |a Patel, Maulik |4 oth | |
| 700 | 1 | |a Patel, Nainesh |4 oth | |
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10.1016/j.jenvman.2019.06.043 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001160.pica (DE-627)ELV047568984 (ELSEVIER)S0301-4797(19)30838-2 DE-627 ger DE-627 rakwb eng 300 VZ 70.00 bkl 71.00 bkl Thorat, Nirmala verfasserin aut Ag loaded B-doped-g C3N4 nanosheet with efficient properties for photocatalysis 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. B doping Elsevier Ag nanoparticle Elsevier Recombination rate Elsevier Plasmonic Elsevier g-C3N4 nanosheet Elsevier Graphitic carbon nitride Elsevier Yadav, Asha oth Yadav, Manisha oth Gupta, Suraj oth Varma, Ranjana oth Pillai, Saju oth Fernandes, Rohan oth Patel, Maulik oth Patel, Nainesh oth Enthalten in Elsevier Ren, Chunhui ELSEVIER Cohort, signaling, and early-career dynamics: The hidden significance of class in black-white earnings inequality 2022 Amsterdam [u.a.] (DE-627)ELV008002754 volume:247 year:2019 day:1 month:10 pages:57-66 extent:10 https://doi.org/10.1016/j.jenvman.2019.06.043 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 70.00 Sozialwissenschaften allgemein: Allgemeines VZ 71.00 Soziologie: Allgemeines VZ AR 247 2019 1 1001 57-66 10 |
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10.1016/j.jenvman.2019.06.043 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001160.pica (DE-627)ELV047568984 (ELSEVIER)S0301-4797(19)30838-2 DE-627 ger DE-627 rakwb eng 300 VZ 70.00 bkl 71.00 bkl Thorat, Nirmala verfasserin aut Ag loaded B-doped-g C3N4 nanosheet with efficient properties for photocatalysis 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. B doping Elsevier Ag nanoparticle Elsevier Recombination rate Elsevier Plasmonic Elsevier g-C3N4 nanosheet Elsevier Graphitic carbon nitride Elsevier Yadav, Asha oth Yadav, Manisha oth Gupta, Suraj oth Varma, Ranjana oth Pillai, Saju oth Fernandes, Rohan oth Patel, Maulik oth Patel, Nainesh oth Enthalten in Elsevier Ren, Chunhui ELSEVIER Cohort, signaling, and early-career dynamics: The hidden significance of class in black-white earnings inequality 2022 Amsterdam [u.a.] (DE-627)ELV008002754 volume:247 year:2019 day:1 month:10 pages:57-66 extent:10 https://doi.org/10.1016/j.jenvman.2019.06.043 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 70.00 Sozialwissenschaften allgemein: Allgemeines VZ 71.00 Soziologie: Allgemeines VZ AR 247 2019 1 1001 57-66 10 |
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10.1016/j.jenvman.2019.06.043 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001160.pica (DE-627)ELV047568984 (ELSEVIER)S0301-4797(19)30838-2 DE-627 ger DE-627 rakwb eng 300 VZ 70.00 bkl 71.00 bkl Thorat, Nirmala verfasserin aut Ag loaded B-doped-g C3N4 nanosheet with efficient properties for photocatalysis 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. B doping Elsevier Ag nanoparticle Elsevier Recombination rate Elsevier Plasmonic Elsevier g-C3N4 nanosheet Elsevier Graphitic carbon nitride Elsevier Yadav, Asha oth Yadav, Manisha oth Gupta, Suraj oth Varma, Ranjana oth Pillai, Saju oth Fernandes, Rohan oth Patel, Maulik oth Patel, Nainesh oth Enthalten in Elsevier Ren, Chunhui ELSEVIER Cohort, signaling, and early-career dynamics: The hidden significance of class in black-white earnings inequality 2022 Amsterdam [u.a.] (DE-627)ELV008002754 volume:247 year:2019 day:1 month:10 pages:57-66 extent:10 https://doi.org/10.1016/j.jenvman.2019.06.043 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 70.00 Sozialwissenschaften allgemein: Allgemeines VZ 71.00 Soziologie: Allgemeines VZ AR 247 2019 1 1001 57-66 10 |
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10.1016/j.jenvman.2019.06.043 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001160.pica (DE-627)ELV047568984 (ELSEVIER)S0301-4797(19)30838-2 DE-627 ger DE-627 rakwb eng 300 VZ 70.00 bkl 71.00 bkl Thorat, Nirmala verfasserin aut Ag loaded B-doped-g C3N4 nanosheet with efficient properties for photocatalysis 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. B doping Elsevier Ag nanoparticle Elsevier Recombination rate Elsevier Plasmonic Elsevier g-C3N4 nanosheet Elsevier Graphitic carbon nitride Elsevier Yadav, Asha oth Yadav, Manisha oth Gupta, Suraj oth Varma, Ranjana oth Pillai, Saju oth Fernandes, Rohan oth Patel, Maulik oth Patel, Nainesh oth Enthalten in Elsevier Ren, Chunhui ELSEVIER Cohort, signaling, and early-career dynamics: The hidden significance of class in black-white earnings inequality 2022 Amsterdam [u.a.] (DE-627)ELV008002754 volume:247 year:2019 day:1 month:10 pages:57-66 extent:10 https://doi.org/10.1016/j.jenvman.2019.06.043 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 70.00 Sozialwissenschaften allgemein: Allgemeines VZ 71.00 Soziologie: Allgemeines VZ AR 247 2019 1 1001 57-66 10 |
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10.1016/j.jenvman.2019.06.043 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001160.pica (DE-627)ELV047568984 (ELSEVIER)S0301-4797(19)30838-2 DE-627 ger DE-627 rakwb eng 300 VZ 70.00 bkl 71.00 bkl Thorat, Nirmala verfasserin aut Ag loaded B-doped-g C3N4 nanosheet with efficient properties for photocatalysis 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. B doping Elsevier Ag nanoparticle Elsevier Recombination rate Elsevier Plasmonic Elsevier g-C3N4 nanosheet Elsevier Graphitic carbon nitride Elsevier Yadav, Asha oth Yadav, Manisha oth Gupta, Suraj oth Varma, Ranjana oth Pillai, Saju oth Fernandes, Rohan oth Patel, Maulik oth Patel, Nainesh oth Enthalten in Elsevier Ren, Chunhui ELSEVIER Cohort, signaling, and early-career dynamics: The hidden significance of class in black-white earnings inequality 2022 Amsterdam [u.a.] (DE-627)ELV008002754 volume:247 year:2019 day:1 month:10 pages:57-66 extent:10 https://doi.org/10.1016/j.jenvman.2019.06.043 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 70.00 Sozialwissenschaften allgemein: Allgemeines VZ 71.00 Soziologie: Allgemeines VZ AR 247 2019 1 1001 57-66 10 |
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Enthalten in Cohort, signaling, and early-career dynamics: The hidden significance of class in black-white earnings inequality Amsterdam [u.a.] volume:247 year:2019 day:1 month:10 pages:57-66 extent:10 |
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Enthalten in Cohort, signaling, and early-career dynamics: The hidden significance of class in black-white earnings inequality Amsterdam [u.a.] volume:247 year:2019 day:1 month:10 pages:57-66 extent:10 |
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Ag loaded B-doped-g C3N4 nanosheet with efficient properties for photocatalysis |
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Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. |
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Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. |
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Three material engineering strategies in the form of doping (Boron-doping), nanostructuring (nanosheet (NS) formation) and decorating with plasmonic nanoparticles (loading with Ag metal), were integrated to improve the photocatalytic activity of graphitic carbon nitride (gC3N4). Concentrations of B-doping and Ag-loading were optimized to maximize the catalytic performance in the final nanocomposite of Ag-loaded B-doped gC3N4 NS. Combined effect of all three strategies successfully produced over 5 times higher rate towards degradation of organic dye pollutant, when compared to unmodified bulk gC3N4. Detailed characterization results revealed that incorporation of B in gC3N4 matrix reduces the band gap to increase the visible light absorption, while specific surface area is significantly enhanced upon formation of NS. Decoration of Ag nanoparticles (NPs) on B-doped gC3N4 NS assists in fast transfer of photogenerated electrons from gC3N4 to Ag NPs owing to the interfacial electric field across the junctions and thus reduces the recombination process. Investigations on individual strategies revealed that decoration of Ag NPs to induce better charge separation, is the most effective route for enhancing the photocatalytic activity. |
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