Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere
Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chem...
Ausführliche Beschreibung
Autor*in: |
Sarwar, Golam [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
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2019transfer abstract |
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Umfang: |
10 |
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Übergeordnetes Werk: |
Enthalten in: The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction - Nassar, M.K. ELSEVIER, 2021, Amsterdam [u.a.] |
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Übergeordnetes Werk: |
volume:213 ; year:2019 ; day:15 ; month:09 ; pages:395-404 ; extent:10 |
Links: |
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DOI / URN: |
10.1016/j.atmosenv.2019.06.020 |
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ELV047615532 |
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520 | |a Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. | ||
520 | |a Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. | ||
650 | 7 | |a Bromine |2 Elsevier | |
650 | 7 | |a CMAQ |2 Elsevier | |
650 | 7 | |a Ozone |2 Elsevier | |
650 | 7 | |a Background ozone |2 Elsevier | |
650 | 7 | |a Iodine |2 Elsevier | |
700 | 1 | |a Gantt, Brett |4 oth | |
700 | 1 | |a Foley, Kristen |4 oth | |
700 | 1 | |a Fahey, Kathleen |4 oth | |
700 | 1 | |a Spero, Tanya L. |4 oth | |
700 | 1 | |a Kang, Daiwen |4 oth | |
700 | 1 | |a Mathur, Rohit |4 oth | |
700 | 1 | |a Foroutan, Hosein |4 oth | |
700 | 1 | |a Xing, Jia |4 oth | |
700 | 1 | |a Sherwen, Tomás |4 oth | |
700 | 1 | |a Saiz-Lopez, Alfonso |4 oth | |
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10.1016/j.atmosenv.2019.06.020 doi GBV00000000000739.pica (DE-627)ELV047615532 (ELSEVIER)S1352-2310(19)30411-X DE-627 ger DE-627 rakwb eng 610 VZ 44.65 bkl Sarwar, Golam verfasserin aut Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine Elsevier CMAQ Elsevier Ozone Elsevier Background ozone Elsevier Iodine Elsevier Gantt, Brett oth Foley, Kristen oth Fahey, Kathleen oth Spero, Tanya L. oth Kang, Daiwen oth Mathur, Rohit oth Foroutan, Hosein oth Xing, Jia oth Sherwen, Tomás oth Saiz-Lopez, Alfonso oth Enthalten in Elsevier Science Nassar, M.K. ELSEVIER The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction 2021 Amsterdam [u.a.] (DE-627)ELV00656139X volume:213 year:2019 day:15 month:09 pages:395-404 extent:10 https://doi.org/10.1016/j.atmosenv.2019.06.020 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.65 Chirurgie VZ AR 213 2019 15 0915 395-404 10 |
spelling |
10.1016/j.atmosenv.2019.06.020 doi GBV00000000000739.pica (DE-627)ELV047615532 (ELSEVIER)S1352-2310(19)30411-X DE-627 ger DE-627 rakwb eng 610 VZ 44.65 bkl Sarwar, Golam verfasserin aut Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine Elsevier CMAQ Elsevier Ozone Elsevier Background ozone Elsevier Iodine Elsevier Gantt, Brett oth Foley, Kristen oth Fahey, Kathleen oth Spero, Tanya L. oth Kang, Daiwen oth Mathur, Rohit oth Foroutan, Hosein oth Xing, Jia oth Sherwen, Tomás oth Saiz-Lopez, Alfonso oth Enthalten in Elsevier Science Nassar, M.K. ELSEVIER The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction 2021 Amsterdam [u.a.] (DE-627)ELV00656139X volume:213 year:2019 day:15 month:09 pages:395-404 extent:10 https://doi.org/10.1016/j.atmosenv.2019.06.020 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.65 Chirurgie VZ AR 213 2019 15 0915 395-404 10 |
allfields_unstemmed |
10.1016/j.atmosenv.2019.06.020 doi GBV00000000000739.pica (DE-627)ELV047615532 (ELSEVIER)S1352-2310(19)30411-X DE-627 ger DE-627 rakwb eng 610 VZ 44.65 bkl Sarwar, Golam verfasserin aut Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine Elsevier CMAQ Elsevier Ozone Elsevier Background ozone Elsevier Iodine Elsevier Gantt, Brett oth Foley, Kristen oth Fahey, Kathleen oth Spero, Tanya L. oth Kang, Daiwen oth Mathur, Rohit oth Foroutan, Hosein oth Xing, Jia oth Sherwen, Tomás oth Saiz-Lopez, Alfonso oth Enthalten in Elsevier Science Nassar, M.K. ELSEVIER The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction 2021 Amsterdam [u.a.] (DE-627)ELV00656139X volume:213 year:2019 day:15 month:09 pages:395-404 extent:10 https://doi.org/10.1016/j.atmosenv.2019.06.020 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.65 Chirurgie VZ AR 213 2019 15 0915 395-404 10 |
allfieldsGer |
10.1016/j.atmosenv.2019.06.020 doi GBV00000000000739.pica (DE-627)ELV047615532 (ELSEVIER)S1352-2310(19)30411-X DE-627 ger DE-627 rakwb eng 610 VZ 44.65 bkl Sarwar, Golam verfasserin aut Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine Elsevier CMAQ Elsevier Ozone Elsevier Background ozone Elsevier Iodine Elsevier Gantt, Brett oth Foley, Kristen oth Fahey, Kathleen oth Spero, Tanya L. oth Kang, Daiwen oth Mathur, Rohit oth Foroutan, Hosein oth Xing, Jia oth Sherwen, Tomás oth Saiz-Lopez, Alfonso oth Enthalten in Elsevier Science Nassar, M.K. ELSEVIER The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction 2021 Amsterdam [u.a.] (DE-627)ELV00656139X volume:213 year:2019 day:15 month:09 pages:395-404 extent:10 https://doi.org/10.1016/j.atmosenv.2019.06.020 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.65 Chirurgie VZ AR 213 2019 15 0915 395-404 10 |
allfieldsSound |
10.1016/j.atmosenv.2019.06.020 doi GBV00000000000739.pica (DE-627)ELV047615532 (ELSEVIER)S1352-2310(19)30411-X DE-627 ger DE-627 rakwb eng 610 VZ 44.65 bkl Sarwar, Golam verfasserin aut Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere 2019transfer abstract 10 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. Bromine Elsevier CMAQ Elsevier Ozone Elsevier Background ozone Elsevier Iodine Elsevier Gantt, Brett oth Foley, Kristen oth Fahey, Kathleen oth Spero, Tanya L. oth Kang, Daiwen oth Mathur, Rohit oth Foroutan, Hosein oth Xing, Jia oth Sherwen, Tomás oth Saiz-Lopez, Alfonso oth Enthalten in Elsevier Science Nassar, M.K. ELSEVIER The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction 2021 Amsterdam [u.a.] (DE-627)ELV00656139X volume:213 year:2019 day:15 month:09 pages:395-404 extent:10 https://doi.org/10.1016/j.atmosenv.2019.06.020 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.65 Chirurgie VZ AR 213 2019 15 0915 395-404 10 |
language |
English |
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Enthalten in The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction Amsterdam [u.a.] volume:213 year:2019 day:15 month:09 pages:395-404 extent:10 |
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Enthalten in The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction Amsterdam [u.a.] volume:213 year:2019 day:15 month:09 pages:395-404 extent:10 |
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The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction |
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The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction |
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Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere |
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The internal pudendal artery turnover (IPAT) flap: A new, simple and reliable technique for perineal reconstruction |
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influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: cmaq simulations over the northern hemisphere |
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Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere |
abstract |
Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. |
abstractGer |
Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. |
abstract_unstemmed |
Bromine and iodine chemistry has been updated in the Community Multiscale Air Quality (CMAQ) model to better capture the influence of natural emissions from the oceans on ozone concentrations. Annual simulations were performed using the hemispheric CMAQ model without and with bromine and iodine chemistry. Model results over the Northern Hemisphere show that including bromine and iodine chemistry in CMAQ not only reduces ozone concentrations within the marine boundary layer but also aloft and inland. Bromine and iodine chemistry reduces annual mean surface ozone over seawater by 25%, with lesser ozone reductions over land. The bromine and iodine chemistry decreases ozone concentration without changing the diurnal profile and is active throughout the year. However, it does not have a strong seasonal influence on ozone over the Northern Hemisphere. Model performance of CMAQ is improved by the bromine and iodine chemistry when compared to observations, especially at coastal sites and over seawater. Relative to bromine, iodine chemistry is approximately four times more effective in reducing ozone over seawater over the Northern Hemisphere (on an annual basis). Model results suggest that the chemistry modulates intercontinental transport and lowers the background ozone imported to the United States. |
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Influence of bromine and iodine chemistry on annual, seasonal, diurnal, and background ozone: CMAQ simulations over the Northern Hemisphere |
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https://doi.org/10.1016/j.atmosenv.2019.06.020 |
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