Enhancing efficiency of hydrocarbons to synthesis gas conversion in a counterflow moving bed filtration combustion reactor
An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchange...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Dorofeenko, S.O. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019transfer abstract |
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| Schlagwörter: |
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| Umfang: |
14 |
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| Übergeordnetes Werk: |
Enthalten in: External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs - Dedhia, Kavita ELSEVIER, 2018, official journal of the International Association for Hydrogen Energy, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:44 ; year:2019 ; number:57 ; day:15 ; month:11 ; pages:30039-30052 ; extent:14 |
| Links: |
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| DOI / URN: |
10.1016/j.ijhydene.2019.09.208 |
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ELV048387452 |
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| 520 | |a An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. | ||
| 520 | |a An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. | ||
| 650 | 7 | |a Porous media |2 Elsevier | |
| 650 | 7 | |a Filtration combustion |2 Elsevier | |
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| 650 | 7 | |a Reactor design |2 Elsevier | |
| 650 | 7 | |a Partial oxidation |2 Elsevier | |
| 700 | 1 | |a Polianczyk, E.V. |4 oth | |
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10.1016/j.ijhydene.2019.09.208 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000802.pica (DE-627)ELV048387452 (ELSEVIER)S0360-3199(19)33656-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Dorofeenko, S.O. verfasserin aut Enhancing efficiency of hydrocarbons to synthesis gas conversion in a counterflow moving bed filtration combustion reactor 2019transfer abstract 14 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. Porous media Elsevier Filtration combustion Elsevier Syngas production Elsevier Reactor design Elsevier Partial oxidation Elsevier Polianczyk, E.V. oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:44 year:2019 number:57 day:15 month:11 pages:30039-30052 extent:14 https://doi.org/10.1016/j.ijhydene.2019.09.208 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 44 2019 57 15 1115 30039-30052 14 |
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10.1016/j.ijhydene.2019.09.208 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000802.pica (DE-627)ELV048387452 (ELSEVIER)S0360-3199(19)33656-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Dorofeenko, S.O. verfasserin aut Enhancing efficiency of hydrocarbons to synthesis gas conversion in a counterflow moving bed filtration combustion reactor 2019transfer abstract 14 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. Porous media Elsevier Filtration combustion Elsevier Syngas production Elsevier Reactor design Elsevier Partial oxidation Elsevier Polianczyk, E.V. oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:44 year:2019 number:57 day:15 month:11 pages:30039-30052 extent:14 https://doi.org/10.1016/j.ijhydene.2019.09.208 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 44 2019 57 15 1115 30039-30052 14 |
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10.1016/j.ijhydene.2019.09.208 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000802.pica (DE-627)ELV048387452 (ELSEVIER)S0360-3199(19)33656-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Dorofeenko, S.O. verfasserin aut Enhancing efficiency of hydrocarbons to synthesis gas conversion in a counterflow moving bed filtration combustion reactor 2019transfer abstract 14 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. Porous media Elsevier Filtration combustion Elsevier Syngas production Elsevier Reactor design Elsevier Partial oxidation Elsevier Polianczyk, E.V. oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:44 year:2019 number:57 day:15 month:11 pages:30039-30052 extent:14 https://doi.org/10.1016/j.ijhydene.2019.09.208 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 44 2019 57 15 1115 30039-30052 14 |
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10.1016/j.ijhydene.2019.09.208 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000802.pica (DE-627)ELV048387452 (ELSEVIER)S0360-3199(19)33656-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Dorofeenko, S.O. verfasserin aut Enhancing efficiency of hydrocarbons to synthesis gas conversion in a counterflow moving bed filtration combustion reactor 2019transfer abstract 14 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. Porous media Elsevier Filtration combustion Elsevier Syngas production Elsevier Reactor design Elsevier Partial oxidation Elsevier Polianczyk, E.V. oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:44 year:2019 number:57 day:15 month:11 pages:30039-30052 extent:14 https://doi.org/10.1016/j.ijhydene.2019.09.208 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 44 2019 57 15 1115 30039-30052 14 |
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10.1016/j.ijhydene.2019.09.208 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000802.pica (DE-627)ELV048387452 (ELSEVIER)S0360-3199(19)33656-0 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Dorofeenko, S.O. verfasserin aut Enhancing efficiency of hydrocarbons to synthesis gas conversion in a counterflow moving bed filtration combustion reactor 2019transfer abstract 14 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. Porous media Elsevier Filtration combustion Elsevier Syngas production Elsevier Reactor design Elsevier Partial oxidation Elsevier Polianczyk, E.V. oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:44 year:2019 number:57 day:15 month:11 pages:30039-30052 extent:14 https://doi.org/10.1016/j.ijhydene.2019.09.208 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 44 2019 57 15 1115 30039-30052 14 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:44 year:2019 number:57 day:15 month:11 pages:30039-30052 extent:14 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:44 year:2019 number:57 day:15 month:11 pages:30039-30052 extent:14 |
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The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. 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Enhancing efficiency of hydrocarbons to synthesis gas conversion in a counterflow moving bed filtration combustion reactor |
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An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. |
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An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. |
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An improvement is considered for the partial oxidation conversion of hydrocarbon gases to synthesis gas in a continuous non-premixed filtration combustion reactor with inert solid granular material flowing countercurrently to the gas flow. The reactor is supplemented with an additional heat exchanger, wherein the second reactant gas is preheated prior to supply to the middle part of the reactor. The composition of the gaseous products self-consistent with the temperature of combustion are assessed using approximation of established thermodynamic equilibrium in the products. The parametric domain for major control parameters, namely oxygen-to-fuel supply ratio, granular solid flowrate, and steam supply rate providing highly efficient conversion is determined. Calculations for the POX conversion of methane and a model biogas composition (50% methane, 40% carbon dioxide, 10% nitrogen) with air and steam are provided as examples. The calculations show that the process gives a possibility to substantially improve energy efficiency and provides a flexibility to control hydrogen yield through steam supply. The process provides a high chemical efficiency of conversion even with air used as an oxidant for conversion of low-caloric gases. |
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