Two-dimensional nitrogen and oxygen Co-doping porous carbon nanosheets for high volumetric performance supercapacitors
Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation meth...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Liu, Ruonan [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020transfer abstract |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Impact of North Atlantic-East Asian teleconnections on extremely high January PM - Kim, Jeong-Hun ELSEVIER, 2021, the official journal of the International Zeolite Association, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:295 ; year:2020 ; day:15 ; month:03 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.micromeso.2019.109954 |
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| 520 | |a Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. | ||
| 520 | |a Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. | ||
| 650 | 7 | |a Carbon nanosheets |2 Elsevier | |
| 650 | 7 | |a Polyacrylamide |2 Elsevier | |
| 650 | 7 | |a Supercapacitor |2 Elsevier | |
| 650 | 7 | |a Graphene oxide |2 Elsevier | |
| 650 | 7 | |a Electrostatic self-assembly |2 Elsevier | |
| 700 | 1 | |a Wang, Yahui |4 oth | |
| 700 | 1 | |a Wu, Xiaoliang |4 oth | |
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10.1016/j.micromeso.2019.109954 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000887.pica (DE-627)ELV049181637 (ELSEVIER)S1387-1811(19)30813-3 DE-627 ger DE-627 rakwb eng 333.7 570 690 VZ BIODIV DE-30 fid 48.00 bkl Liu, Ruonan verfasserin aut Two-dimensional nitrogen and oxygen Co-doping porous carbon nanosheets for high volumetric performance supercapacitors 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Carbon nanosheets Elsevier Polyacrylamide Elsevier Supercapacitor Elsevier Graphene oxide Elsevier Electrostatic self-assembly Elsevier Wang, Yahui oth Wu, Xiaoliang oth Enthalten in Elsevier Kim, Jeong-Hun ELSEVIER Impact of North Atlantic-East Asian teleconnections on extremely high January PM 2021 the official journal of the International Zeolite Association Amsterdam [u.a.] (DE-627)ELV006778283 volume:295 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.micromeso.2019.109954 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 295 2020 15 0315 0 |
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10.1016/j.micromeso.2019.109954 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000887.pica (DE-627)ELV049181637 (ELSEVIER)S1387-1811(19)30813-3 DE-627 ger DE-627 rakwb eng 333.7 570 690 VZ BIODIV DE-30 fid 48.00 bkl Liu, Ruonan verfasserin aut Two-dimensional nitrogen and oxygen Co-doping porous carbon nanosheets for high volumetric performance supercapacitors 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Carbon nanosheets Elsevier Polyacrylamide Elsevier Supercapacitor Elsevier Graphene oxide Elsevier Electrostatic self-assembly Elsevier Wang, Yahui oth Wu, Xiaoliang oth Enthalten in Elsevier Kim, Jeong-Hun ELSEVIER Impact of North Atlantic-East Asian teleconnections on extremely high January PM 2021 the official journal of the International Zeolite Association Amsterdam [u.a.] (DE-627)ELV006778283 volume:295 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.micromeso.2019.109954 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 295 2020 15 0315 0 |
| allfields_unstemmed |
10.1016/j.micromeso.2019.109954 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000887.pica (DE-627)ELV049181637 (ELSEVIER)S1387-1811(19)30813-3 DE-627 ger DE-627 rakwb eng 333.7 570 690 VZ BIODIV DE-30 fid 48.00 bkl Liu, Ruonan verfasserin aut Two-dimensional nitrogen and oxygen Co-doping porous carbon nanosheets for high volumetric performance supercapacitors 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Carbon nanosheets Elsevier Polyacrylamide Elsevier Supercapacitor Elsevier Graphene oxide Elsevier Electrostatic self-assembly Elsevier Wang, Yahui oth Wu, Xiaoliang oth Enthalten in Elsevier Kim, Jeong-Hun ELSEVIER Impact of North Atlantic-East Asian teleconnections on extremely high January PM 2021 the official journal of the International Zeolite Association Amsterdam [u.a.] (DE-627)ELV006778283 volume:295 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.micromeso.2019.109954 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 295 2020 15 0315 0 |
| allfieldsGer |
10.1016/j.micromeso.2019.109954 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000887.pica (DE-627)ELV049181637 (ELSEVIER)S1387-1811(19)30813-3 DE-627 ger DE-627 rakwb eng 333.7 570 690 VZ BIODIV DE-30 fid 48.00 bkl Liu, Ruonan verfasserin aut Two-dimensional nitrogen and oxygen Co-doping porous carbon nanosheets for high volumetric performance supercapacitors 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Carbon nanosheets Elsevier Polyacrylamide Elsevier Supercapacitor Elsevier Graphene oxide Elsevier Electrostatic self-assembly Elsevier Wang, Yahui oth Wu, Xiaoliang oth Enthalten in Elsevier Kim, Jeong-Hun ELSEVIER Impact of North Atlantic-East Asian teleconnections on extremely high January PM 2021 the official journal of the International Zeolite Association Amsterdam [u.a.] (DE-627)ELV006778283 volume:295 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.micromeso.2019.109954 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 295 2020 15 0315 0 |
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10.1016/j.micromeso.2019.109954 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000887.pica (DE-627)ELV049181637 (ELSEVIER)S1387-1811(19)30813-3 DE-627 ger DE-627 rakwb eng 333.7 570 690 VZ BIODIV DE-30 fid 48.00 bkl Liu, Ruonan verfasserin aut Two-dimensional nitrogen and oxygen Co-doping porous carbon nanosheets for high volumetric performance supercapacitors 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. Carbon nanosheets Elsevier Polyacrylamide Elsevier Supercapacitor Elsevier Graphene oxide Elsevier Electrostatic self-assembly Elsevier Wang, Yahui oth Wu, Xiaoliang oth Enthalten in Elsevier Kim, Jeong-Hun ELSEVIER Impact of North Atlantic-East Asian teleconnections on extremely high January PM 2021 the official journal of the International Zeolite Association Amsterdam [u.a.] (DE-627)ELV006778283 volume:295 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.micromeso.2019.109954 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR 48.00 Land- und Forstwirtschaft: Allgemeines VZ AR 295 2020 15 0315 0 |
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two-dimensional nitrogen and oxygen co-doping porous carbon nanosheets for high volumetric performance supercapacitors |
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Two-dimensional nitrogen and oxygen Co-doping porous carbon nanosheets for high volumetric performance supercapacitors |
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Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. |
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Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. |
| abstract_unstemmed |
Two-dimensional (2D) porous carbon nanosheets possess large open flat layer with high surface area, short ion diffusion route and small diffusion resistance have attracted greatly attention as electrode materials for supercapacitors. However, developing a simple and widely available preparation method remains a major challenge. Herein, we demonstrate a new, widely available way to rationally design the nitrogen and oxygen co-doping porous carbon nanosheets (PCN) utilizing graphene oxide as template by an electrostatic self-assembly process with cationic polyacrylamide and subsequent KOH activation. Benefiting from the open and accessible surface, short ion diffusion route and rich nitrogen and oxygen functional groups, the optimized PCN-3 electrode shows a high volumetric specific capacitance of 325.7 F cm−3 at 0.5 A g −1 with a high capacitance retention of 66% at 50 A g−1 (215.3 F cm−3). Moreover, the PCN-3//PCN-3 symmetric supercapacitor shows a high volumetric energy density of 22.1 Wh L−1 and outstanding cycling stability in 1 M Na2SO4 aqueous elec1trolyte. Consequently, the work highlights a convenient and widely available preparation way to prepare heteroatom doped porous carbon nanosheets for supercapacitors. |
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