Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene
Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-...
Ausführliche Beschreibung
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| Autor*in: |
Kwon, Hyeok-jin [verfasserIn] |
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E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020transfer abstract |
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| Übergeordnetes Werk: |
Enthalten in: Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands - saleh, Dalia I ELSEVIER, 2022, physics, materials and applications, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:77 ; year:2020 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.orgel.2019.105485 |
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| 520 | |a Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. | ||
| 520 | |a Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. | ||
| 650 | 7 | |a Cytop |2 Elsevier | |
| 650 | 7 | |a Organic field-effect transistor |2 Elsevier | |
| 650 | 7 | |a Hydrophobicity |2 Elsevier | |
| 650 | 7 | |a Interfacial properties |2 Elsevier | |
| 650 | 7 | |a Dielectric |2 Elsevier | |
| 650 | 7 | |a Polystyrene |2 Elsevier | |
| 700 | 1 | |a Gao, Chun Yan |4 oth | |
| 700 | 1 | |a Tang, Xiaowu |4 oth | |
| 700 | 1 | |a Hong, Jisu |4 oth | |
| 700 | 1 | |a Park, Chan Eon |4 oth | |
| 700 | 1 | |a Kong, Hoyoul |4 oth | |
| 700 | 1 | |a Kim, Se Hyun |4 oth | |
| 700 | 1 | |a Yang, Hoichang |4 oth | |
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10.1016/j.orgel.2019.105485 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000941.pica (DE-627)ELV049553038 (ELSEVIER)S1566-1199(19)30512-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Kwon, Hyeok-jin verfasserin aut Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Cytop Elsevier Organic field-effect transistor Elsevier Hydrophobicity Elsevier Interfacial properties Elsevier Dielectric Elsevier Polystyrene Elsevier Gao, Chun Yan oth Tang, Xiaowu oth Hong, Jisu oth Park, Chan Eon oth Kong, Hoyoul oth Kim, Se Hyun oth Yang, Hoichang oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:77 year:2020 pages:0 https://doi.org/10.1016/j.orgel.2019.105485 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 77 2020 0 |
| spelling |
10.1016/j.orgel.2019.105485 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000941.pica (DE-627)ELV049553038 (ELSEVIER)S1566-1199(19)30512-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Kwon, Hyeok-jin verfasserin aut Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Cytop Elsevier Organic field-effect transistor Elsevier Hydrophobicity Elsevier Interfacial properties Elsevier Dielectric Elsevier Polystyrene Elsevier Gao, Chun Yan oth Tang, Xiaowu oth Hong, Jisu oth Park, Chan Eon oth Kong, Hoyoul oth Kim, Se Hyun oth Yang, Hoichang oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:77 year:2020 pages:0 https://doi.org/10.1016/j.orgel.2019.105485 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 77 2020 0 |
| allfields_unstemmed |
10.1016/j.orgel.2019.105485 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000941.pica (DE-627)ELV049553038 (ELSEVIER)S1566-1199(19)30512-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Kwon, Hyeok-jin verfasserin aut Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Cytop Elsevier Organic field-effect transistor Elsevier Hydrophobicity Elsevier Interfacial properties Elsevier Dielectric Elsevier Polystyrene Elsevier Gao, Chun Yan oth Tang, Xiaowu oth Hong, Jisu oth Park, Chan Eon oth Kong, Hoyoul oth Kim, Se Hyun oth Yang, Hoichang oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:77 year:2020 pages:0 https://doi.org/10.1016/j.orgel.2019.105485 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 77 2020 0 |
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10.1016/j.orgel.2019.105485 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000941.pica (DE-627)ELV049553038 (ELSEVIER)S1566-1199(19)30512-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Kwon, Hyeok-jin verfasserin aut Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Cytop Elsevier Organic field-effect transistor Elsevier Hydrophobicity Elsevier Interfacial properties Elsevier Dielectric Elsevier Polystyrene Elsevier Gao, Chun Yan oth Tang, Xiaowu oth Hong, Jisu oth Park, Chan Eon oth Kong, Hoyoul oth Kim, Se Hyun oth Yang, Hoichang oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:77 year:2020 pages:0 https://doi.org/10.1016/j.orgel.2019.105485 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 77 2020 0 |
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10.1016/j.orgel.2019.105485 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000941.pica (DE-627)ELV049553038 (ELSEVIER)S1566-1199(19)30512-9 DE-627 ger DE-627 rakwb eng 540 VZ 35.00 bkl Kwon, Hyeok-jin verfasserin aut Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. Cytop Elsevier Organic field-effect transistor Elsevier Hydrophobicity Elsevier Interfacial properties Elsevier Dielectric Elsevier Polystyrene Elsevier Gao, Chun Yan oth Tang, Xiaowu oth Hong, Jisu oth Park, Chan Eon oth Kong, Hoyoul oth Kim, Se Hyun oth Yang, Hoichang oth Enthalten in Elsevier Science saleh, Dalia I ELSEVIER Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands 2022 physics, materials and applications Amsterdam [u.a.] (DE-627)ELV007843747 volume:77 year:2020 pages:0 https://doi.org/10.1016/j.orgel.2019.105485 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 35.00 Chemie: Allgemeines VZ AR 77 2020 0 |
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Enthalten in Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands Amsterdam [u.a.] volume:77 year:2020 pages:0 |
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Enthalten in Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands Amsterdam [u.a.] volume:77 year:2020 pages:0 |
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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
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However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. 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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
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Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene |
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Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene |
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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
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Ultrasound-assisted synthesis and biological activity of nanosized supramolecular coordination polymers of silver(I) with chloride, thiocyanate, and 4,4′-bipyridine ligands |
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comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: cytop vs. polystyrene |
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Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene |
| abstract |
Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. |
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Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. |
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Organic field-effect transistors (OFETs) have been fabricated by deposition of an organic semiconductor on inorganic dielectric layers like SiO2. However, inorganic oxide dielectrics have hydrophilic surface properties, which interrupts the growth of organic semiconductors with highly aligned and π-extended domains, and provide many absorbing sites for moisture that work as trap sites for charge carriers. To overcome this problem, a proper surface-treatment method is required to improve the morphology of organic semiconductors. In this study, we treat SiO2 dielectrics with polystyrene (PS) and Cytop (a fluorinated cross-linkable polymer) to tune the surface properties when fabricating pentacene-based bottom-gate top-contact OFETs, and analyzed the influence of surface functionalization on the growth of the pentacene crystals under different deposition conditions and electrical device characteristics. By comparing the morphological features of pentacene with the device characteristics, the effect of hydrophobicity on the morphology of the pentacene polymorph, strongly related to the charge-transport mechanism, could be described. |
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Comparison of semiconductor growth and charge transport on hydrophobic polymer dielectrics of organic field-effect transistors: Cytop vs. polystyrene |
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Gao, Chun Yan Tang, Xiaowu Hong, Jisu Park, Chan Eon Kong, Hoyoul Kim, Se Hyun Yang, Hoichang |
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