Development of a fluorescent chemosensor for chloride ion detection in sweat using Ag+-benzimidazole complexes
The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was dev...
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Gespeichert in:
| Autor*in: |
Kim, Jaewon [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020transfer abstract |
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| Übergeordnetes Werk: |
Enthalten in: A multiscale analysis for free vibration of fuzzy fiber-reinforced nanocomposite conical shells - Haghgoo, M. ELSEVIER, 2020, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:177 ; year:2020 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.dyepig.2020.108291 |
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| 245 | 1 | 0 | |a Development of a fluorescent chemosensor for chloride ion detection in sweat using Ag+-benzimidazole complexes |
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| 520 | |a The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. | ||
| 520 | |a The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. | ||
| 650 | 7 | |a Metal-ligand exchange |2 Elsevier | |
| 650 | 7 | |a Sweat test |2 Elsevier | |
| 650 | 7 | |a Fluorescent chemosensor |2 Elsevier | |
| 650 | 7 | |a Cystic fibrosis |2 Elsevier | |
| 650 | 7 | |a Ligand displacement |2 Elsevier | |
| 650 | 7 | |a Chloride ion |2 Elsevier | |
| 700 | 1 | |a Lee, Suji |4 oth | |
| 700 | 1 | |a Kim, Sudeok |4 oth | |
| 700 | 1 | |a Jung, Minhyuk |4 oth | |
| 700 | 1 | |a Lee, Hohjai |4 oth | |
| 700 | 1 | |a Han, Min Su |4 oth | |
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10.1016/j.dyepig.2020.108291 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000947.pica (DE-627)ELV049754009 (ELSEVIER)S0143-7208(19)32715-9 DE-627 ger DE-627 rakwb eng 690 VZ 50.31 bkl 56.11 bkl Kim, Jaewon verfasserin aut Development of a fluorescent chemosensor for chloride ion detection in sweat using Ag+-benzimidazole complexes 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. Metal-ligand exchange Elsevier Sweat test Elsevier Fluorescent chemosensor Elsevier Cystic fibrosis Elsevier Ligand displacement Elsevier Chloride ion Elsevier Lee, Suji oth Kim, Sudeok oth Jung, Minhyuk oth Lee, Hohjai oth Han, Min Su oth Enthalten in Elsevier Science Haghgoo, M. ELSEVIER A multiscale analysis for free vibration of fuzzy fiber-reinforced nanocomposite conical shells 2020 Amsterdam [u.a.] (DE-627)ELV004269640 volume:177 year:2020 pages:0 https://doi.org/10.1016/j.dyepig.2020.108291 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.31 Technische Mechanik VZ 56.11 Baukonstruktion VZ AR 177 2020 0 |
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10.1016/j.dyepig.2020.108291 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000947.pica (DE-627)ELV049754009 (ELSEVIER)S0143-7208(19)32715-9 DE-627 ger DE-627 rakwb eng 690 VZ 50.31 bkl 56.11 bkl Kim, Jaewon verfasserin aut Development of a fluorescent chemosensor for chloride ion detection in sweat using Ag+-benzimidazole complexes 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. Metal-ligand exchange Elsevier Sweat test Elsevier Fluorescent chemosensor Elsevier Cystic fibrosis Elsevier Ligand displacement Elsevier Chloride ion Elsevier Lee, Suji oth Kim, Sudeok oth Jung, Minhyuk oth Lee, Hohjai oth Han, Min Su oth Enthalten in Elsevier Science Haghgoo, M. ELSEVIER A multiscale analysis for free vibration of fuzzy fiber-reinforced nanocomposite conical shells 2020 Amsterdam [u.a.] (DE-627)ELV004269640 volume:177 year:2020 pages:0 https://doi.org/10.1016/j.dyepig.2020.108291 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.31 Technische Mechanik VZ 56.11 Baukonstruktion VZ AR 177 2020 0 |
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10.1016/j.dyepig.2020.108291 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000947.pica (DE-627)ELV049754009 (ELSEVIER)S0143-7208(19)32715-9 DE-627 ger DE-627 rakwb eng 690 VZ 50.31 bkl 56.11 bkl Kim, Jaewon verfasserin aut Development of a fluorescent chemosensor for chloride ion detection in sweat using Ag+-benzimidazole complexes 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. Metal-ligand exchange Elsevier Sweat test Elsevier Fluorescent chemosensor Elsevier Cystic fibrosis Elsevier Ligand displacement Elsevier Chloride ion Elsevier Lee, Suji oth Kim, Sudeok oth Jung, Minhyuk oth Lee, Hohjai oth Han, Min Su oth Enthalten in Elsevier Science Haghgoo, M. ELSEVIER A multiscale analysis for free vibration of fuzzy fiber-reinforced nanocomposite conical shells 2020 Amsterdam [u.a.] (DE-627)ELV004269640 volume:177 year:2020 pages:0 https://doi.org/10.1016/j.dyepig.2020.108291 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.31 Technische Mechanik VZ 56.11 Baukonstruktion VZ AR 177 2020 0 |
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10.1016/j.dyepig.2020.108291 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000947.pica (DE-627)ELV049754009 (ELSEVIER)S0143-7208(19)32715-9 DE-627 ger DE-627 rakwb eng 690 VZ 50.31 bkl 56.11 bkl Kim, Jaewon verfasserin aut Development of a fluorescent chemosensor for chloride ion detection in sweat using Ag+-benzimidazole complexes 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. Metal-ligand exchange Elsevier Sweat test Elsevier Fluorescent chemosensor Elsevier Cystic fibrosis Elsevier Ligand displacement Elsevier Chloride ion Elsevier Lee, Suji oth Kim, Sudeok oth Jung, Minhyuk oth Lee, Hohjai oth Han, Min Su oth Enthalten in Elsevier Science Haghgoo, M. ELSEVIER A multiscale analysis for free vibration of fuzzy fiber-reinforced nanocomposite conical shells 2020 Amsterdam [u.a.] (DE-627)ELV004269640 volume:177 year:2020 pages:0 https://doi.org/10.1016/j.dyepig.2020.108291 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.31 Technische Mechanik VZ 56.11 Baukonstruktion VZ AR 177 2020 0 |
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10.1016/j.dyepig.2020.108291 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000947.pica (DE-627)ELV049754009 (ELSEVIER)S0143-7208(19)32715-9 DE-627 ger DE-627 rakwb eng 690 VZ 50.31 bkl 56.11 bkl Kim, Jaewon verfasserin aut Development of a fluorescent chemosensor for chloride ion detection in sweat using Ag+-benzimidazole complexes 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. Metal-ligand exchange Elsevier Sweat test Elsevier Fluorescent chemosensor Elsevier Cystic fibrosis Elsevier Ligand displacement Elsevier Chloride ion Elsevier Lee, Suji oth Kim, Sudeok oth Jung, Minhyuk oth Lee, Hohjai oth Han, Min Su oth Enthalten in Elsevier Science Haghgoo, M. ELSEVIER A multiscale analysis for free vibration of fuzzy fiber-reinforced nanocomposite conical shells 2020 Amsterdam [u.a.] (DE-627)ELV004269640 volume:177 year:2020 pages:0 https://doi.org/10.1016/j.dyepig.2020.108291 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 50.31 Technische Mechanik VZ 56.11 Baukonstruktion VZ AR 177 2020 0 |
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Enthalten in A multiscale analysis for free vibration of fuzzy fiber-reinforced nanocomposite conical shells Amsterdam [u.a.] volume:177 year:2020 pages:0 |
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Enthalten in A multiscale analysis for free vibration of fuzzy fiber-reinforced nanocomposite conical shells Amsterdam [u.a.] volume:177 year:2020 pages:0 |
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The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. 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Development of a fluorescent chemosensor for chloride ion detection in sweat using Ag+-benzimidazole complexes |
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The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. |
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The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. |
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The level of chloride ions (Cl⁻) in sweat is a recognized biomarker for the genetic disorder cystic fibrosis (CF). The accurate quantitation of chloride ions in sweat is therefore a vital diagnostic tool for this life-threatening disease. In this work, a fluorescent, chloride ion chemosensor was developed by exploiting the strong interaction between silver (Ag+) and chloride ions. Using the concept of ligand displacement, six Ag+-benzimidazole complexes were prepared as candidate chloride ion chemosensors. The Ag+-2-(Furan-2-yl)-1H-benzo[d]imidazole (Ag+-FBI) complex was identified as the optimal sensor owing to its Ag+-FBI high sensitivity (limit of detection = 19 μM), short response time (<3 min), and remarkable fluorescence turn-on response across a broad pH range (pH 6–9). The Ag+-FBI complex exhibited high selectivity for Cl⁻ ions and was successfully used to quantify chloride ions in artificial sweat samples containing multiple ions and other biological constituents. This unique, simple, and effective probe thus shows great potential for clinical diagnostic applications. |
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