Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth
The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysi...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Lin, Chong [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020transfer abstract |
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| Übergeordnetes Werk: |
Enthalten in: Enhancement with physicochemical and biological treatments in the removal of pharmaceutically active compounds during sewage sludge anaerobic digestion processes - Zhou, Haidong ELSEVIER, 2017, an international journal devoted to all aspects of electrode kinetics, interfacial structure, properties of electrolytes, colloid and biological electrochemistry, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:861 ; year:2020 ; day:15 ; month:03 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.jelechem.2020.113946 |
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| 245 | 1 | 0 | |a Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth |
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| 520 | |a The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. | ||
| 520 | |a The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. | ||
| 700 | 1 | |a Li, Huiqin |4 oth | |
| 700 | 1 | |a Zhang, Panjing |4 oth | |
| 700 | 1 | |a Deng, Cui |4 oth | |
| 700 | 1 | |a Meng, Liqing |4 oth | |
| 700 | 1 | |a Zhou, Qiaoli |4 oth | |
| 700 | 1 | |a Wang, Shengying |4 oth | |
| 700 | 1 | |a Wu, Jiaxin |4 oth | |
| 700 | 1 | |a Liu, Chengzhi |4 oth | |
| 700 | 1 | |a Tian, Jingyang |4 oth | |
| 700 | 1 | |a Qian, Yong |4 oth | |
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10.1016/j.jelechem.2020.113946 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000978.pica (DE-627)ELV049795287 (ELSEVIER)S1572-6657(20)30129-6 DE-627 ger DE-627 rakwb eng 660 VZ 660 VZ 530 600 670 VZ 51.00 bkl Lin, Chong verfasserin aut Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. Li, Huiqin oth Zhang, Panjing oth Deng, Cui oth Meng, Liqing oth Zhou, Qiaoli oth Wang, Shengying oth Wu, Jiaxin oth Liu, Chengzhi oth Tian, Jingyang oth Qian, Yong oth Enthalten in Elsevier Zhou, Haidong ELSEVIER Enhancement with physicochemical and biological treatments in the removal of pharmaceutically active compounds during sewage sludge anaerobic digestion processes 2017 an international journal devoted to all aspects of electrode kinetics, interfacial structure, properties of electrolytes, colloid and biological electrochemistry New York, NY [u.a.] (DE-627)ELV014792559 volume:861 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.jelechem.2020.113946 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_22 GBV_ILN_40 GBV_ILN_105 51.00 Werkstoffkunde: Allgemeines VZ AR 861 2020 15 0315 0 |
| spelling |
10.1016/j.jelechem.2020.113946 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000978.pica (DE-627)ELV049795287 (ELSEVIER)S1572-6657(20)30129-6 DE-627 ger DE-627 rakwb eng 660 VZ 660 VZ 530 600 670 VZ 51.00 bkl Lin, Chong verfasserin aut Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. Li, Huiqin oth Zhang, Panjing oth Deng, Cui oth Meng, Liqing oth Zhou, Qiaoli oth Wang, Shengying oth Wu, Jiaxin oth Liu, Chengzhi oth Tian, Jingyang oth Qian, Yong oth Enthalten in Elsevier Zhou, Haidong ELSEVIER Enhancement with physicochemical and biological treatments in the removal of pharmaceutically active compounds during sewage sludge anaerobic digestion processes 2017 an international journal devoted to all aspects of electrode kinetics, interfacial structure, properties of electrolytes, colloid and biological electrochemistry New York, NY [u.a.] (DE-627)ELV014792559 volume:861 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.jelechem.2020.113946 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_22 GBV_ILN_40 GBV_ILN_105 51.00 Werkstoffkunde: Allgemeines VZ AR 861 2020 15 0315 0 |
| allfields_unstemmed |
10.1016/j.jelechem.2020.113946 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000978.pica (DE-627)ELV049795287 (ELSEVIER)S1572-6657(20)30129-6 DE-627 ger DE-627 rakwb eng 660 VZ 660 VZ 530 600 670 VZ 51.00 bkl Lin, Chong verfasserin aut Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. Li, Huiqin oth Zhang, Panjing oth Deng, Cui oth Meng, Liqing oth Zhou, Qiaoli oth Wang, Shengying oth Wu, Jiaxin oth Liu, Chengzhi oth Tian, Jingyang oth Qian, Yong oth Enthalten in Elsevier Zhou, Haidong ELSEVIER Enhancement with physicochemical and biological treatments in the removal of pharmaceutically active compounds during sewage sludge anaerobic digestion processes 2017 an international journal devoted to all aspects of electrode kinetics, interfacial structure, properties of electrolytes, colloid and biological electrochemistry New York, NY [u.a.] (DE-627)ELV014792559 volume:861 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.jelechem.2020.113946 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_22 GBV_ILN_40 GBV_ILN_105 51.00 Werkstoffkunde: Allgemeines VZ AR 861 2020 15 0315 0 |
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10.1016/j.jelechem.2020.113946 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000978.pica (DE-627)ELV049795287 (ELSEVIER)S1572-6657(20)30129-6 DE-627 ger DE-627 rakwb eng 660 VZ 660 VZ 530 600 670 VZ 51.00 bkl Lin, Chong verfasserin aut Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. Li, Huiqin oth Zhang, Panjing oth Deng, Cui oth Meng, Liqing oth Zhou, Qiaoli oth Wang, Shengying oth Wu, Jiaxin oth Liu, Chengzhi oth Tian, Jingyang oth Qian, Yong oth Enthalten in Elsevier Zhou, Haidong ELSEVIER Enhancement with physicochemical and biological treatments in the removal of pharmaceutically active compounds during sewage sludge anaerobic digestion processes 2017 an international journal devoted to all aspects of electrode kinetics, interfacial structure, properties of electrolytes, colloid and biological electrochemistry New York, NY [u.a.] (DE-627)ELV014792559 volume:861 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.jelechem.2020.113946 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_22 GBV_ILN_40 GBV_ILN_105 51.00 Werkstoffkunde: Allgemeines VZ AR 861 2020 15 0315 0 |
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10.1016/j.jelechem.2020.113946 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000978.pica (DE-627)ELV049795287 (ELSEVIER)S1572-6657(20)30129-6 DE-627 ger DE-627 rakwb eng 660 VZ 660 VZ 530 600 670 VZ 51.00 bkl Lin, Chong verfasserin aut Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. Li, Huiqin oth Zhang, Panjing oth Deng, Cui oth Meng, Liqing oth Zhou, Qiaoli oth Wang, Shengying oth Wu, Jiaxin oth Liu, Chengzhi oth Tian, Jingyang oth Qian, Yong oth Enthalten in Elsevier Zhou, Haidong ELSEVIER Enhancement with physicochemical and biological treatments in the removal of pharmaceutically active compounds during sewage sludge anaerobic digestion processes 2017 an international journal devoted to all aspects of electrode kinetics, interfacial structure, properties of electrolytes, colloid and biological electrochemistry New York, NY [u.a.] (DE-627)ELV014792559 volume:861 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.jelechem.2020.113946 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_22 GBV_ILN_40 GBV_ILN_105 51.00 Werkstoffkunde: Allgemeines VZ AR 861 2020 15 0315 0 |
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Enthalten in Enhancement with physicochemical and biological treatments in the removal of pharmaceutically active compounds during sewage sludge anaerobic digestion processes New York, NY [u.a.] volume:861 year:2020 day:15 month:03 pages:0 |
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However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. 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boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth |
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Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth |
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The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. |
| abstractGer |
The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. |
| abstract_unstemmed |
The pursuit of low cell voltage for water splitting is urgent for the clean and sustainable energy. However, the cell voltage is limited by the anodic oxygen evolution reaction (OER), requiring a higher overpotential than cathodic hydrogen evolution reaction (HER). Herein, to boost water electrolysis, we replace the anodic OER with glucose oxidation reaction (GOR) over engineered ultra-thin cobalt nickel hydroxide nanosheet on carbon cloth, in which can synergistically improve its numbers of active sites, conductivity, intrinsic activity and stability with the Co doped α-Ni(OH)2. When it couples with Pt cathode, the resulting cell voltage to drive water splitting at the current density of 100 mA cm−2 with the assistance of glucose is as low as 1.56 V. While without the glucose in the electrolyte, the potential reaches as high as 1.75 V. Therefore, replacing OER with the GOR can reduce the potential of water electrolysis. This work is contributed to the development the other highly active and robust electrocatalysts in water electrolysis with the assistance of glucose or similar organic molecular. |
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Boosting water electrolysis with anodic glucose oxidation reaction over engineered cobalt nickel hydroxide nanosheet on carbon cloth |
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Li, Huiqin Zhang, Panjing Deng, Cui Meng, Liqing Zhou, Qiaoli Wang, Shengying Wu, Jiaxin Liu, Chengzhi Tian, Jingyang Qian, Yong |
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Li, Huiqin Zhang, Panjing Deng, Cui Meng, Liqing Zhou, Qiaoli Wang, Shengying Wu, Jiaxin Liu, Chengzhi Tian, Jingyang Qian, Yong |
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