Effects of cold SF6 plasma treatment on a-C:H, polypropylene and polystyrene
The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all...
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Gespeichert in:
| Autor*in: |
Amorim, Milena Kowalczuk Manosso [verfasserIn] |
|---|
| Format: |
E-Artikel |
|---|---|
| Sprache: |
Englisch |
| Erschienen: |
2020transfer abstract |
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| Übergeordnetes Werk: |
Enthalten in: A high efficiency solar steam generation system with using residual heat to enhance steam escape - Bai, Binglin ELSEVIER, 2020, Amsterdam [u.a.] |
|---|---|
| Übergeordnetes Werk: |
volume:385 ; year:2020 ; day:15 ; month:03 ; pages:0 |
| Links: |
|---|
| DOI / URN: |
10.1016/j.surfcoat.2020.125398 |
|---|
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ELV049894544 |
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| 520 | |a The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. | ||
| 520 | |a The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. | ||
| 700 | 1 | |a Rangel, Elidiane Cipriano |4 oth | |
| 700 | 1 | |a Landers, Richard |4 oth | |
| 700 | 1 | |a Durrant, Steven F. |4 oth | |
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10.1016/j.surfcoat.2020.125398 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000963.pica (DE-627)ELV049894544 (ELSEVIER)S0257-8972(20)30067-0 DE-627 ger DE-627 rakwb eng 570 690 VZ 58.51 bkl Amorim, Milena Kowalczuk Manosso verfasserin aut Effects of cold SF6 plasma treatment on a-C:H, polypropylene and polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. Rangel, Elidiane Cipriano oth Landers, Richard oth Durrant, Steven F. oth Enthalten in Elsevier Science Bai, Binglin ELSEVIER A high efficiency solar steam generation system with using residual heat to enhance steam escape 2020 Amsterdam [u.a.] (DE-627)ELV004415906 volume:385 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.surfcoat.2020.125398 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 58.51 Abwassertechnik Wasseraufbereitung VZ AR 385 2020 15 0315 0 |
| spelling |
10.1016/j.surfcoat.2020.125398 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000963.pica (DE-627)ELV049894544 (ELSEVIER)S0257-8972(20)30067-0 DE-627 ger DE-627 rakwb eng 570 690 VZ 58.51 bkl Amorim, Milena Kowalczuk Manosso verfasserin aut Effects of cold SF6 plasma treatment on a-C:H, polypropylene and polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. Rangel, Elidiane Cipriano oth Landers, Richard oth Durrant, Steven F. oth Enthalten in Elsevier Science Bai, Binglin ELSEVIER A high efficiency solar steam generation system with using residual heat to enhance steam escape 2020 Amsterdam [u.a.] (DE-627)ELV004415906 volume:385 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.surfcoat.2020.125398 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 58.51 Abwassertechnik Wasseraufbereitung VZ AR 385 2020 15 0315 0 |
| allfields_unstemmed |
10.1016/j.surfcoat.2020.125398 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000963.pica (DE-627)ELV049894544 (ELSEVIER)S0257-8972(20)30067-0 DE-627 ger DE-627 rakwb eng 570 690 VZ 58.51 bkl Amorim, Milena Kowalczuk Manosso verfasserin aut Effects of cold SF6 plasma treatment on a-C:H, polypropylene and polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. Rangel, Elidiane Cipriano oth Landers, Richard oth Durrant, Steven F. oth Enthalten in Elsevier Science Bai, Binglin ELSEVIER A high efficiency solar steam generation system with using residual heat to enhance steam escape 2020 Amsterdam [u.a.] (DE-627)ELV004415906 volume:385 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.surfcoat.2020.125398 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 58.51 Abwassertechnik Wasseraufbereitung VZ AR 385 2020 15 0315 0 |
| allfieldsGer |
10.1016/j.surfcoat.2020.125398 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000963.pica (DE-627)ELV049894544 (ELSEVIER)S0257-8972(20)30067-0 DE-627 ger DE-627 rakwb eng 570 690 VZ 58.51 bkl Amorim, Milena Kowalczuk Manosso verfasserin aut Effects of cold SF6 plasma treatment on a-C:H, polypropylene and polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. Rangel, Elidiane Cipriano oth Landers, Richard oth Durrant, Steven F. oth Enthalten in Elsevier Science Bai, Binglin ELSEVIER A high efficiency solar steam generation system with using residual heat to enhance steam escape 2020 Amsterdam [u.a.] (DE-627)ELV004415906 volume:385 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.surfcoat.2020.125398 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 58.51 Abwassertechnik Wasseraufbereitung VZ AR 385 2020 15 0315 0 |
| allfieldsSound |
10.1016/j.surfcoat.2020.125398 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000000963.pica (DE-627)ELV049894544 (ELSEVIER)S0257-8972(20)30067-0 DE-627 ger DE-627 rakwb eng 570 690 VZ 58.51 bkl Amorim, Milena Kowalczuk Manosso verfasserin aut Effects of cold SF6 plasma treatment on a-C:H, polypropylene and polystyrene 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. Rangel, Elidiane Cipriano oth Landers, Richard oth Durrant, Steven F. oth Enthalten in Elsevier Science Bai, Binglin ELSEVIER A high efficiency solar steam generation system with using residual heat to enhance steam escape 2020 Amsterdam [u.a.] (DE-627)ELV004415906 volume:385 year:2020 day:15 month:03 pages:0 https://doi.org/10.1016/j.surfcoat.2020.125398 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 58.51 Abwassertechnik Wasseraufbereitung VZ AR 385 2020 15 0315 0 |
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Enthalten in A high efficiency solar steam generation system with using residual heat to enhance steam escape Amsterdam [u.a.] volume:385 year:2020 day:15 month:03 pages:0 |
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Amorim, Milena Kowalczuk Manosso @@aut@@ Rangel, Elidiane Cipriano @@oth@@ Landers, Richard @@oth@@ Durrant, Steven F. @@oth@@ |
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An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. 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effects of cold sf6 plasma treatment on a-c:h, polypropylene and polystyrene |
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Effects of cold SF6 plasma treatment on a-C:H, polypropylene and polystyrene |
| abstract |
The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. |
| abstractGer |
The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. |
| abstract_unstemmed |
The effects of cold SF6 plasma treatment on amorphous hydrogenated carbon (FA), polypropylene (PP) and polystyrene (PS) were investigated as functions of gas pressure and applied power. An anticipated increase in hydrophobicity was confirmed by the greater water contact angles, θ, observed after all the treatments. Under the best conditions θ was increased by 50.8°, 57.2° and 21°, respectively. A rise and fall in θ was observed as the pressure of SF6 was increased, this trend being most consistent for FA. Although the plasma treatments caused some changes in surface roughness, measured using profilometry, there were no clear correlations between this parameter and θ. As revealed by Energy Dispersive X-ray Spectroscopy (EDS) and X-ray Photoelectron Spectroscopy (XPS), the treated surfaces were fluorinated. As the degree of fluorination under optimal conditions was 2.2 at.%, 10.4 at.% and 36.3 at.% for the FA, PP and PS, respectively, this factor was not alone responsible for the observed increases in θ. Sulfur was attached to the surface of all the treated samples. The relative surface carbon content was reduced by the treatments. The main causes of the changes in θ upon treatment were the induced compositional and structural changes. Ageing for ten days caused a typical decrease in θ of ~10°, probably caused by rotation of hydrophobic surface groups into the surface. |
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Effects of cold SF6 plasma treatment on a-C:H, polypropylene and polystyrene |
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