High crystallinity and photovoltaic performance of CsPbI3 film enabled by secondary dimension
The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Wu, Min [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020transfer abstract |
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| Umfang: |
6 |
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| Übergeordnetes Werk: |
Enthalten in: Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation - Praveen Kumar, D. ELSEVIER, 2015transfer abstract, Amsterdam [u.a.] |
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| Übergeordnetes Werk: |
volume:48 ; year:2020 ; pages:181-186 ; extent:6 |
| Links: |
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| DOI / URN: |
10.1016/j.jechem.2020.01.009 |
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ELV050384805 |
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| 520 | |a The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. | ||
| 520 | |a The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. | ||
| 700 | 1 | |a Yan, Keyou |4 oth | |
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10.1016/j.jechem.2020.01.009 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001145.pica (DE-627)ELV050384805 (ELSEVIER)S2095-4956(20)30024-3 DE-627 ger DE-627 rakwb eng 530 VZ 620 VZ 690 VZ 56.03 bkl Wu, Min verfasserin aut High crystallinity and photovoltaic performance of CsPbI3 film enabled by secondary dimension 2020transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. Yan, Keyou oth Wang, Yong oth Kang, Xiongwu oth Enthalten in Elsevier Praveen Kumar, D. ELSEVIER Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation 2015transfer abstract Amsterdam [u.a.] (DE-627)ELV01862751X volume:48 year:2020 pages:181-186 extent:6 https://doi.org/10.1016/j.jechem.2020.01.009 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_21 GBV_ILN_40 56.03 Methoden im Bauingenieurwesen VZ AR 48 2020 181-186 6 |
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10.1016/j.jechem.2020.01.009 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001145.pica (DE-627)ELV050384805 (ELSEVIER)S2095-4956(20)30024-3 DE-627 ger DE-627 rakwb eng 530 VZ 620 VZ 690 VZ 56.03 bkl Wu, Min verfasserin aut High crystallinity and photovoltaic performance of CsPbI3 film enabled by secondary dimension 2020transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. Yan, Keyou oth Wang, Yong oth Kang, Xiongwu oth Enthalten in Elsevier Praveen Kumar, D. ELSEVIER Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation 2015transfer abstract Amsterdam [u.a.] (DE-627)ELV01862751X volume:48 year:2020 pages:181-186 extent:6 https://doi.org/10.1016/j.jechem.2020.01.009 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_21 GBV_ILN_40 56.03 Methoden im Bauingenieurwesen VZ AR 48 2020 181-186 6 |
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10.1016/j.jechem.2020.01.009 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001145.pica (DE-627)ELV050384805 (ELSEVIER)S2095-4956(20)30024-3 DE-627 ger DE-627 rakwb eng 530 VZ 620 VZ 690 VZ 56.03 bkl Wu, Min verfasserin aut High crystallinity and photovoltaic performance of CsPbI3 film enabled by secondary dimension 2020transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. Yan, Keyou oth Wang, Yong oth Kang, Xiongwu oth Enthalten in Elsevier Praveen Kumar, D. ELSEVIER Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation 2015transfer abstract Amsterdam [u.a.] (DE-627)ELV01862751X volume:48 year:2020 pages:181-186 extent:6 https://doi.org/10.1016/j.jechem.2020.01.009 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_21 GBV_ILN_40 56.03 Methoden im Bauingenieurwesen VZ AR 48 2020 181-186 6 |
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10.1016/j.jechem.2020.01.009 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001145.pica (DE-627)ELV050384805 (ELSEVIER)S2095-4956(20)30024-3 DE-627 ger DE-627 rakwb eng 530 VZ 620 VZ 690 VZ 56.03 bkl Wu, Min verfasserin aut High crystallinity and photovoltaic performance of CsPbI3 film enabled by secondary dimension 2020transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. Yan, Keyou oth Wang, Yong oth Kang, Xiongwu oth Enthalten in Elsevier Praveen Kumar, D. ELSEVIER Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation 2015transfer abstract Amsterdam [u.a.] (DE-627)ELV01862751X volume:48 year:2020 pages:181-186 extent:6 https://doi.org/10.1016/j.jechem.2020.01.009 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_21 GBV_ILN_40 56.03 Methoden im Bauingenieurwesen VZ AR 48 2020 181-186 6 |
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10.1016/j.jechem.2020.01.009 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001145.pica (DE-627)ELV050384805 (ELSEVIER)S2095-4956(20)30024-3 DE-627 ger DE-627 rakwb eng 530 VZ 620 VZ 690 VZ 56.03 bkl Wu, Min verfasserin aut High crystallinity and photovoltaic performance of CsPbI3 film enabled by secondary dimension 2020transfer abstract 6 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. Yan, Keyou oth Wang, Yong oth Kang, Xiongwu oth Enthalten in Elsevier Praveen Kumar, D. ELSEVIER Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation 2015transfer abstract Amsterdam [u.a.] (DE-627)ELV01862751X volume:48 year:2020 pages:181-186 extent:6 https://doi.org/10.1016/j.jechem.2020.01.009 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U GBV_ILN_21 GBV_ILN_40 56.03 Methoden im Bauingenieurwesen VZ AR 48 2020 181-186 6 |
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Enthalten in Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation Amsterdam [u.a.] volume:48 year:2020 pages:181-186 extent:6 |
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Enthalten in Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation Amsterdam [u.a.] volume:48 year:2020 pages:181-186 extent:6 |
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Cu2O-sensitized TiO2 nanorods with nanocavities for highly efficient photocatalytic hydrogen production under solar irradiation |
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High crystallinity and photovoltaic performance of CsPbI3 film enabled by secondary dimension |
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The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. |
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The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. |
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The photovoltaic performance of perovskite sloar cells (PSCs) is strongly dependent on the crystallinity, morphorlogy and defects of perovskite films. In the present work, a novel strategy was developed to fabricate the high quality CsPbI3 inorganic perovskite by tuning the growth dynamics of CsPbI3 by pretreatment of fresh CsPbI3 films with phenylethylamine iodide (PEAI). The PEAI can mediate the phase transformation from 1D (DMAPbI3) (DMA: dimethylammonium) to 3D CsPbI3 all-inorganic perovskite films via the PEA2CsPb2I7 of 2D perovskite intermediate phase, resulting in highly crystalline CsPbI3 perovskite films with remarkably enlarged grains and reduced defects. The as-achieved highly crystalline CsPbI3 inorganic perovskite not only exhibited improved phase stability but also significant reduced defects. The perovskite solar cells based on these CsPbI3 thin films exhibited a champion efficiency of 17.08%, much higher than those prepared through posttreatment or direct addition of PEAI into CsPbI3 precursor solution. This work not only developed an effective strategy to prepare high crystalline CsPbI3 film and highly efficient CsPbI3-based all-inorganic PSCs, but also unraveled the mediation mechanism of CsPbI3 by pre-treatment of PEAI, shedding light for further development of high perfomance perovskite-based optoelectronics. |
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