Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering
Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunabil...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Gao, Tongyu [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020transfer abstract |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners - Jacobs, Jacquelyn A. ELSEVIER, 2017, JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics, Lausanne |
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| Übergeordnetes Werk: |
volume:848 ; year:2020 ; day:25 ; month:12 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.jallcom.2020.156557 |
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| 245 | 1 | 0 | |a Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering |
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| 520 | |a Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. | ||
| 520 | |a Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. | ||
| 650 | 7 | |a Luminescence tuning |2 Elsevier | |
| 650 | 7 | |a Crystal field engineering |2 Elsevier | |
| 650 | 7 | |a Near-infrared (NIR) phosphor |2 Elsevier | |
| 700 | 1 | |a Zhuang, Weidong |4 oth | |
| 700 | 1 | |a Liu, Ronghui |4 oth | |
| 700 | 1 | |a Liu, Yuanhong |4 oth | |
| 700 | 1 | |a Chen, Xiaoxia |4 oth | |
| 700 | 1 | |a Xue, Yuan |4 oth | |
| 773 | 0 | 8 | |i Enthalten in |n Elsevier |a Jacobs, Jacquelyn A. ELSEVIER |t Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners |d 2017 |d JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics |g Lausanne |w (DE-627)ELV001115774 |
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10.1016/j.jallcom.2020.156557 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001195.pica (DE-627)ELV05136297X (ELSEVIER)S0925-8388(20)32921-2 DE-627 ger DE-627 rakwb eng 630 VZ Gao, Tongyu verfasserin aut Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Luminescence tuning Elsevier Crystal field engineering Elsevier Near-infrared (NIR) phosphor Elsevier Zhuang, Weidong oth Liu, Ronghui oth Liu, Yuanhong oth Chen, Xiaoxia oth Xue, Yuan oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:848 year:2020 day:25 month:12 pages:0 https://doi.org/10.1016/j.jallcom.2020.156557 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 848 2020 25 1225 0 |
| spelling |
10.1016/j.jallcom.2020.156557 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001195.pica (DE-627)ELV05136297X (ELSEVIER)S0925-8388(20)32921-2 DE-627 ger DE-627 rakwb eng 630 VZ Gao, Tongyu verfasserin aut Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Luminescence tuning Elsevier Crystal field engineering Elsevier Near-infrared (NIR) phosphor Elsevier Zhuang, Weidong oth Liu, Ronghui oth Liu, Yuanhong oth Chen, Xiaoxia oth Xue, Yuan oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:848 year:2020 day:25 month:12 pages:0 https://doi.org/10.1016/j.jallcom.2020.156557 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 848 2020 25 1225 0 |
| allfields_unstemmed |
10.1016/j.jallcom.2020.156557 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001195.pica (DE-627)ELV05136297X (ELSEVIER)S0925-8388(20)32921-2 DE-627 ger DE-627 rakwb eng 630 VZ Gao, Tongyu verfasserin aut Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Luminescence tuning Elsevier Crystal field engineering Elsevier Near-infrared (NIR) phosphor Elsevier Zhuang, Weidong oth Liu, Ronghui oth Liu, Yuanhong oth Chen, Xiaoxia oth Xue, Yuan oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:848 year:2020 day:25 month:12 pages:0 https://doi.org/10.1016/j.jallcom.2020.156557 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 848 2020 25 1225 0 |
| allfieldsGer |
10.1016/j.jallcom.2020.156557 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001195.pica (DE-627)ELV05136297X (ELSEVIER)S0925-8388(20)32921-2 DE-627 ger DE-627 rakwb eng 630 VZ Gao, Tongyu verfasserin aut Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Luminescence tuning Elsevier Crystal field engineering Elsevier Near-infrared (NIR) phosphor Elsevier Zhuang, Weidong oth Liu, Ronghui oth Liu, Yuanhong oth Chen, Xiaoxia oth Xue, Yuan oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:848 year:2020 day:25 month:12 pages:0 https://doi.org/10.1016/j.jallcom.2020.156557 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 848 2020 25 1225 0 |
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10.1016/j.jallcom.2020.156557 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001195.pica (DE-627)ELV05136297X (ELSEVIER)S0925-8388(20)32921-2 DE-627 ger DE-627 rakwb eng 630 VZ Gao, Tongyu verfasserin aut Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. Luminescence tuning Elsevier Crystal field engineering Elsevier Near-infrared (NIR) phosphor Elsevier Zhuang, Weidong oth Liu, Ronghui oth Liu, Yuanhong oth Chen, Xiaoxia oth Xue, Yuan oth Enthalten in Elsevier Jacobs, Jacquelyn A. ELSEVIER Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners 2017 JAL : an interdisciplinary journal of materials science and solid-state chemistry and physics Lausanne (DE-627)ELV001115774 volume:848 year:2020 day:25 month:12 pages:0 https://doi.org/10.1016/j.jallcom.2020.156557 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA AR 848 2020 25 1225 0 |
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Enthalten in Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners Lausanne volume:848 year:2020 day:25 month:12 pages:0 |
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Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. 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Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners |
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Factors associated with canine resource guarding behaviour in the presence of people: A cross-sectional survey of dog owners |
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design and control of the luminescence in cr3+-doped nir phosphors via crystal field engineering |
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Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering |
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Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. |
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Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. |
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Near-infrared (NIR) light-emitting diodes (LEDs) have currently attracted increasing attention owing to high efficiency and longevity. Accordingly, NIR phosphor, as the indispensable role in NIR LEDs, needs to be enriched to meet widespread applications worldwide. Benefitting from structural tunability of LaSc3B4O12(LSB), a sequence of broadband phosphors, with continuous-tunable luminescence toward longer wavelength, can be designed by regulating the crystal field environment of the Cr3+ via substituting the Sc3+ by Y3+ in LSB host. The correlations among structural evolution, crystal field environment, and luminescence properties of LaSc3-x Y x B4O12(LSYB): Cr3+ (0 ≤ x ≤ 1.3) have been discussed in detail. Furthermore, substitution Y3+ for Sc3+ in LSB causes band gap variation of host lattice, demonstrated by the diffuse reflectance spectra, consequently resulting in improved quantum yield (QY), and mitigated thermal quenching behavior of LSYB: Cr3+ compared to that of Y3+-free sample. The above results demonstrate the superiority of crystal field engineering in exploring broadband NIR phosphors with modified luminescence performance for potential application in NIR pc-LEDs. |
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Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering |
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Zhuang, Weidong Liu, Ronghui Liu, Yuanhong Chen, Xiaoxia Xue, Yuan |
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