A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission
A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluoresc...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Yuan, Kaixuan [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020transfer abstract |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: New ablation evolution behaviors in micro-hole drilling of 2.5D C - Liu, Chang ELSEVIER, 2021, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:228 ; year:2020 ; pages:0 |
| Links: |
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| DOI / URN: |
10.1016/j.jlumin.2020.117595 |
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ELV051690926 |
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| 245 | 1 | 0 | |a A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission |
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| 520 | |a A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. | ||
| 520 | |a A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. | ||
| 650 | 7 | |a 1,5-dihydroxy naphthalene |2 Elsevier | |
| 650 | 7 | |a Acid-base response fluorescence |2 Elsevier | |
| 650 | 7 | |a Fluorescent polyurethane |2 Elsevier | |
| 650 | 7 | |a Solid-state fluorescence |2 Elsevier | |
| 700 | 1 | |a Peng, Qinghai |4 oth | |
| 700 | 1 | |a Yuan, Dandan |4 oth | |
| 700 | 1 | |a Cai, Xufu |4 oth | |
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10.1016/j.jlumin.2020.117595 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001169.pica (DE-627)ELV051690926 (ELSEVIER)S0022-2313(20)30873-5 DE-627 ger DE-627 rakwb eng 670 VZ 51.60 bkl 58.45 bkl Yuan, Kaixuan verfasserin aut A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. 1,5-dihydroxy naphthalene Elsevier Acid-base response fluorescence Elsevier Fluorescent polyurethane Elsevier Solid-state fluorescence Elsevier Peng, Qinghai oth Yuan, Dandan oth Cai, Xufu oth Enthalten in Elsevier Liu, Chang ELSEVIER New ablation evolution behaviors in micro-hole drilling of 2.5D C 2021 New York, NY [u.a.] (DE-627)ELV00662605X volume:228 year:2020 pages:0 https://doi.org/10.1016/j.jlumin.2020.117595 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 228 2020 0 |
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10.1016/j.jlumin.2020.117595 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001169.pica (DE-627)ELV051690926 (ELSEVIER)S0022-2313(20)30873-5 DE-627 ger DE-627 rakwb eng 670 VZ 51.60 bkl 58.45 bkl Yuan, Kaixuan verfasserin aut A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. 1,5-dihydroxy naphthalene Elsevier Acid-base response fluorescence Elsevier Fluorescent polyurethane Elsevier Solid-state fluorescence Elsevier Peng, Qinghai oth Yuan, Dandan oth Cai, Xufu oth Enthalten in Elsevier Liu, Chang ELSEVIER New ablation evolution behaviors in micro-hole drilling of 2.5D C 2021 New York, NY [u.a.] (DE-627)ELV00662605X volume:228 year:2020 pages:0 https://doi.org/10.1016/j.jlumin.2020.117595 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 228 2020 0 |
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10.1016/j.jlumin.2020.117595 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001169.pica (DE-627)ELV051690926 (ELSEVIER)S0022-2313(20)30873-5 DE-627 ger DE-627 rakwb eng 670 VZ 51.60 bkl 58.45 bkl Yuan, Kaixuan verfasserin aut A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. 1,5-dihydroxy naphthalene Elsevier Acid-base response fluorescence Elsevier Fluorescent polyurethane Elsevier Solid-state fluorescence Elsevier Peng, Qinghai oth Yuan, Dandan oth Cai, Xufu oth Enthalten in Elsevier Liu, Chang ELSEVIER New ablation evolution behaviors in micro-hole drilling of 2.5D C 2021 New York, NY [u.a.] (DE-627)ELV00662605X volume:228 year:2020 pages:0 https://doi.org/10.1016/j.jlumin.2020.117595 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 228 2020 0 |
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10.1016/j.jlumin.2020.117595 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001169.pica (DE-627)ELV051690926 (ELSEVIER)S0022-2313(20)30873-5 DE-627 ger DE-627 rakwb eng 670 VZ 51.60 bkl 58.45 bkl Yuan, Kaixuan verfasserin aut A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. 1,5-dihydroxy naphthalene Elsevier Acid-base response fluorescence Elsevier Fluorescent polyurethane Elsevier Solid-state fluorescence Elsevier Peng, Qinghai oth Yuan, Dandan oth Cai, Xufu oth Enthalten in Elsevier Liu, Chang ELSEVIER New ablation evolution behaviors in micro-hole drilling of 2.5D C 2021 New York, NY [u.a.] (DE-627)ELV00662605X volume:228 year:2020 pages:0 https://doi.org/10.1016/j.jlumin.2020.117595 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 228 2020 0 |
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10.1016/j.jlumin.2020.117595 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001169.pica (DE-627)ELV051690926 (ELSEVIER)S0022-2313(20)30873-5 DE-627 ger DE-627 rakwb eng 670 VZ 51.60 bkl 58.45 bkl Yuan, Kaixuan verfasserin aut A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission 2020transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. 1,5-dihydroxy naphthalene Elsevier Acid-base response fluorescence Elsevier Fluorescent polyurethane Elsevier Solid-state fluorescence Elsevier Peng, Qinghai oth Yuan, Dandan oth Cai, Xufu oth Enthalten in Elsevier Liu, Chang ELSEVIER New ablation evolution behaviors in micro-hole drilling of 2.5D C 2021 New York, NY [u.a.] (DE-627)ELV00662605X volume:228 year:2020 pages:0 https://doi.org/10.1016/j.jlumin.2020.117595 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde VZ 58.45 Gesteinshüttenkunde VZ AR 228 2020 0 |
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a multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission |
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A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission |
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A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. |
| abstractGer |
A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. |
| abstract_unstemmed |
A multifunctional fluorescent polyurethane (MFP) with solid-state and acid-base responsive fluorescence emission was reported by bonding 1,5-dihydroxy naphthalene(1,5-DN) into polyurethane backbone. The structure of MFP was confirmed by characterization with 1H NMR, FTIR and UV spectra. The fluorescent emission property and acid-base response behavior of MFP samples were studied on fluorescence spectrophotometer. The structural characterization revealed that 1,5-dihydroxy naphthalene was introduced into the polyurethane chain in the form of chemical bond. The physical entanglement and interactions of polymer chains could limit the strong π-π stacking between 1,5-DN. Therefore, MFP exhibited an obvious fluorescence emission at around 460 nm both in solution and solid state, which indicated that the “aggregation-caused quenching” (ACQ) phenomenon had been successfully eliminated. More interestingly, we found that the MFP solution samples have different fluorescence emission wavelengths in the acid (490 nm, blue-green light) and base (460 nm, blue light) environments, with a maximum displacement of over 30 nm. Meanwhile, the fluorescence intensity in strong base (pH = 11) environment decreased by 89% compared with that in strong acid (pH = 3) environment. Base on the dual feature response behavior, MFP has the potential to be used for double signal detection in strong acid and base environments. |
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A multifunctional polyurethane with solid-state and acid-base responsive fluorescent emission |
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