Facilitating the formation of SnO 2 film via hydroxyl groups for efficient perovskite solar cells
Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl grou...
Ausführliche Beschreibung
Autor*in: |
Bai, Yuchi [verfasserIn] Xing, Dongliang [verfasserIn] Luo, Huiming [verfasserIn] Jiang, Qing-Song [verfasserIn] Yuan, Ligang [verfasserIn] Ge, Xuehao [verfasserIn] Yang, Xiao [verfasserIn] Zhang, Yulin [verfasserIn] Xie, Fangyan [verfasserIn] Yan, Keyou [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2021 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Applied surface science - Amsterdam : Elsevier, 1985, 552 |
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Übergeordnetes Werk: |
volume:552 |
DOI / URN: |
10.1016/j.apsusc.2021.149459 |
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Katalog-ID: |
ELV053639804 |
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520 | |a Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. | ||
650 | 4 | |a Perovskite | |
650 | 4 | |a Solar cells | |
650 | 4 | |a SnO | |
650 | 4 | |a Hydroxyl groups | |
650 | 4 | |a SnCl | |
700 | 1 | |a Xing, Dongliang |e verfasserin |4 aut | |
700 | 1 | |a Luo, Huiming |e verfasserin |4 aut | |
700 | 1 | |a Jiang, Qing-Song |e verfasserin |4 aut | |
700 | 1 | |a Yuan, Ligang |e verfasserin |4 aut | |
700 | 1 | |a Ge, Xuehao |e verfasserin |4 aut | |
700 | 1 | |a Yang, Xiao |e verfasserin |4 aut | |
700 | 1 | |a Zhang, Yulin |e verfasserin |4 aut | |
700 | 1 | |a Xie, Fangyan |e verfasserin |4 aut | |
700 | 1 | |a Yan, Keyou |e verfasserin |4 aut | |
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10.1016/j.apsusc.2021.149459 doi (DE-627)ELV053639804 (ELSEVIER)S0169-4332(21)00535-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Bai, Yuchi verfasserin aut Facilitating the formation of SnO 2 film via hydroxyl groups for efficient perovskite solar cells 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. Perovskite Solar cells SnO Hydroxyl groups SnCl Xing, Dongliang verfasserin aut Luo, Huiming verfasserin aut Jiang, Qing-Song verfasserin aut Yuan, Ligang verfasserin aut Ge, Xuehao verfasserin aut Yang, Xiao verfasserin aut Zhang, Yulin verfasserin aut Xie, Fangyan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 552 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:552 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 552 |
spelling |
10.1016/j.apsusc.2021.149459 doi (DE-627)ELV053639804 (ELSEVIER)S0169-4332(21)00535-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Bai, Yuchi verfasserin aut Facilitating the formation of SnO 2 film via hydroxyl groups for efficient perovskite solar cells 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. Perovskite Solar cells SnO Hydroxyl groups SnCl Xing, Dongliang verfasserin aut Luo, Huiming verfasserin aut Jiang, Qing-Song verfasserin aut Yuan, Ligang verfasserin aut Ge, Xuehao verfasserin aut Yang, Xiao verfasserin aut Zhang, Yulin verfasserin aut Xie, Fangyan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 552 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:552 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 552 |
allfields_unstemmed |
10.1016/j.apsusc.2021.149459 doi (DE-627)ELV053639804 (ELSEVIER)S0169-4332(21)00535-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Bai, Yuchi verfasserin aut Facilitating the formation of SnO 2 film via hydroxyl groups for efficient perovskite solar cells 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. Perovskite Solar cells SnO Hydroxyl groups SnCl Xing, Dongliang verfasserin aut Luo, Huiming verfasserin aut Jiang, Qing-Song verfasserin aut Yuan, Ligang verfasserin aut Ge, Xuehao verfasserin aut Yang, Xiao verfasserin aut Zhang, Yulin verfasserin aut Xie, Fangyan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 552 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:552 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 552 |
allfieldsGer |
10.1016/j.apsusc.2021.149459 doi (DE-627)ELV053639804 (ELSEVIER)S0169-4332(21)00535-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Bai, Yuchi verfasserin aut Facilitating the formation of SnO 2 film via hydroxyl groups for efficient perovskite solar cells 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. Perovskite Solar cells SnO Hydroxyl groups SnCl Xing, Dongliang verfasserin aut Luo, Huiming verfasserin aut Jiang, Qing-Song verfasserin aut Yuan, Ligang verfasserin aut Ge, Xuehao verfasserin aut Yang, Xiao verfasserin aut Zhang, Yulin verfasserin aut Xie, Fangyan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 552 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:552 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 552 |
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10.1016/j.apsusc.2021.149459 doi (DE-627)ELV053639804 (ELSEVIER)S0169-4332(21)00535-3 DE-627 ger DE-627 rda eng 670 530 660 VZ 33.68 bkl 35.18 bkl 52.78 bkl Bai, Yuchi verfasserin aut Facilitating the formation of SnO 2 film via hydroxyl groups for efficient perovskite solar cells 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. Perovskite Solar cells SnO Hydroxyl groups SnCl Xing, Dongliang verfasserin aut Luo, Huiming verfasserin aut Jiang, Qing-Song verfasserin aut Yuan, Ligang verfasserin aut Ge, Xuehao verfasserin aut Yang, Xiao verfasserin aut Zhang, Yulin verfasserin aut Xie, Fangyan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Applied surface science Amsterdam : Elsevier, 1985 552 Online-Ressource (DE-627)312151128 (DE-600)2002520-8 (DE-576)094476985 nnns volume:552 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.68 Oberflächen Dünne Schichten Grenzflächen Physik VZ 35.18 Kolloidchemie Grenzflächenchemie VZ 52.78 Oberflächentechnik Wärmebehandlung VZ AR 552 |
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Bai, Yuchi @@aut@@ Xing, Dongliang @@aut@@ Luo, Huiming @@aut@@ Jiang, Qing-Song @@aut@@ Yuan, Ligang @@aut@@ Ge, Xuehao @@aut@@ Yang, Xiao @@aut@@ Zhang, Yulin @@aut@@ Xie, Fangyan @@aut@@ Yan, Keyou @@aut@@ |
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facilitating the formation of sno 2 film via hydroxyl groups for efficient perovskite solar cells |
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Facilitating the formation of SnO 2 film via hydroxyl groups for efficient perovskite solar cells |
abstract |
Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. |
abstractGer |
Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. |
abstract_unstemmed |
Interfacial engineering has been considered as an effective technique to improve the photovoltaic performance of perovskite solar cells (PSCs). Here, the interface between tin oxide (SnO2) film and fluorine-doped tin oxide (FTO) glass is dealt with a piranha solution, resulting in more hydroxyl groups on the surface of FTO glass. SnO2 film is fabricated by spin-coating SnCl2·2H2O precursor. Our results demonstrate that SnO2 film exhibits high electricalconductivity, low electron trap density, and suitable energy level. Furthermore, SnO2 film with low roughness is beneficial to fabricate high-quality perovskite film. Then, the PSCs with the structure of FTO/SnO2/Cs0.05(MA0.17FA0.83)0.95Pb(I0.83Br0.17)3/Spiro-OMeTAD/Au are also fabricated. The highest power conversion efficiency (PCE) of PSCs increases from 18.28% to 19.51%, and the average PCE enhances from 17.82% to 18.89%. The optimized PSC shows the long-term stability and remains 97% of its initial PCE after 4000 h on-shelf lifetime test. |
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Xing, Dongliang Luo, Huiming Jiang, Qing-Song Yuan, Ligang Ge, Xuehao Yang, Xiao Zhang, Yulin Xie, Fangyan Yan, Keyou |
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|
score |
7.39849 |