Effect of La2O3 on the viscosity and structure of CaO–SiO2(–Al2O3)–La2O3 melts
The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that...
Ausführliche Beschreibung
Autor*in: |
Guo, Wentao [verfasserIn] |
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Englisch |
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2021transfer abstract |
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Enthalten in: Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving - Lu, Li ELSEVIER, 2020, including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science, New York, NY [u.a.] |
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Übergeordnetes Werk: |
volume:266 ; year:2021 ; day:1 ; month:07 ; pages:0 |
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DOI / URN: |
10.1016/j.matchemphys.2021.124526 |
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ELV053756568 |
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520 | |a The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. | ||
520 | |a The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. | ||
650 | 7 | |a La2O3 |2 Elsevier | |
650 | 7 | |a Viscosity |2 Elsevier | |
650 | 7 | |a La2O3/Al2O3 ratio |2 Elsevier | |
650 | 7 | |a Silica tetrahedron structure |2 Elsevier | |
700 | 1 | |a Ding, Ziqi |4 oth | |
700 | 1 | |a Wang, Jinming |4 oth | |
700 | 1 | |a Wu, Jun |4 oth | |
700 | 1 | |a Wang, Zhi |4 oth | |
773 | 0 | 8 | |i Enthalten in |n Elsevier |a Lu, Li ELSEVIER |t Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving |d 2020 |d including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science |g New York, NY [u.a.] |w (DE-627)ELV005250781 |
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10.1016/j.matchemphys.2021.124526 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001369.pica (DE-627)ELV053756568 (ELSEVIER)S0254-0584(21)00309-6 DE-627 ger DE-627 rakwb eng 610 VZ 44.38 bkl 44.91 bkl Guo, Wentao verfasserin aut Effect of La2O3 on the viscosity and structure of CaO–SiO2(–Al2O3)–La2O3 melts 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. La2O3 Elsevier Viscosity Elsevier La2O3/Al2O3 ratio Elsevier Silica tetrahedron structure Elsevier Ding, Ziqi oth Wang, Jinming oth Wu, Jun oth Wang, Zhi oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:266 year:2021 day:1 month:07 pages:0 https://doi.org/10.1016/j.matchemphys.2021.124526 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 266 2021 1 0701 0 |
spelling |
10.1016/j.matchemphys.2021.124526 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001369.pica (DE-627)ELV053756568 (ELSEVIER)S0254-0584(21)00309-6 DE-627 ger DE-627 rakwb eng 610 VZ 44.38 bkl 44.91 bkl Guo, Wentao verfasserin aut Effect of La2O3 on the viscosity and structure of CaO–SiO2(–Al2O3)–La2O3 melts 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. La2O3 Elsevier Viscosity Elsevier La2O3/Al2O3 ratio Elsevier Silica tetrahedron structure Elsevier Ding, Ziqi oth Wang, Jinming oth Wu, Jun oth Wang, Zhi oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:266 year:2021 day:1 month:07 pages:0 https://doi.org/10.1016/j.matchemphys.2021.124526 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 266 2021 1 0701 0 |
allfields_unstemmed |
10.1016/j.matchemphys.2021.124526 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001369.pica (DE-627)ELV053756568 (ELSEVIER)S0254-0584(21)00309-6 DE-627 ger DE-627 rakwb eng 610 VZ 44.38 bkl 44.91 bkl Guo, Wentao verfasserin aut Effect of La2O3 on the viscosity and structure of CaO–SiO2(–Al2O3)–La2O3 melts 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. La2O3 Elsevier Viscosity Elsevier La2O3/Al2O3 ratio Elsevier Silica tetrahedron structure Elsevier Ding, Ziqi oth Wang, Jinming oth Wu, Jun oth Wang, Zhi oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:266 year:2021 day:1 month:07 pages:0 https://doi.org/10.1016/j.matchemphys.2021.124526 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 266 2021 1 0701 0 |
allfieldsGer |
10.1016/j.matchemphys.2021.124526 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001369.pica (DE-627)ELV053756568 (ELSEVIER)S0254-0584(21)00309-6 DE-627 ger DE-627 rakwb eng 610 VZ 44.38 bkl 44.91 bkl Guo, Wentao verfasserin aut Effect of La2O3 on the viscosity and structure of CaO–SiO2(–Al2O3)–La2O3 melts 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. La2O3 Elsevier Viscosity Elsevier La2O3/Al2O3 ratio Elsevier Silica tetrahedron structure Elsevier Ding, Ziqi oth Wang, Jinming oth Wu, Jun oth Wang, Zhi oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:266 year:2021 day:1 month:07 pages:0 https://doi.org/10.1016/j.matchemphys.2021.124526 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 266 2021 1 0701 0 |
allfieldsSound |
10.1016/j.matchemphys.2021.124526 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001369.pica (DE-627)ELV053756568 (ELSEVIER)S0254-0584(21)00309-6 DE-627 ger DE-627 rakwb eng 610 VZ 44.38 bkl 44.91 bkl Guo, Wentao verfasserin aut Effect of La2O3 on the viscosity and structure of CaO–SiO2(–Al2O3)–La2O3 melts 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. La2O3 Elsevier Viscosity Elsevier La2O3/Al2O3 ratio Elsevier Silica tetrahedron structure Elsevier Ding, Ziqi oth Wang, Jinming oth Wu, Jun oth Wang, Zhi oth Enthalten in Elsevier Lu, Li ELSEVIER Road traffic crash characteristics of drivers who take prescription medicines that carry a risk to driving 2020 including materials science communications : an international, interdisciplinary journal on science characterization and processing of advanced materials : the international journal of the Chinese Society for Materials Science New York, NY [u.a.] (DE-627)ELV005250781 volume:266 year:2021 day:1 month:07 pages:0 https://doi.org/10.1016/j.matchemphys.2021.124526 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.38 Pharmakologie VZ 44.91 Psychiatrie Psychopathologie VZ AR 266 2021 1 0701 0 |
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effect of la2o3 on the viscosity and structure of cao–sio2(–al2o3)–la2o3 melts |
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Effect of La2O3 on the viscosity and structure of CaO–SiO2(–Al2O3)–La2O3 melts |
abstract |
The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. |
abstractGer |
The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. |
abstract_unstemmed |
The rotating cylinder method was used to understand the effects of La2O3 and the La2O3/Al2O3 ratios on the melt viscosity of CaO–SiO2(–Al2O3)–La2O3 at high temperatures. The structural characterization of these quenched glass samples were investigated using Raman spectroscopy. The results show that the viscosity of the CaO–SiO2(–Al2O3)–La2O3 melt is significantly reduced due to additions of La2O3. The La2O3 additions simplified the structure of the silicon-oxygen ion groups in the melt, which created a smaller melt viscosity. The critical transition temperature is proportional to the La2O3 content and inversely proportional to the La2O3/Al2O3 ratio. La3+ and Al3+ make the viscosity-temperature curve of CaO–SiO2–Al2O3–La2O3 melt show different characteristics. There is no critical transition temperature when the melt without La2O3, and the critical transition temperature appears after adding La2O3. The La2O3 plays a role like alkaline oxide in the CaO–SiO2–Al2O3–La2O3 melt. In addition, the degree of polymerization of the melt decreased relative to the La2O3 content and La2O3/Al2O3 ratio. Consequently, the La2O3 behaves as a network modifier for the complex silicate anions of CaO–SiO2–La2O3 and CaO–SiO2–Al2O3–La2O3 melts. |
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Effect of La2O3 on the viscosity and structure of CaO–SiO2(–Al2O3)–La2O3 melts |
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