Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light
Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Zhao, Shiyin [verfasserIn] Li, Shun [verfasserIn] Long, Yangke [verfasserIn] Shen, Xuehua [verfasserIn] Zhao, Zhicheng [verfasserIn] Wei, Qiliang [verfasserIn] Wang, Shubin [verfasserIn] Zhang, Zhen [verfasserIn] Zhang, Xuanjun [verfasserIn] Zhang, Zuotai [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Chemosphere - Amsterdam [u.a.] : Elsevier Science, 1972, 280 |
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| Übergeordnetes Werk: |
volume:280 |
| DOI / URN: |
10.1016/j.chemosphere.2021.130637 |
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| Katalog-ID: |
ELV054458617 |
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| 245 | 1 | 0 | |a Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light |
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| 520 | |a Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. | ||
| 650 | 4 | |a MOF derivatives | |
| 650 | 4 | |a Heterostructures | |
| 650 | 4 | |a Z-scheme photocatalysts | |
| 650 | 4 | |a Peroxymonosulfate | |
| 650 | 4 | |a Pollutant degradation | |
| 700 | 1 | |a Li, Shun |e verfasserin |0 (orcid)0000-0002-9488-8279 |4 aut | |
| 700 | 1 | |a Long, Yangke |e verfasserin |4 aut | |
| 700 | 1 | |a Shen, Xuehua |e verfasserin |4 aut | |
| 700 | 1 | |a Zhao, Zhicheng |e verfasserin |4 aut | |
| 700 | 1 | |a Wei, Qiliang |e verfasserin |4 aut | |
| 700 | 1 | |a Wang, Shubin |e verfasserin |0 (orcid)0000-0002-7626-3080 |4 aut | |
| 700 | 1 | |a Zhang, Zhen |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Xuanjun |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Zuotai |e verfasserin |4 aut | |
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10.1016/j.chemosphere.2021.130637 doi (DE-627)ELV054458617 (ELSEVIER)S0045-6535(21)01108-5 DE-627 ger DE-627 rda eng 333.7 VZ 43.00 bkl Zhao, Shiyin verfasserin aut Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. MOF derivatives Heterostructures Z-scheme photocatalysts Peroxymonosulfate Pollutant degradation Li, Shun verfasserin (orcid)0000-0002-9488-8279 aut Long, Yangke verfasserin aut Shen, Xuehua verfasserin aut Zhao, Zhicheng verfasserin aut Wei, Qiliang verfasserin aut Wang, Shubin verfasserin (orcid)0000-0002-7626-3080 aut Zhang, Zhen verfasserin aut Zhang, Xuanjun verfasserin aut Zhang, Zuotai verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 280 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:280 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines VZ AR 280 |
| spelling |
10.1016/j.chemosphere.2021.130637 doi (DE-627)ELV054458617 (ELSEVIER)S0045-6535(21)01108-5 DE-627 ger DE-627 rda eng 333.7 VZ 43.00 bkl Zhao, Shiyin verfasserin aut Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. MOF derivatives Heterostructures Z-scheme photocatalysts Peroxymonosulfate Pollutant degradation Li, Shun verfasserin (orcid)0000-0002-9488-8279 aut Long, Yangke verfasserin aut Shen, Xuehua verfasserin aut Zhao, Zhicheng verfasserin aut Wei, Qiliang verfasserin aut Wang, Shubin verfasserin (orcid)0000-0002-7626-3080 aut Zhang, Zhen verfasserin aut Zhang, Xuanjun verfasserin aut Zhang, Zuotai verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 280 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:280 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines VZ AR 280 |
| allfields_unstemmed |
10.1016/j.chemosphere.2021.130637 doi (DE-627)ELV054458617 (ELSEVIER)S0045-6535(21)01108-5 DE-627 ger DE-627 rda eng 333.7 VZ 43.00 bkl Zhao, Shiyin verfasserin aut Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. MOF derivatives Heterostructures Z-scheme photocatalysts Peroxymonosulfate Pollutant degradation Li, Shun verfasserin (orcid)0000-0002-9488-8279 aut Long, Yangke verfasserin aut Shen, Xuehua verfasserin aut Zhao, Zhicheng verfasserin aut Wei, Qiliang verfasserin aut Wang, Shubin verfasserin (orcid)0000-0002-7626-3080 aut Zhang, Zhen verfasserin aut Zhang, Xuanjun verfasserin aut Zhang, Zuotai verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 280 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:280 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines VZ AR 280 |
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10.1016/j.chemosphere.2021.130637 doi (DE-627)ELV054458617 (ELSEVIER)S0045-6535(21)01108-5 DE-627 ger DE-627 rda eng 333.7 VZ 43.00 bkl Zhao, Shiyin verfasserin aut Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. MOF derivatives Heterostructures Z-scheme photocatalysts Peroxymonosulfate Pollutant degradation Li, Shun verfasserin (orcid)0000-0002-9488-8279 aut Long, Yangke verfasserin aut Shen, Xuehua verfasserin aut Zhao, Zhicheng verfasserin aut Wei, Qiliang verfasserin aut Wang, Shubin verfasserin (orcid)0000-0002-7626-3080 aut Zhang, Zhen verfasserin aut Zhang, Xuanjun verfasserin aut Zhang, Zuotai verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 280 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:280 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines VZ AR 280 |
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10.1016/j.chemosphere.2021.130637 doi (DE-627)ELV054458617 (ELSEVIER)S0045-6535(21)01108-5 DE-627 ger DE-627 rda eng 333.7 VZ 43.00 bkl Zhao, Shiyin verfasserin aut Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. MOF derivatives Heterostructures Z-scheme photocatalysts Peroxymonosulfate Pollutant degradation Li, Shun verfasserin (orcid)0000-0002-9488-8279 aut Long, Yangke verfasserin aut Shen, Xuehua verfasserin aut Zhao, Zhicheng verfasserin aut Wei, Qiliang verfasserin aut Wang, Shubin verfasserin (orcid)0000-0002-7626-3080 aut Zhang, Zhen verfasserin aut Zhang, Xuanjun verfasserin aut Zhang, Zuotai verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 280 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:280 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines VZ AR 280 |
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Zhao, Shiyin @@aut@@ Li, Shun @@aut@@ Long, Yangke @@aut@@ Shen, Xuehua @@aut@@ Zhao, Zhicheng @@aut@@ Wei, Qiliang @@aut@@ Wang, Shubin @@aut@@ Zhang, Zhen @@aut@@ Zhang, Xuanjun @@aut@@ Zhang, Zuotai @@aut@@ |
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333.7 VZ 43.00 bkl Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light MOF derivatives Heterostructures Z-scheme photocatalysts Peroxymonosulfate Pollutant degradation |
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Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light |
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Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light |
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Zhao, Shiyin Li, Shun Long, Yangke Shen, Xuehua Zhao, Zhicheng Wei, Qiliang Wang, Shubin Zhang, Zhen Zhang, Xuanjun Zhang, Zuotai |
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ce-based heterogeneous catalysts by partial thermal decomposition of ce-mofs in activation of peroxymonosulfate for the removal of organic pollutants under visible light |
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Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light |
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Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. |
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Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. |
| abstract_unstemmed |
Metal-organic framework (MOF) derivatives have drawn considerable attention for applications in various fields. In this work, spindle-shaped Ce-TCPPs were assembled by a rapid microwave-assisted hydrothermal method. After thermal treatment at low temperature under a N2 atmosphere, the Ce-TCPPs were partially pyrolyzed and converted to a novel CeO2/N-doped carbon/Ce-TCPP nanocomposite. Compared to completely decomposed materials, these partially decomposed heterogeneous catalysts exhibited significantly higher photocatalytic activation ability toward PMS for the removal of organic pollutants (e.g., rhodamine B, methylene blue, methyl orange, tetracycline and oxytetracycline). For the optimized sample thermal treated at 450 °C, a 100 mL RhB solution (10 mg/L) can be removed within 20 min with the assistance of PMS under visible light. The significantly enhanced activity can be attributed to the effective spatial separation of photogenerated electrons and holes in the formed Z-scheme CeO2/N-doped carbon/Ce-TCPP system. This work may provide useful guidance for the design and fabrication of MOF-derived photocatalytic systems for environmental remediation. |
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Ce-based heterogeneous catalysts by partial thermal decomposition of Ce-MOFs in activation of peroxymonosulfate for the removal of organic pollutants under visible light |
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