Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction
Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed...
Ausführliche Beschreibung
Autor*in: |
Wang, Xiaoyu [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2021transfer abstract |
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Übergeordnetes Werk: |
Enthalten in: Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch - Zhang, Lei ELSEVIER, 2018, the journal of the International Society of Electrochemistry (ISE), New York, NY [u.a.] |
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Übergeordnetes Werk: |
volume:390 ; year:2021 ; day:10 ; month:09 ; pages:0 |
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DOI / URN: |
10.1016/j.electacta.2021.138872 |
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520 | |a Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. | ||
520 | |a Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. | ||
700 | 1 | |a Liu, Hao |4 oth | |
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700 | 1 | |a Li, Jun |4 oth | |
700 | 1 | |a Lu, Yi |4 oth | |
700 | 1 | |a Wang, Lixi |4 oth | |
700 | 1 | |a Wang, Zhihong |4 oth | |
700 | 1 | |a Zhang, Xinping |4 oth | |
700 | 1 | |a Ding, Xifeng |4 oth | |
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10.1016/j.electacta.2021.138872 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001477.pica (DE-627)ELV054851114 (ELSEVIER)S0013-4686(21)01162-2 DE-627 ger DE-627 rakwb eng 610 VZ 44.00 bkl Wang, Xiaoyu verfasserin aut Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Liu, Hao oth Li, Mingze oth Li, Jun oth Lu, Yi oth Wang, Lixi oth Wang, Zhihong oth Zhang, Xinping oth Ding, Xifeng oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:390 year:2021 day:10 month:09 pages:0 https://doi.org/10.1016/j.electacta.2021.138872 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 390 2021 10 0910 0 |
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10.1016/j.electacta.2021.138872 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001477.pica (DE-627)ELV054851114 (ELSEVIER)S0013-4686(21)01162-2 DE-627 ger DE-627 rakwb eng 610 VZ 44.00 bkl Wang, Xiaoyu verfasserin aut Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Liu, Hao oth Li, Mingze oth Li, Jun oth Lu, Yi oth Wang, Lixi oth Wang, Zhihong oth Zhang, Xinping oth Ding, Xifeng oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:390 year:2021 day:10 month:09 pages:0 https://doi.org/10.1016/j.electacta.2021.138872 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 390 2021 10 0910 0 |
allfields_unstemmed |
10.1016/j.electacta.2021.138872 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001477.pica (DE-627)ELV054851114 (ELSEVIER)S0013-4686(21)01162-2 DE-627 ger DE-627 rakwb eng 610 VZ 44.00 bkl Wang, Xiaoyu verfasserin aut Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Liu, Hao oth Li, Mingze oth Li, Jun oth Lu, Yi oth Wang, Lixi oth Wang, Zhihong oth Zhang, Xinping oth Ding, Xifeng oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:390 year:2021 day:10 month:09 pages:0 https://doi.org/10.1016/j.electacta.2021.138872 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 390 2021 10 0910 0 |
allfieldsGer |
10.1016/j.electacta.2021.138872 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001477.pica (DE-627)ELV054851114 (ELSEVIER)S0013-4686(21)01162-2 DE-627 ger DE-627 rakwb eng 610 VZ 44.00 bkl Wang, Xiaoyu verfasserin aut Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Liu, Hao oth Li, Mingze oth Li, Jun oth Lu, Yi oth Wang, Lixi oth Wang, Zhihong oth Zhang, Xinping oth Ding, Xifeng oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:390 year:2021 day:10 month:09 pages:0 https://doi.org/10.1016/j.electacta.2021.138872 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 390 2021 10 0910 0 |
allfieldsSound |
10.1016/j.electacta.2021.138872 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001477.pica (DE-627)ELV054851114 (ELSEVIER)S0013-4686(21)01162-2 DE-627 ger DE-627 rakwb eng 610 VZ 44.00 bkl Wang, Xiaoyu verfasserin aut Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction 2021transfer abstract nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. Liu, Hao oth Li, Mingze oth Li, Jun oth Lu, Yi oth Wang, Lixi oth Wang, Zhihong oth Zhang, Xinping oth Ding, Xifeng oth Enthalten in Elsevier Zhang, Lei ELSEVIER Computed tomographic morphometric analysis of lateral inclination C1 pedicle screw for atlantoaxial instability patients with a narrow C1 posterior arch 2018 the journal of the International Society of Electrochemistry (ISE) New York, NY [u.a.] (DE-627)ELV001212419 volume:390 year:2021 day:10 month:09 pages:0 https://doi.org/10.1016/j.electacta.2021.138872 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.00 Medizin: Allgemeines VZ AR 390 2021 10 0910 0 |
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Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction |
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modulation of electronic structure and oxygen vacancies of perovskites srcoo3-δ by sulfur doping enables highly active and stable oxygen evolution reaction |
title_auth |
Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction |
abstract |
Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. |
abstractGer |
Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. |
abstract_unstemmed |
Resolving the energy crisis and advancing the commercialization of electrochemical conversion devices is urgent tasks nowadays. Developing cost-effective electrocatalysts for oxygen evolution reaction (OER) is of foremost importance for these electrochemical conversion devices. Herein, we developed a non-metallic and cost-effective sulfur-doped SrCoO3-δ perovskite electrocatalyst, namely SrCoO3- x S x (x = 0.02, 0.04, 0.06, 0.08 and 0.1, denoted as SCS2, SCS4, SCS6, SCS8 and SCS10, respectively) for water splitting in alkaline solution. Sulfur doping results in a structural change of SrCoO3-δ perovskite from hexagonal to cubic perovskite. The electrochemical performance of this catalyst indicates that an optimal sulfur doping could enhance the conductivity of SrCoO3-δ, resulting in a remarkable improvement on OER activity. The DFT calculation also confirm S doping can improve the electron conduction by lowering the activation energy of electron conductivity. Moreover, the doped SrCoO3- x S x also show enhanced durability due to the stable cubic structure with sulfur substitution. This work offers an inexpensive doping strategy for SrCoO3-δ perovskite as an efficient electrocatalyst for the enhanced electrochemical performance of OER activity in water splitting. |
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title_short |
Modulation of electronic structure and oxygen vacancies of perovskites SrCoO3-δ by sulfur doping enables highly active and stable oxygen evolution reaction |
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