Construction of dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst via incomplete solid state chemical combustion reactions for organic pollutant degradation with simultaneous hydrogen production
A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degr...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Ma, Xiaoxue [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021transfer abstract |
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| Schlagwörter: |
Simultaneous hydrogen production |
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| Umfang: |
15 |
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| Übergeordnetes Werk: |
Enthalten in: External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs - Dedhia, Kavita ELSEVIER, 2018, official journal of the International Association for Hydrogen Energy, New York, NY [u.a.] |
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| Übergeordnetes Werk: |
volume:46 ; year:2021 ; number:62 ; day:8 ; month:09 ; pages:31659-31673 ; extent:15 |
| Links: |
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| DOI / URN: |
10.1016/j.ijhydene.2021.07.076 |
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| 245 | 1 | 0 | |a Construction of dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst via incomplete solid state chemical combustion reactions for organic pollutant degradation with simultaneous hydrogen production |
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| 520 | |a A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. | ||
| 520 | |a A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. | ||
| 650 | 7 | |a Dual Z-scheme photocatalyst |2 Elsevier | |
| 650 | 7 | |a Photocatalytic degradation |2 Elsevier | |
| 650 | 7 | |a Blurred contact interface |2 Elsevier | |
| 650 | 7 | |a Simultaneous hydrogen production |2 Elsevier | |
| 650 | 7 | |a NiO/NiFe2O4/Fe2O3 ternary composite |2 Elsevier | |
| 650 | 7 | |a Incomplete solid state chemical combustion reaction method |2 Elsevier | |
| 700 | 1 | |a Liu, Xueke |4 oth | |
| 700 | 1 | |a Zhang, Xing |4 oth | |
| 700 | 1 | |a Piao, Congcong |4 oth | |
| 700 | 1 | |a Liu, Zhiyu |4 oth | |
| 700 | 1 | |a Fang, Dawei |4 oth | |
| 700 | 1 | |a Wang, Jun |4 oth | |
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10.1016/j.ijhydene.2021.07.076 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001669.pica (DE-627)ELV05501643X (ELSEVIER)S0360-3199(21)02717-8 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Ma, Xiaoxue verfasserin aut Construction of dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst via incomplete solid state chemical combustion reactions for organic pollutant degradation with simultaneous hydrogen production 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. Dual Z-scheme photocatalyst Elsevier Photocatalytic degradation Elsevier Blurred contact interface Elsevier Simultaneous hydrogen production Elsevier NiO/NiFe2O4/Fe2O3 ternary composite Elsevier Incomplete solid state chemical combustion reaction method Elsevier Liu, Xueke oth Zhang, Xing oth Piao, Congcong oth Liu, Zhiyu oth Fang, Dawei oth Wang, Jun oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:46 year:2021 number:62 day:8 month:09 pages:31659-31673 extent:15 https://doi.org/10.1016/j.ijhydene.2021.07.076 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 46 2021 62 8 0908 31659-31673 15 |
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10.1016/j.ijhydene.2021.07.076 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001669.pica (DE-627)ELV05501643X (ELSEVIER)S0360-3199(21)02717-8 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Ma, Xiaoxue verfasserin aut Construction of dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst via incomplete solid state chemical combustion reactions for organic pollutant degradation with simultaneous hydrogen production 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. Dual Z-scheme photocatalyst Elsevier Photocatalytic degradation Elsevier Blurred contact interface Elsevier Simultaneous hydrogen production Elsevier NiO/NiFe2O4/Fe2O3 ternary composite Elsevier Incomplete solid state chemical combustion reaction method Elsevier Liu, Xueke oth Zhang, Xing oth Piao, Congcong oth Liu, Zhiyu oth Fang, Dawei oth Wang, Jun oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:46 year:2021 number:62 day:8 month:09 pages:31659-31673 extent:15 https://doi.org/10.1016/j.ijhydene.2021.07.076 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 46 2021 62 8 0908 31659-31673 15 |
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10.1016/j.ijhydene.2021.07.076 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001669.pica (DE-627)ELV05501643X (ELSEVIER)S0360-3199(21)02717-8 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Ma, Xiaoxue verfasserin aut Construction of dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst via incomplete solid state chemical combustion reactions for organic pollutant degradation with simultaneous hydrogen production 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. Dual Z-scheme photocatalyst Elsevier Photocatalytic degradation Elsevier Blurred contact interface Elsevier Simultaneous hydrogen production Elsevier NiO/NiFe2O4/Fe2O3 ternary composite Elsevier Incomplete solid state chemical combustion reaction method Elsevier Liu, Xueke oth Zhang, Xing oth Piao, Congcong oth Liu, Zhiyu oth Fang, Dawei oth Wang, Jun oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:46 year:2021 number:62 day:8 month:09 pages:31659-31673 extent:15 https://doi.org/10.1016/j.ijhydene.2021.07.076 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 46 2021 62 8 0908 31659-31673 15 |
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10.1016/j.ijhydene.2021.07.076 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001669.pica (DE-627)ELV05501643X (ELSEVIER)S0360-3199(21)02717-8 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Ma, Xiaoxue verfasserin aut Construction of dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst via incomplete solid state chemical combustion reactions for organic pollutant degradation with simultaneous hydrogen production 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. Dual Z-scheme photocatalyst Elsevier Photocatalytic degradation Elsevier Blurred contact interface Elsevier Simultaneous hydrogen production Elsevier NiO/NiFe2O4/Fe2O3 ternary composite Elsevier Incomplete solid state chemical combustion reaction method Elsevier Liu, Xueke oth Zhang, Xing oth Piao, Congcong oth Liu, Zhiyu oth Fang, Dawei oth Wang, Jun oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:46 year:2021 number:62 day:8 month:09 pages:31659-31673 extent:15 https://doi.org/10.1016/j.ijhydene.2021.07.076 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 46 2021 62 8 0908 31659-31673 15 |
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10.1016/j.ijhydene.2021.07.076 doi /cbs_pica/cbs_olc/import_discovery/elsevier/einzuspielen/GBV00000000001669.pica (DE-627)ELV05501643X (ELSEVIER)S0360-3199(21)02717-8 DE-627 ger DE-627 rakwb eng 610 VZ 44.94 bkl Ma, Xiaoxue verfasserin aut Construction of dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst via incomplete solid state chemical combustion reactions for organic pollutant degradation with simultaneous hydrogen production 2021transfer abstract 15 nicht spezifiziert zzz rdacontent nicht spezifiziert z rdamedia nicht spezifiziert zu rdacarrier A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. Dual Z-scheme photocatalyst Elsevier Photocatalytic degradation Elsevier Blurred contact interface Elsevier Simultaneous hydrogen production Elsevier NiO/NiFe2O4/Fe2O3 ternary composite Elsevier Incomplete solid state chemical combustion reaction method Elsevier Liu, Xueke oth Zhang, Xing oth Piao, Congcong oth Liu, Zhiyu oth Fang, Dawei oth Wang, Jun oth Enthalten in Elsevier Dedhia, Kavita ELSEVIER External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs 2018 official journal of the International Association for Hydrogen Energy New York, NY [u.a.] (DE-627)ELV000127019 volume:46 year:2021 number:62 day:8 month:09 pages:31659-31673 extent:15 https://doi.org/10.1016/j.ijhydene.2021.07.076 Volltext GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA 44.94 Hals-Nasen-Ohrenheilkunde VZ AR 46 2021 62 8 0908 31659-31673 15 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:46 year:2021 number:62 day:8 month:09 pages:31659-31673 extent:15 |
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Enthalten in External auditory canal: Inferior, posterior-inferior, and anterior canal wall overhangs New York, NY [u.a.] volume:46 year:2021 number:62 day:8 month:09 pages:31659-31673 extent:15 |
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Construction of dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst via incomplete solid state chemical combustion reactions for organic pollutant degradation with simultaneous hydrogen production |
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A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. |
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A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. |
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A dual Z-scheme NiO/NiFe2O4/Fe2O3 photocatalyst is prepared via incomplete solid state chemical combustion reaction of Ni(OH)2 and Fe(OH)3. The formed perfect interfaces between NiO and NiFe2O4 and between NiFe2O4 and Fe2O3 facilitate the transfers of photo-induced electrons. The photocatalytic degradation of methylene blue and simultaneous production of hydrogen was performed to evaluate the activity of the prepared samples. The dual Z-scheme NiO/NiFe2O4/Fe2O3 (600–2) photocatalyst obtained by heat treatment of Ni(OH)2 and Fe(OH)3 at 600 °C for 2.0 h shows an excellent photocatalytic performance. Additionally, the influences of simulated sunlight irradiation time and methylene blue concentration on the photocatalytic reactions are investigated. Besides, the reusability of sample is assessed via four cycle experiments. Further, a possible mechanism on the photocatalytic reaction is proposed. Maybe, this work would provide an ingenious idea for the construction of dual Z-scheme photocatalyst and the exploration for photocatalytic degradation of organic pollutants with simultaneous hydrogen production. |
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